It is a fundamental prediction of quantum theory that states of physical systems are described by complex vectors or density operators on a Hilbert space. However, many experiments admit effective descriptions in terms of other state spaces, such as classical probability distributions or quantum systems with superselection rules. Which kind of effective statistics would allow us to experimentally falsify quantum theory as a fundamental description of nature? Here, we address this question by introducing a methodological principle that generalizes Spekkens’s notion of noncontextuality: Processes that are statistically indistinguishable in an effective theory should not require explanation by multiple distinguishable processes in a more fundamental theory. We formulate this principle in terms of linear embeddings and simulations of one probabilistic theory by another, show how this concept subsumes standard notions of contextuality, and prove a multitude of fundamental results on the exact and approximate embedding of theories (in particular, into quantum theory). We prove that only Jordan-algebraic state spaces are exactly embeddable into quantum theory, and show how results on Bell inequalities can be used for the certification of nonapproximate embeddability. From this, we propose an experimental test of quantum theory by probing single physical systems without assuming access to a tomographically complete set of procedures or calibration of the devices, arguably avoiding a significant loophole of earlier approaches.

We present a method for deriving bulk and edge invariants for interacting, many-body localized Floquet systems in two spatial dimensions. This method is based on a general mathematical object which we call a flow. As an application of our method, we derive bulk invariants for Floquet systems without symmetry, as well as for systems with U(1) symmetry. We also derive new formulations of previously known single-particle and many-body invariants. For bosonic systems without symmetry, our invariant gives a bulk counterpart of the rational-valued Gross-Nesme-Vogts-Werner index $p/q$ quantifying transport of quantum information along the edge.

The interaction between a mobile quantum impurity and a bosonic bath leads to the formation of quasiparticles, termed Bose polarons. The elementary properties of Bose polarons, such as their mutual interactions, can differ drastically from those of the bare impurities. Here, we explore Bose polaron physics in a two-dimensional nonequilibrium setting by injecting ${\sigma }^{-}$ polarized exciton-polariton impurities into a bath of coherent ${\sigma }^{+}$ polarized polaritons generated by resonant laser excitation of monolayer ${\mathrm{MoSe}}_2$ embedded in an optical cavity. By exploiting a biexciton Feshbach resonance between the impurity and the bath polaritons, we tune the interacting system to the strong-coupling regime and demonstrate the coexistence of two new quasiparticle branches. Using time-resolved pump-probe measurements, we observe how polaron dressing modifies the interaction between impurity polaritons. Remarkably, we find that the interactions between high-energy polaron quasiparticles, which are repulsive for small bath occupancy, can become attractive in the strong impurity-bath coupling regime. Our experiments provide the first direct measurement of Bose polaron-polaron interaction strength in any physical system and pave the way for exploration and control of many-body correlations in driven-dissipative settings.

We propose and demonstrate an architecture for fluxonium-fluxonium two-qubit gates mediated by transmon couplers (FTF, for fluxonium-transmon-fluxonium). Relative to architectures that exclusively rely on a direct coupling between fluxonium qubits, FTF enables stronger couplings for gates using noncomputational states while simultaneously suppressing the static controlled-phase entangling rate ($ZZ$) down to kilohertz levels, all without requiring strict parameter matching. Here, we implement FTF with a flux-tunable transmon coupler and demonstrate a microwave-activated controlled-$Z$ (CZ) gate whose operation frequency can be tuned over a 2-GHz range, adding frequency allocation freedom for FTFs in larger systems. Across this range, state-of-the-art CZ gate fidelities are observed over many bias points and reproduced across the two devices characterized in this work. After optimizing both the operation frequency and the gate duration, we achieve peak CZ fidelities in the 99.85%–99.9% range. Finally, we implement model-free reinforcement learning of the pulse parameters to boost the mean gate fidelity up to $99.922\%\pm 0.009\%$, averaged over roughly an hour between scheduled training runs. Beyond the microwave-activated CZ gate we present here, FTF can be applied to a variety of other fluxonium gate schemes to improve gate fidelities and passively reduce unwanted $ZZ$ interactions.

Recent years have witnessed tremendous progress in creating and manipulating ground-state ultracold polar molecules. However, the two-body loss regardless of the chemical reactivities is still a hurdle for many future explorations. Here, we investigate the loss suppression of nonreactive bosonic ${}^{23}\mathrm{Na}{}^{87}\mathrm{Rb}$ molecules with a circularly polarized microwave blue detuned to the rotational transition. We achieve suppression of the loss by 2 orders of magnitude with the lowest two-body loss rate coefficient reduced to $3\times {10}^{-12}{\mathrm{cm}}^3/\mathrm{s}$. Meanwhile, the elastic collision rate coefficient is increased to the ${10}^{-8}{\mathrm{cm}}^3/\mathrm{s}$ level. The large good-to-bad collision ratio has allowed us to carry out evaporative cooling of ${}^{23}\mathrm{Na}{}^{87}\mathrm{Rb}$ with an efficiency of 1.7(2), increasing the phase-space density by a factor of 10. With further improvements, this technique holds great promises for creating a Bose-Einstein condensate of ultracold polar molecules.

