Highlights

Dynamic response functions and helical gaps in interacting Rashba nanowires with and without magnetic fields

Christopher J. Pedder, Tobias Meng, Rakesh P. Tiwari, and Thomas L. Schmidt

Phys. Rev. B 94, 245414 (2016) - Published 12 December, 2016

One of the fundamental prerequisites for the formation of exotic anyonic bound states in superconducting quantum wires is that their normal-state band structure exhibits a so-called helical gap. Besides application of an external magnetic field, such a helical gap can also arise as a consequence of strong electron-electron interactions. The authors show that one possible realization of such an interaction-driven helical gap can be found in wires with transverse subbands and spin-orbit coupling. This state can be described in terms of quasiparticles with fractional charge e/2. These fractional charges in turn lead to important modifications of the threshold behavior of measurable dynamic response functions, such as the spectral function and the density structure factor. These experimentally accessible quantities can therefore be used to discriminate between interaction-induced helical gaps, and the more mundane gaps opened by an applied magnetic field.

Electron spin dynamics in cubic GaN

J. H. Buß, T. Schupp, D. J. As, O. Brandt, D. Hägele, and J. Rudolph

Phys. Rev. B 94, 235202 (2016) - Published 9 December, 2016

Electron spin relaxation in bulk cubic GaN is investigated by time-resolved magneto-optical spectroscopy over a wide range of temperatures, external magnetic fields, and doping densities. Very long spin relaxation times in the nanosecond range are found even up to room temperature, making cubic GaN a highly interesting material for spintronics. These results on a system with relatively weak spin-orbit coupling differ significantly from previous results for bulk III-V semiconductors such as GaAs. There are several possible reasons for the observed discrepancy, including the role of charged dislocations and a phase mixture of cubic GaN with inclusions of hexagonal GaN. Spin relaxation in such disordered materials is still poorly understood, and so this work should stimulate further research on this relevant topic.

Evolution of electronic structure of few-layer phosphorene from angle-resolved photoemission spectroscopy of black phosphorous

N. Ehlen, B. V. Senkovskiy, A. V. Fedorov, A. Perucchi, P. Di Pietro, A. Sanna, G. Profeta, L. Petaccia, and A. Grüneis

Phys. Rev. B 94, 245410 (2016) - Published 7 December, 2016

Samples of few-layer phosphorene can be produced by mechanical or liquid exfoliation. However, it remains challenging to produce flakes with large sizes. Optical spectroscopy performed on phosphorene has revealed a peculiar gap dependence that is roughly inversely proportional to the layer number. This dependence has been poorly understood to date. Because of their small size, these samples have been out of reach of powerful electronic structure characterization techniques such as angle-resolved photoemission (ARPES). The present work shows how to get a handle on the experimental band structure of few-layer black phosphorus. The authors conjecture that the bulk black phosphorous crystal already provides all the necessary information regarding the electronic structure of few-layer phosphorene. They perform ARPES measurements of the bulk crystal to fit to an experimental tight-binding model. Then, they apply the zone-folding method to the three-dimensional electronic dispersion. By quantizing the electron wavevector component perpendicular to the layers, they are able to not only extract reliable band structure data for few-layer phosphorene from the bulk band structure but also to fully explain the peculiar band-gap dependence. In particular, the band gaps as predicted by zone-folding are in excellent agreement with optical experiments and ab initio calculations.

Weyl node with random vector potential

Björn Sbierski, Kevin S. C. Decker, and Piet W. Brouwer

Phys. Rev. B 94, 220202(R) (2016) - Published 5 December, 2016

Weyl nodes, the essential low-energy theory of Weyl semimetals, are theoretically predicted to show a novel type of disorder-driven quantum phase transition. At a critical disorder strength, the system passes from a semimetal phase to a diffusive metal phase. Crucially, these theoretical predictions rest on the assumption that the disorder is of potential type, i.e., a spatially modulated energy offset for the two bands crossing at the Weyl node. However, there is no symmetry reason restricting realistic disorder to the potential case. In this Rapid Communication, the authors generalize the above setup to include generic spatially dependent couplings of the two bands, which can be interpreted as a random vector potential. Using a variety of analytical and numerical methods, the authors discover a phase diagram controlled by the number of independent components of the disorder vector. Surprisingly, no phase transition into a diffusive metal phase could be found for disorder of the single Pauli-matrix type. In contrast, all other forms of vector disorder are capable of driving a transition.

