Analog quantum simulators, which efficiently represent model systems, have the potential to provide new insight toward naturally occurring phenomena beyond the capabilities of classical computers. Incorporating dissipation as a resource unlocks a wider range of out-of-equilibrium processes such as chemical reactions. Here, we operate a hybrid qubit-oscillator circuit quantum electrodynamics simulator and model nonadiabatic molecular dynamics through a conical intersection. We identify dephasing of the electronic qubit as the mechanism that drives wave-packet branching when the corresponding oscillator undergoes large amplitude motion. Furthermore, we directly observe enhanced branching when the wave-packet passes through the conical intersection. Thus, the forces that influence a chemical reaction can be viewed from the perspective of measurement backaction in quantum mechanics—there is an effective measurement-induced dephasing rate that depends on the position of the wave packet relative to the conical intersection. Our results set the groundwork for more complex simulations of chemical dynamics using quantum simulators, offering deeper insight into the role of dissipation in determining macroscopic quantities of interest such as the quantum yield of a chemical reaction.

Competing and intertwined orders including inhomogeneous patterns of spin and charge are observed in many correlated electron materials, such as high-temperature superconductors. Introducing a new development of the constrained-path auxiliary-field quantum Monte Carlo method, we study the interplay between thermal and quantum fluctuations in the two-dimensional Hubbard model. We obtain an accurate and systematic characterization of the evolution of the spin and charge correlations as a function of temperature $T$ and how it connects to the ground state, at three representative hole doping levels $\delta =1/5$, $1/8$, and $1/10$. We find increasing short-range commensurate antiferromagnetic correlations as $T$ is lowered. As the correlation length grows sufficiently large, a modulated spin-density wave (SDW) appears. At $\delta =1/5$ and $U/t=6$, the SDW saturates and remains short-ranged as $T\to 0$. In contrast, at $\delta =1/8$, $1/10$ and $U/t=8$, this evolves into a ground-state stripe phase. We study the relation between spin and charge orders and find that formation of charge order appears to be driven by that of the spin order. We identify a finite-temperature phase transition below which charge ordering sets in and discuss the implications of our results for the nature of this transition.

The distant projection of high-peak and average-power laser beams in the atmosphere is a long-standing goal with a wide range of applications. Our early proof-of-principle experiments [Phys. Rev. X 4, 011027 (2014)] presented one solution to this problem, employing the energy deposition of femtosecond filaments in air to sculpt millisecond-lifetime sub-meter-length air waveguides. Here, we demonstrate air waveguiding at the 50-m scale, $60\times \text{longer}$, making many practical applications now possible. We employ a new method for filament energy deposition: multifilamentation of Laguerre-Gaussian ${\mathrm{LG}}_{01}$ “donut” modes. We first investigate the detailed physics of this scheme over a shorter 8-m in-lab propagation range corresponding to 13 Rayleigh lengths of the guided pulse. We then use these results to demonstrate optical guiding over 45 m in the hallway adjacent to the lab, corresponding to 70 Rayleigh lengths. Injection of a continuous-wave probe beam into these waveguides demonstrates very long lifetimes of tens of milliseconds.

Color centers are point defects in crystals that can provide an optical interface to a long-lived spin state for distributed quantum information processing applications. An outstanding challenge for color center quantum technologies is the integration of optically coherent emitters into scalable thin-film photonics, a prerequisite for large-scale photonics integration of color centers within a commercial foundry process. Here, we report on the integration of near-transform-limited silicon vacancy (${\mathrm{V}}_{\mathrm{Si}}$) defects into microdisk resonators fabricated in a CMOS-compatible $4H$-silicon carbide-on-insulator platform. We demonstrate a single-emitter cooperativity of up to 0.8 as well as optical superradiance from a pair of color centers coupled to the same cavity mode. We investigate the effect of multimode interference on the photon scattering dynamics from this multiemitter cavity quantum electrodynamics system. These results are crucial for the development of quantum networks in silicon carbide and bridge the classical-quantum photonics gap by uniting optically coherent spin defects with wafer-scalable, state-of-the-art photonics.