The negatively charged tin-vacancy (${\mathrm{SnV}}^{-}$) center in diamond is a promising solid-state qubit for applications in quantum networking due to its high quantum efficiency, strong zero phonon emission, and reduced sensitivity to electrical noise. The ${\mathrm{SnV}}^{-}$ has a large spin-orbit coupling, which allows for long spin lifetimes at elevated temperatures, but unfortunately suppresses the magnetic dipole transitions desired for quantum control. Here, by use of a naturally strained center, we overcome this limitation and achieve high-fidelity microwave spin control. We demonstrate a $\pi$-pulse fidelity of up to $99.51\pm 0.03\%$ and a Hahn-echo coherence time of $T_2^{\mathrm{echo}}=170.0\pm 2.8\mathrm{\mu }\mathrm{s}$, both the highest yet reported for ${\mathrm{SnV}}^{-}$ platform. This performance comes without compromise to optical stability, and is demonstrated at 1.7 K where ample cooling power is available to mitigate drive-induced heating. These results pave the way for ${\mathrm{SnV}}^{-}$ spins to be used as a building block for future quantum technologies.

We perform a systematic symmetry classification of many-body Lindblad superoperators describing general (interacting) open quantum systems coupled to a Markovian environment. Our classification is based on the behavior of the many-body Lindbladian under antiunitary symmetries and unitary involutions. We find that Hermiticity preservation reduces the number of symmetry classes, while trace preservation and complete positivity do not, and that the set of admissible classes depends on the presence of additional unitary symmetries: in their absence or in symmetry sectors containing steady states, many-body Lindbladians belong to one of ten non-Hermitian symmetry classes; if however, there are additional symmetries and we consider non-steady-state sectors, they belong to a different set of 19 classes. In both cases, it does not include classes with Kramers degeneracy. Remarkably, our classification admits a straightforward generalization to the case of non-Markovian, and even non-trace-preserving, open quantum dynamics. While the abstract classification is completely general, we then apply it to general (long-range, interacting, spatially inhomogeneous) spin-$1/2$ chains. We explicitly build examples in all ten classes of Lindbladians in steady-state sectors, describing standard physical processes such as dephasing, spin injection and absorption, and incoherent hopping, thus illustrating the relevance of our classification for practical physics applications. Finally, we show that the examples in each class display unique random-matrix correlations. To fully resolve all symmetries, we employ the combined analysis of bulk complex spacing ratios and the overlap of eigenvector pairs related by symmetry operations. We further find that statistics of levels constrained onto the real and imaginary axes or close to the origin are not universal due to spontaneous breaking of Lindbladian $PT$ symmetry.

Collisional resonances of molecules can offer a deeper understanding of interaction potentials and collision complexes, and allow control of chemical reactions. Here, we experimentally map out the spectrum of Feshbach resonances in collisions between ultracold triplet rovibrational ground-state NaLi molecules and Na atoms over a range of 1400 G. Preparation of the spin-stretched state puts the system initially into the nonreactive quartet potential. A total of 25 resonances are observed, in qualitative agreement with quantum-chemistry calculations using a coupled-channels approach. Although the theory cannot predict the positions of resonances, it can account for several experimental findings and provide unprecedented insight into the nature and couplings of ultracold, strongly interacting complexes. Previous work has addressed only weakly bound complexes. We show that the main coupling mechanism results from spin-rotation and spin-spin couplings in combination with the anisotropic atom-molecule interaction, and that the collisional complexes which support the resonances have a size of $30a_0–40a_0$. This study illustrates the potential of a combined experimental and theoretical approach.

Over the recent years, coherent, time-periodic modulation has been established as a versatile tool for realizing novel Hamiltonians. Using this approach, known as Floquet engineering, we experimentally realize a long-ranged, anisotropic Heisenberg model with tunable interactions in a trapped ion quantum simulator. We demonstrate that the spectrum of the model contains not only single-magnon excitations, but also composite magnon bound states. For long-range interactions with the experimentally realized power-law exponent, the group velocity of magnons is unbounded. Nonetheless, for sufficiently strong interactions, we observe bound states of these unconventional magnons which possess a nondiverging group velocity. By measuring the configurational mutual information between two disjoint intervals, we demonstrate the implications of bound-state formation on the entanglement dynamics of the system. Our observations provide key insights into the peculiar role of composite excitations in the nonequilibrium dynamics of quantum many-body systems.