Composite Fermi liquids in the lowest Landau level

Chong Wang and T. Senthil

Phys. Rev. B 94, 245107 (2016) - Published 5 December, 2016

A quantum vortex liquid theory for composite Fermi liquid (CFL) states in the lowest Landau level is proposed. Contrary to the traditional Halperin-Lee-Read approach, the composite fermions in this formulation are vortices carrying no physical charge. Furthermore, a Berry phase ϕB=-2πν is enclosed by the composite Fermi surface, where ν is the total filling fraction. This vortex liquid theory is closely related to Read’s formulation of bosonic CFL at ν=1 in the 1990’s, and to Son’s recent formulation of the half-filled Landau level in terms of Dirac composite fermions. Various consequences of this new picture are studied, including some nontrivial predictions for transport properties, and an emergent particle-hole symmetry for bosons at ν=1.

Microscopic theory of equilibrium polariton condensates

Fei Xue, Fengcheng Wu, Ming Xie, Jung-Jung Su, and A. H. MacDonald

Phys. Rev. B 94, 235302 (2016) - Published 2 December, 2016

Exciton-polariton condensates have been realized by illuminating a microcavity system containing 2D quantum wells. When the polariton scattering rates exceed polariton lifetimes, the polariton condensate states can be described microscopically using equilibrium statistical mechanics. This work describes a fully microscopic mean-field theory of equilibrium polariton condensates that treats quantum well band states explicitly and goes beyond the commonly used model in which excitons are treated as Bose particles that are coupled to cavity photons. The authors compare their results with the predictions of simplified bosonic theory, and explain the quantitative differences in condensate properties. Their theory predicts that effective polariton-polariton interaction strengths are weaker and that exciton-fractions in the condensate are smaller than in the simplified exciton-photon model, and that the effective Rabi coupling strengths depends on detuning. The quasiparticle bands that appear in their theory are dressed by both electron-electron and electron-photon interactions, with the electron-electron contribution dominating even when the photon fraction of the condensate is relatively large. The properties of the dressed bands suggest novel mechanisms for the electrical manipulation of polariton condensates.

Emergence of an excitonic collective mode in the dilute electron gas

Yasutami Takada

Phys. Rev. B 94, 245106 (2016) - Published 2 December, 2016

In the early 1950s, Bohm and Pines (BP) developed the random-phase approximation (RPA) theory and revealed the plasmon as an emergent collective mode in metals. In this paper, for the first time ever since the original BP theory, a novel collective mode is predicted to emerge in the dilute electron liquid. The electronic compressibility of this mode is negative and thus dielectric catastrophe appears, predicted by a theory that goes far beyond RPA and fully satisfies various sum rules, constraints, and asymptotic behavior. While the plasmon occurs by the coherent excitations of mutually uncorrelated electrons and holes, the new mode is associated with the excitations of a large collection of excitons (or tightly bound electron-hole pairs). Mathematically, this excitonic collective mode is intimately connected with a newly discovered singularity in the dielectric function in the electron liquid. This collective mode should add a new dimension to plasmonics in nanotechnology in the future.

