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Millisecond-long electron spin lifetime in CsPbI3 perovskite nanocrystals revealed by optically detected magnetic resonance

Vasilii V. Belykh, Mikhail M. Glazov, Sergey R. Meliakov, Dmitri R. Yakovlev, Evgeniya V. Kulebyakina, Mikhail L. Skorikov, Mikhail V. Kochiev, Maria S. Kuznetsova, Elena V. Kolobkova, and Manfred Bayer

Phys. Rev. B 114, 225301 (2026) - Published 1 October, 2026

Here, the authors reveal millisecond-long electron spin relaxation in CsPbI3 perovskite nanocrystals at low temperatures using the resonant spin inertia technique based on optically detected magnetic resonance. The authors uncover the role of slowly fluctuating nuclear spins in the spin relaxation at low magnetic fields and show that a two-LO-phonon Raman process governs the temperature dependence of the spin relaxation.

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Semiconductors II: surfaces, interfaces, microstructures, and related topics

Millisecond-long electron spin lifetime in CsPbI3 perovskite nanocrystals revealed by optically detected magnetic resonance

Vasilii V. Belykh, Mikhail M. Glazov, Sergey R. Meliakov, Dmitri R. Yakovlev, Evgeniya V. Kulebyakina, Mikhail L. Skorikov, Mikhail V. Kochiev, Maria S. Kuznetsova, Elena V. Kolobkova, and Manfred Bayer

Phys. Rev. B 114, 225301 (2026) - Published 1 October, 2026

Here, the authors reveal millisecond-long electron spin relaxation in CsPbI3 perovskite nanocrystals at low temperatures using the resonant spin inertia technique based on optically detected magnetic resonance. The authors uncover the role of slowly fluctuating nuclear spins in the spin relaxation at low magnetic fields and show that a two-LO-phonon Raman process governs the temperature dependence of the spin relaxation.

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