Explaining quantum many-body dynamics is a long-held goal of physics. A rigorous operator algebraic theory of dynamics in locally interacting systems in any dimension is provided here in terms of time-dependent equilibrium (Gibbs) ensembles. The theory explains dynamics in closed, open, and time-dependent systems, provided that relevant pseudolocal quantities can be identified, and time-dependent Gibbs ensembles unify wide classes of quantum nonergodic and ergodic systems. The theory is applied to quantum many-body scars, continuous, discrete, and dissipative time crystals, Hilbert space fragmentation, lattice gauge theories, and disorder-free localization, among other cases. Novel pseudolocal classes of operators are introduced in the process: projected-local, which are local only for some states, cryptolocal, whose locality is not manifest in terms of any finite number of local densities, and transient ones, that dictate finite-time relaxation dynamics. An immediate corollary is proving saturation of the Mazur bound for the Drude weight. This proven theory is intuitively the rigorous algebraic counterpart of the weak eigenstate thermalization hypothesis and has deep implications for thermodynamics: Quantum many-body systems “out of equilibrium” are actually always in a time-dependent equilibrium state for any natural initial state. The work opens the possibility of designing novel out-of-equilibrium phases, with the newly identified scarring and fragmentation phase transitions being examples.

Continuous monitoring of driven-dissipative quantum-optical systems is a crucial element in the implementation of quantum metrology, providing essential strategies for achieving highly precise measurements beyond the classical limit. In this context, the relevant figure of merit is the quantum Fisher information of the radiation field emitted by the driven-dissipative sensor. Saturation of the corresponding precision limit as defined by the quantum Cramér-Rao bound is typically not achieved by conventional, temporally local continuous-measurement schemes such as counting or homodyning. To address the outstanding open challenge of efficient retrieval of the quantum Fisher information of the emission field, we design a novel continuous-measurement strategy featuring temporally quasilocal measurement bases as captured by matrix-product states. Such a measurement can be implemented effectively by injecting the emission field of the sensor into an auxiliary open system, a “quantum-decoder” module, which “decodes” specific input matrix-product states into simple product states as its output field, and performing conventional continuous measurement at the output. We devise a universal recipe for the construction of the decoder by exploiting the time-reversal transformation of quantum-optical input-output channels, thereby establishing a universal method to achieve the quantum Cramér-Rao precision limit for generic sensor designs based on continuous measurement. As a by-product, we establish an effective formula for the evaluation of the quantum Fisher information of the emission field of generic driven-dissipative open sensors. We illustrate the power of our scheme with paramagnetic open sensor designs including linear force sensors, fiber-interfaced nonlinear emitters, and driven-dissipative many-body sensors, and demonstrate that it can be robustly implemented under realistic experimental imperfections.

Exploring non-Hermitian phenomenology is an exciting frontier of modern physics. However, the demonstration of a non-Hermitian phenomenon that is quantum in nature has remained elusive. Here, we predict quantum non-Hermitian phenomena: the fractional quantum Zeno (FQZ) effect and FQZ-induced photon antibunching. We consider a quantum optics platform with reservoir engineering, where nonlinear emitters are coupled to a bath of decaying bosonic modes whose own decay rates form band structures. By engineering the dissipation band, the spontaneous emission of emitters can be suppressed by strong dissipation through an algebraic scaling with fractional exponents—the FQZ effect. This fractional scaling originates uniquely from the divergent dissipative density of states near the dissipation band edge, different from the traditional closed-bath context. We find FQZ-induced strong photon antibunching in the steady state of a driven emitter even for weak nonlinearities. Remarkably, we identify that the sub-Poissonian quantum statistics of photons, which has no classical analogs, stems here from the key role of non-Hermiticity. Our setup is experimentally feasible with the techniques used to design lattice models with dissipative couplings.