Many-terminal Majorana island: From topological to multichannel Kondo model

Loïc Herviou, Karyn Le Hur, and Christophe Mora

Phys. Rev. B 94, 235102 (2016) - Published 1 December, 2016

The Kondo effect refers to a localized spin impurity that is screened by conduction electrons at low temperatures, leading to entanglement and nontrivial transport properties. Connecting zero-energy Majorana bound states of a charge-quantized superconducting island to M normal metallic leads realizes exotic SO(M) Kondo models with mesoscopic systems. In the Coulomb-blockade regime, the Majorana fermions lead to a family of non-Fermi-liquid fixed points and symmetric correlated transport between the leads, dubbed the topological Kondo effect (TKE). This work brings light to the resonant limit, where the charging energy selects two consecutive macroscopic charge states. The interplay between the charge states and the Majorana fermions allows for an exact mapping to the interacting multichannel Kondo model (MCKM). The quantum Brownian motion analogy proves the existence of a continuously varying line of fixed points between the MCKM and the TKE, characterized by fractional conductance, depending on the electron-electron interactions in the leads.

Magnetic structures and excitations in a multiferroic Y-type hexaferrite BaSrCo2Fe11AlO22

Taro Nakajima, Yusuke Tokunaga, Masaaki Matsuda, Sachith Dissanayake, Jaime Fernandez-Baca, Kazuhisa Kakurai, Yasujiro Taguchi, Yoshinori Tokura, and Taka-hisa Arima

Phys. Rev. B 94, 195154 (2016) - Published 30 November, 2016

Multiferroic hexaferrites have been extensively investigated because they exhibit ferroelectricity associated with noncollinear magnetic orders in relatively low magnetic field and high temperature regions. To understand the static and dynamical spin-polarization coupling in such systems, it is necessary to determine the magnetic structures and spin-wave modes. This is impossible for polycrystalline samples. Here, the authors have successfully grown single crystals of BaSrCo2Fe12AlO22 by means of a laser floating zone technique. They perform magnetization, electric polarization, and neutron diffraction measurements to establish the magnetic phase diagram. Several interesting features are seen and the new understanding should provide a useful guide for developing multiferroic-based functional devices working at room temperature.

Transparency of graphene and other direct-gap two-dimensional materials

Daniel J. Merthe and Vitaly V. Kresin

Phys. Rev. B 94, 205439 (2016) - Published 30 November, 2016

The optical properties of graphene are among its remarkable characteristics. Measurements have found that the opacity of a single graphene layer for infrared and visible light is simply equal to π times the fine-structure constant. Explanations of this beautiful relation have tended to view it as a consequence of the material’s Dirac-like band structure. However, in this paper the authors emphasize that the interband absorption rate must be treated by using the underlying nonrelativistic Hamiltonian, not the quasimomentum state label of the bands. They employ both a straightforward model and a tight-binding calculation to show that the opacity of graphene follows not from its celebrated linear dispersion relation but from the fact that it is a two-dimensional material. The same characteristic is therefore present in semiconductor membranes (as revealed by recent experiments) and other two-dimensional systems. This work focuses attention on the universality that reduced dimensionality bestows on optical absorption.

Direct observation of anisotropic magnetic field response of the spin helix in FeGe thin films

N. Kanazawa, J. S. White, H. M. Rønnow, C. D. Dewhurst, Y. Fujishiro, A. Tsukazaki, Y. Kozuka, M. Kawasaki, M. Ichikawa, F. Kagawa, and Y. Tokura

Phys. Rev. B 94, 184432 (2016) - Published 28 November, 2016

Spiral spin orders often produce various fascinating phenomena via interaction with electronic structures. Examples include, but are not limited to, multiferroicity and skyrmion formation. Among them, a deformed spiral spin structure, which can be viewed as a periodic sequence of 2π spin-rotation kinks, can exhibit the functionality of information transmission owing to its phase coherence. This is the chiral magnetic soliton lattice (CSL). Here, the authors have succeeded in building a spin spiral in a thin film of the chiral magnet FeGe, and revealed its characteristic magnetic responses. Magnetic anisotropy and boundary conditions inherent to the epitaxial thin film secure the alignment of the spiral winding direction along the film normal, even under external magnetic fields. This constraint leads to the anisotropic deformation of the spin spiral with respect to the magnetic field direction. Especially, the CSL, which is realized under an in-plane magnetic field, transforms with field between states with different numbers of kinks. The authors clearly demonstrate the deformation by direct observation of the spiral propagation vector by use of the small-angle neutron scattering technique.

Direct observation of charge order in underdoped and optimally doped Bi2(Sr,La)2CuO6+δ by resonant inelastic x-ray scattering

Y. Y. Peng, M. Salluzzo, X. Sun, A. Ponti, D. Betto, A. M. Ferretti, F. Fumagalli, K. Kummer, M. Le Tacon, X. J. Zhou, N. B. Brookes, L. Braicovich, and G. Ghiringhelli

Phys. Rev. B 94, 184511 (2016) - Published 28 November, 2016

The already overcrowded phase diagram of cuprate superconductors has recently accommodated a region characterized by incommensurate charge density waves (CDW), partly overlapping with superconductivity, and included in the pseudogap regime. Although charge order is strengthened by high magnetic fields and competes with superconductivity, its role in Cooper pairing is still unassessed, calling for more complete characterization in different families of cuprates. The authors present an extensive x-ray scattering study of charge order in single layer La-doped Bi2201, and they show it extends up to optimal-doping (OP33K, p=0.16) in this family too. The CDW peak sharpens at Tc and disappears above the pseudogap onset at temperature T*. They also demonstrate that in the underdoped sample (OD15K, p=0.115) the charge density wave has no out-of-plane correlation and has dominant unidirectional nature within the planes.

The “parity” anomaly on an unorientable manifold

Edward Witten

Phys. Rev. B 94, 195150 (2016) - Published 28 November, 2016

The “parity” anomaly is a potential violation of time-reversal and reflection symmetry that can occur for relativistic fermions coupled to gauge fields and/or gravity in 2+1 dimensional spacetime. It has played a role in condensed matter physics since the work of Haldane and others in the 1980’s. Only recently, as a result of developments in the theory of topological superconductors, has it been understood that the extension of this anomaly to an unorientable spacetime is significant. In the present paper, a systematic description is given of the “parity” anomaly on an unorientable spacetime. This is used to get a fuller understanding of gapped symmetry-preserving boundary states of a topological superconductor and to resolve some questions about the world-volume path integral of M-theory membranes.

Slow light and slow acoustic phonons in optophononic resonators

V. Villafañe, P. Soubelet, A. E. Bruchhausen, N. D. Lanzillotti-Kimura, B. Jusserand, A. Lemaître, and A. Fainstein

Phys. Rev. B 94, 205308 (2016) - Published 28 November, 2016

Slow light has been exploited in optoelectronics to enhance the light-matter interaction, including light absorption and emission, nonlinear processes such as sum-frequency generation and phase modulation, and lasing. Modulated structures that modify the propagation of light can also be tailored to alter the propagation of sound. The question then arises: how can slow high-frequency acoustic waves and slow light in the same device perform with a perspective in optomechanics? This question becomes particularly relevant in view of recent reports of photon lifetimes extended to the millisecond range (lifetimes that are characteristic of phonons) by introducing slow-light effects in microresonators. With this application in mind, this work studies DBR-based GaAs/AlAs microcavities as structures that present both light confinement and slowing-down, depending on whether the laser is tuned resonantly to the cavity or stop-band edge modes. Interestingly, the authors show that for these kind of devices precisely the same happens for acoustic phonons, thus providing a rich playground to investigate confined and slow optomechanical effects. Time-resolved coherent phonon generation experiments using picosecond lasers are reported, showing a strong enhancement of the optomechanical coupling using both confined and also properly designed slow photon and phonon modes. The prospects for the use of these optoelectronic devices in confined and slow optomechanics is addressed.