Understanding topological matter is an outstanding challenge across several disciplines of physical science. Programmable quantum simulators have emerged as a powerful approach to studying such systems. While quantum spin liquids of paradigmatic toric code type have recently been realized in the laboratory, controlled exploration of topological phases with non-Abelian excitations remains an open problem. We introduce and analyze a new approach to simulating topological matter based on periodic driving. Specifically, we describe a model for a so-called Floquet spin liquid, obtained through a periodic sequence of parallel quantum gate operations that effectively simulates the Hamiltonian of the non-Abelian spin liquid in Kitaev’s honeycomb model. We show that this approach, including the toolbox for preparation, control, and readout of topological states, can be efficiently implemented in state-of-the-art experimental platforms. One specific implementation scheme is based on Rydberg atom arrays and utilizes recently demonstrated coherent qubit transport combined with controlled-phase gate operations. We describe methods for probing the non-Abelian excitations, and the associated Majorana zero modes, and simulate possible fusion and braiding experiments. Our analysis demonstrates the potential of programmable quantum simulators for exploring topological phases of matter. Extensions including simulation of Kitaev materials and lattice gauge theories are also discussed.

Realizing the full potential of quantum computation requires quantum error correction (QEC), with most recent breakthrough demonstrations of QEC using the surface code. QEC codes use multiple noisy physical qubits to encode information in fewer logical qubits, enabling the identification of errors through a decoding process. This process increases the logical fidelity (or accuracy) making the computation more reliable. However, most fast (efficient run-time) decoders neglect important noise characteristics, thereby reducing their accuracy. In this work, we introduce decoders that are both fast and accurate, and can be used with a wide class of QEC codes including the surface code. Our decoders, named belief-matching and belief-find, exploit all noise information and thereby unlock higher accuracy demonstrations of QEC. Using the surface code threshold as a performance metric, we observe a threshold at 0.94% error probability for our decoders, outperforming the 0.82% threshold for a standard minimum-weight perfect matching decoder. We also test our belief-matching decoders in a theoretical case study of codes tailored to a biased noise model. We find that the decoders lead to a much higher threshold and lower qubit overhead in the tailored surface code with respect to the standard, square surface code. Surprisingly, in the well-below-threshold regime, the rectangular surface code becomes more resource efficient than the tailored surface code due to a previously unnoticed phenomenon that we call “fragile boundaries.” Our decoders outperform all other fast decoders in terms of threshold and accuracy, enabling better results in current quantum-error-correction experiments and opening up new areas for theoretical case studies.

We show how to define a quantized many-body charge polarization $\overrightarrow{𝒫}$ for $(2+1)\mathrm{D}$ topological phases of matter, even in the presence of nonzero Chern number and magnetic field. For invertible topological states, $\overrightarrow{𝒫}$ is a ${\mathbb{Z}}_2\times {\mathbb{Z}}_2$, ${\mathbb{Z}}_3$, ${\mathbb{Z}}_2$, or ${\mathbb{Z}}_1$ topological invariant in the presence of ($M=2$, 3, 4, or 6)-fold rotational symmetry, lattice (magnetic) translational symmetry, and charge conservation. $\overrightarrow{𝒫}$ manifests in the bulk of the system as (i) a fractional quantized contribution of $\overrightarrow{𝒫}·\overrightarrow{b}\text{mod}1$ to the charge bound to lattice disclinations and dislocations with Burgers vector $\overrightarrow{b}$, (ii) a linear momentum for magnetic flux, and (iii) an oscillatory system size dependent contribution to the effective 1D polarization on a cylinder. We study $\overrightarrow{𝒫}$ in lattice models of spinless free fermions in a magnetic field. We derive predictions from topological field theory, which we match to numerical calculations for the effects (i)–(iii), demonstrating that these can be used to extract $\overrightarrow{𝒫}$ from microscopic models in an intrinsically many-body way. We show how, given a high symmetry point o, there is a topological invariant, the discrete shift ${𝒮}_{\mathrm{o}}$, such that $\overrightarrow{𝒫}$ specifies the dependence of ${𝒮}_{\mathrm{o}}$ on o. We derive colored Hofstadter butterflies, corresponding to the quantized value of $\overrightarrow{𝒫}$, which further refine the colored butterflies from the Chern number and discrete shift.

We demonstrate a superconducting artificial atom with strong unidirectional coupling to a microwave photonic waveguide. Our artificial atom is realized by coupling a transmon qubit to the waveguide at two spatially separated points with time-modulated interactions. Direction-sensitive interference arising from the parametric couplings in our scheme results in a nonreciprocal response, where we measure a forward/backward ratio of spontaneous emission exceeding 100. We verify the quantum nonlinear behavior of this artificial chiral atom by measuring the resonance fluorescence spectrum under a strong resonant drive and observing well-resolved Mollow triplets. Further, we demonstrate chirality for the second transition energy of the artificial atom and control it with a pulse sequence to realize a qubit-state-dependent nonreciprocal phase on itinerant photons. Our demonstration puts forth a superconducting hardware platform for the scalable realization of several key functionalities pursued within the paradigm of chiral quantum optics, including quantum networks with all-to-all connectivity, driven-dissipative stabilization of many-body entanglement, and the generation of complex nonclassical states of light.