Roadmap to Majorana surface codes

S. Plugge, L. A. Landau, E. Sela, A. Altland, K. Flensberg, and R. Egger

Phys. Rev. B 94, 174514 (2016) - Published 23 November, 2016

Surface codes represent a promising route towards universal fault-tolerant quantum computation, allowing for the protection of stored quantum states against many types of errors. This theoretical work shows that, in addition, a significantly enhanced versatility in quantum information processing is expected when qubits are encoded into the Majorana bound states in topological superconductor-semiconductor heterostructures. In view of recent experimental evidence for Majorana states in such heterostructures, a two-dimensional network of interacting Majorana states thus may feature key advantages towards the long-term goal of a functional quantum computer. The authors discuss how topologically protected logical qubits in this Majorana surface code architecture can be defined, initialized, manipulated, and read out. The physical ingredients needed to implement such operations are familiar from topologically trivial quantum devices. In particular, by employing quantum interference terms in conductance measurements, composite single-electron pumping protocols, and gate-tunable tunnel barriers, the full set of gates required for universal quantum computation can be implemented.

Fermi surface evolution of Na-doped PbTe studied through density functional theory calculations and Shubnikov–de Haas measurements

P. Giraldo-Gallo, B. Sangiorgio, P. Walmsley, H. J. Silverstein, M. Fechner, S. C. Riggs, T. H. Geballe, N. A. Spaldin, and I. R. Fisher

Phys. Rev. B 94, 195141 (2016) - Published 23 November, 2016

Lead telluride (PbTe) is a widely known thermoelectric material and a narrow-gap semiconductor. The introduction of impurity dopants in this compound has shown to significantly increase the thermoelectric figure of merit, and for certain dopants, to even lead the material to a superconducting ground state. Understanding the physical origin of these enhanced properties and their dependence on the choice of dopant chemistry requires a detailed knowledge of the electronic structure, in particular its evolution with carrier concentrations. With this in mind, the authors of this paper present a combined experimental and first-principles study of the evolution of the low-temperature Fermi surface of Na-doped PbTe. Their Shubnikov–de Haas measurements allowed the determination of the full morphology of the Fermi surface for hole concentrations one order of magnitude higher than other previous studies in this material, showing that the band dispersion is consistent with a nonparabolic single-band Kane-model dispersion, in which the hole-pockets are ellipsoids of fixed anisotropy throughout the band, but the effective masses depend strongly on Fermi energy. Additionally, the authors show that standard density functional calculations underestimate the energy difference between the first two valence-band maxima, since their experimental data is consistent with a single-band Fermi surface over the entire doping range studied.

Ultrafast terahertz-field-driven ionic response in ferroelectric BaTiO3

F. Chen et al.

Phys. Rev. B 94, 180104(R) (2016) - Published 22 November, 2016

Ferroelectric materials encode information through the displacement of atoms within the unit cell, but the ultimate speed limits governing how fast the polarization can change and how it responds to electric fields remain largely unknown. These processes in turn fundamentally determine the functionality of ferroelectric materials within devices. Here, the authors show that single-cycle light pulses at terahertz frequencies can be used as an ultrafast electric field to drive large amplitude rotations of the ferroelectric polarization on picosecond time scales within the prototypical ferroelectric BaTiO3, probed by femtosecond x-ray scattering to directly resolve the motions of the atoms. These measurements are connected directly to first-principles molecular dynamics simulations of ultrafast electric-field-driven effects in ferroelectrics with good agreement obtained between experiment and theory.