In 1935, Einstein, Podolsky, and Rosen (EPR) conceived a gedanken experiment which became a cornerstone of quantum technology and still challenges our understanding of reality and locality today. While the experiment has been realized with small quantum systems, a demonstration of the EPR paradox with massive many-particle systems remains an important challenge, as such systems are particularly closely tied to the concept of local realism in our everyday experience and may serve as probes for new physics at the quantum-to-classical transition. In this work we report an EPR experiment with two spatially separated Bose-Einstein condensates, each containing about 700 rubidium atoms. Entanglement between the condensates results in strong correlations of their collective spins, allowing us to demonstrate the EPR paradox between them. Our results represent the first observation of the EPR paradox with spatially separated, massive many-particle systems. They show that the conflict between quantum mechanics and local realism does not disappear as the system size increases to more than a thousand massive particles. Furthermore, EPR entanglement in conjunction with individual manipulation of the two condensates on the quantum level, as we demonstrate here, constitutes an important resource for quantum metrology and information processing with many-particle systems.

Quantum-computation architecture based on $d$-level systems, or qudits, has attracted considerable attention recently due to their enlarged Hilbert space. Extensive theoretical and experimental studies have addressed aspects of algorithms and benchmarking techniques for qudit-based quantum computation and quantum-information processing. Here, we report a physical realization of a qudit with up to four embedded levels in a superconducting transmon demonstrating high-fidelity initialization, manipulation, and simultaneous multilevel readout. In addition to constructing $\mathrm{SU}(d)$ operations and benchmarking protocols for quantum-state tomography, quantum-process tomography, randomized benchmarking, etc., we experimentally carry out these operations for $d=3$ and $d=4$. Moreover, we perform prototypical quantum algorithms and observe outcomes consistent with expectations. Our work will hopefully stimulate further research interest in developing manipulation protocols and efficient applications for quantum processors with qudits.

We study theoretically how local measurements performed on critical quantum ground states affect long-distance correlations. These states are highly entangled and feature algebraic correlations between local observables. As a consequence, local measurements can have highly nonlocal effects. Our focus is on Tomonaga-Luttinger liquid ground states, a continuous family of critical states in one dimension whose structure is characterized by a Luttinger parameter $K$. We show that arbitrarily weak local measurements, performed over extended regions of space, can conspire to drive transitions in long-distance correlations. Conditioning first on a translation-invariant set of measurement outcomes, we show that there is a transition in the character of the postmeasurement quantum state for $K<1$, and highlight a formal analogy with the effect of a static defect on transport through a Tomonaga-Luttinger liquid. To investigate the full ensemble of measurement outcomes, we consider averages of physical quantities which are necessarily nonlinear in the system density matrix. We show how their behavior can be understood within a replica field theory, and for the measurements that we consider we find that the symmetry of the theory under exchange of replicas is broken for $K<1/2$. A well-known barrier to experimentally observing the collective effects of multiple measurements has been the need to postselect on random outcomes. Here we resolve this problem by introducing cross-correlations between experimental measurement results and classical simulations, which act as resource-efficient probes of the transition. The phenomena we discuss are, moreover, robust to local decoherence.

Feedback is a powerful and ubiquitous technique both in classical and quantum system control. Its standard implementation relies on measuring the state of a system, processing the classical signal, and feeding it back to the system. In quantum physics, however, measurements not only read out the state of the system but also modify it irreversibly. Coherent feedback is a different kind of feedback that coherently processes and feeds back quantum signals without actually measuring the system. Here, we report on the experimental realization and the theoretical analysis of an optical coherent feedback platform to control the motional state of a nanomechanical membrane in an optical cavity. The coherent feedback loop consists of a light field interacting twice with the same mechanical mode through different cavity modes, without performing any measurement. Tuning the optical phase and delay of the feedback loop allows us to control the motional state of the mechanical oscillator, its resonance frequency, and also its damping rate, which we use to cool the membrane close to the quantum ground state. Our theoretical analysis provides the optimal cooling conditions, showing that this new technique enables ground-state cooling. Experimentally, we show that we can cool the membrane to a state with ${\overline{n}}_m=4.89\pm 0.14$ phonons ($480\mathrm{\mu }\mathrm{K}$) in a 20 K environment. This lies below the theoretical limit of cavity dynamical backaction cooling in the unresolved sideband regime and is achieved with only 1% of the optical power required for cavity cooling. Our feedback scheme is very versatile, offering new opportunities for quantum control in a variety of optomechanical systems.