Enhancing interfacial magnetization with a ferroelectric

Tricia L. Meyer, Andreas Herklotz, Valeria Lauter, John W. Freeland, John Nichols, Er-Jia Guo, Shinbuhm Lee, T. Zac Ward, Nina Balke, Sergei V. Kalinin, Michael R. Fitzsimmons, and Ho Nyung Lee

Phys. Rev. B 94, 174432 (2016) - Published 21 November, 2016

Ferroelectric control of the electronic and magnetic properties of a correlated oxide provides new opportunities for fundamental science and practical device applications. However, the exploding interest in ferroelectric control of magnetic interfaces, which typically happens in a few nanometers, has been inhibited by the lack of appropriate characterization techniques. Here, the authors have used polarized neutron reflectivity (PNR), a nondestructive yet powerful technique, to directly probe the evolution of the interfacial magnetism at the interface between ferromagnetic La0.8Sr0.2MnO3 and ferroelectric PbZr0.2Ti0.8O3. Using PNR, the authors find that the orientation of the ferroelectric polarization of the ferroelectric layer critically determines the interfacial magnetism, which occurs within a few nanometers of the interface. When the polarization is oriented towards the manganite layer, it is capable of enhancing the interfacial magnetization above the bulk region of the film. This finding not only proves the ferroelectric field effect control of magnetism, but also emphasizes the necessity of separating bulk properties from interfacial phenomena in magnetoelectric materials.

Revisiting the ground state of CoAl2O4: Comparison to the conventional antiferromagnet MnAl2O4

G. J. MacDougall, A. A. Aczel, Yixi Su, W. Schweika, E. Faulhaber, A. Schneidewind, A. D. Christianson, J. L. Zarestky, H. D. Zhou, D. Mandrus, and S. E. Nagler

Phys. Rev. B 94, 184422 (2016) - Published 17 November, 2016

The spinel aluminates (AAl2O4) are physical realizations of the diamond-lattice antiferromagnet, a model system wherein competing nearest- (J1) and next-nearest- (J2) exchange interactions frustrate order and can lead to novel magnetic ground states, including a “spiral spin liquid” (SSL). CoAl2O4 has been studied intensely as a SSL candidate, and exhibits unusual low-temperature short-range correlations that have been interpreted as arising from unconventional spin-glass behavior or antiferromagnetism, possibly with SSL correlations, but with no clear consensus to date. It has been suggested that the tendency towards “cation inversion” disorder inhibits long-range order. Here, the authors provide a comparative neutron scattering study of single crystals of the two spinel aluminates CoAl2O4 and MnAl2O4. Despite the fact that MnAl2O4 has greater cation inversion, it clearly behaves as a classical Néel antiferromagnet. In contrast, CoAl2O4 exhibits a freezing transition at T* = 6.5 K into a phase characterized by finite-sized domains separated by a series of sharp walls. The results are consistent with kinetically inhibited domain growth, which can arise naturally in a frustrated magnet containing a first-order phase transition. The ratio J2/J1 is close to the value where theory predicts such a transition. The contrast with MnAl2O4 shows that frustration arising from competing interactions, and not disorder, is the driving factor in determining the low-temperature magnetic state in CoAl2O4.

Hierarchical quantum master equation approach to electronic-vibrational coupling in nonequilibrium transport through nanosystems

C. Schinabeck, A. Erpenbeck, R. Härtle, and M. Thoss

Phys. Rev. B 94, 201407(R) (2016) - Published 15 November, 2016

Quantum transport in nanosystems is often characterized by strong coupling between electronic and vibrational degrees of freedom. Examples include single-molecule junctions, nanoelectromechanical systems, and suspended carbon nanotubes. Electronic-vibrational coupling manifests itself in vibronic structures in the transport characteristics and results in a multitude of nonequilibrium phenomena, such as current-induced local heating and cooling, multistability, switching, hysteresis, and decoherence. The theoretical study of quantum transport, in particular in the strong-coupling regime, requires nonperturbative approaches that can be systematically converged, i.e., numerically exact methods. In this work, the authors outline how the hierarchical quantum master equation approach, which generalizes perturbative master equation methods by including higher-order contributions as well as non-Markovian memory, can be used in this context. The results show that vibrational nonequilibrium effects are important in a broad spectrum of scenarios, which range from the nonadiabatic to the adiabatic regime and include both resonant and off-resonant transport.

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