Quantum networks play an indispensable role in quantum information tasks such as secure communications, enhanced quantum sensing, and distributed computing. Among the most mature and promising platforms for quantum networking are nitrogen-vacancy (NV) centers in diamond and other color centers in solids. One of the challenges in using these systems for networking applications is to controllably manipulate entanglement between the electron and the nuclear spin register despite the always-on nature of the hyperfine interactions, which makes this an inherently many-body quantum system. Here, we develop a general formalism to quantify and control the generation of entanglement in an arbitrarily large nuclear spin register coupled to a color center electronic spin. We provide a reliable measure of nuclear spin selectivity, by exactly incorporating into our treatment the dynamics with unwanted nuclei. We also show how to realize direct multipartite gates through the use of dynamical decoupling sequences, drastically reducing the total gate time compared to protocols based on sequential entanglement with individual nuclear spins. We quantify the performance of such gate operations in the presence of unwanted residual entanglement links, capturing the dynamics of the entire nuclear spin register. Finally, using experimental parameters of a well-characterized 27 nuclear spin register device, we show how to prepare with high-fidelity entangled states for quantum error correction. While in this analysis we focus on a particular NV-diamond-based register, our framework is completely general and applicable to other defects in diamond and in SiC.

With recent advances in time-resolved device control, the dynamical engineering of novel quantum phases is becoming reality. One of the striking new options is the dynamical generation of space-synthetic dimensions, transcending the confines of static crystalline solid-state physics. We apply this principle to propose protocols allowing for the engineered realization of topological surface states in isolation. As a concrete example, we consider $3\mathrm{D}$ topological surface states of a $4\mathrm{D}$ quantum Hall insulator via a $(1+2_{\mathrm{syn}})$-dimensional protocol. We present first-principle analytical calculations demonstrating that no supporting $4\mathrm{D}$ bulk phase is required for a $3\mathrm{D}$ topological surface phase. We back the analytical approach by numerical simulations and present a detailed blueprint for the realization of the synthetic surface phase with existing quantum linear optical network device technology. We then discuss generalizations, including a proposal for a quantum simulator of the $(1+1_{\mathrm{syn}})$-dimensional surface of the common $3\mathrm{D}$ topological insulator.

For over 80 years of research, the conventional description of free-electron radiation phenomena, such as Cherenkov radiation, has remained unchanged: classical three-dimensional electromagnetic waves. Interestingly, in reduced dimensionality, the properties of free-electron radiation are predicted to fundamentally change. Here, we present the first observation of Cherenkov surface waves, wherein free electrons emit narrow-bandwidth photonic quasiparticles propagating in two dimensions. The low dimensionality and narrow bandwidth of the effect enable us to identify quantized emission events through electron energy loss spectroscopy. Our results support the recent theoretical prediction that free electrons do not always emit classical light and can instead become entangled with the photons they emit. The two-dimensional Cherenkov interaction achieves quantum coupling strengths over 2 orders of magnitude larger than ever reported, reaching the single-electron–single-photon interaction regime for the first time with free electrons. Our findings pave the way to previously unexplored phenomena in free-electron quantum optics, facilitating bright, free-electron-based quantum emitters of heralded Fock states.

Intense debate has recently arisen regarding the photoinduced changes to the iron-chalcogenide superconductors, including the enhancement of superconductivity and a metastable state. Here, by employing high-energy resolution, we directly observe the melting of superconductivity on ultrafast timescales. We demonstrate a distinctly nonequilibrium response on short timescales, where the gap fills in prior to the destruction of the superconducting peak, followed by a metastable response. We propose that the former is due to pair phase decoherence and speculate that the latter is due to the increase in double-stripe correlations that are known to compete with superconductivity. Our results add to exciting new developments on the iron-based superconductors, indicating that the photoinduced metastable state possibly competes with superconductivity.

Phase separation of biomolecules gives rise to membraneless organelles that contribute to the spatiotemporal organization of the cell. In most cases, such biomolecular condensates contain multiple components, but the manner in which interactions between components control the stability of condensates have remained challenging to elucidate. Here, we develop an approach to determine tie-line gradients in ternary biomolecular phase-separation systems based on measurements of the dilute phase concentration of only one component. We show that the sign of the tie-line gradient is related to the cross-interaction energy between the polymers in the system and discriminates between associative and segregative phase separation. Using this approach, we study the interaction between protein fused in sarcoma (FUS) and polyethylene glycol (PEG) polymer chains and measure positive tie-line gradients. Our results show that PEG drives phase separation through an associative interaction with FUS, other than through acting as an inert crowder. We further study the interaction between poly(A) ribonucleic acid (RNA) ($\text{700}–\text{3500\hspace{0.17em}\hspace{0.17em}}\mathrm{kDa}$ [kilodalton]) and the protein G3BP1, and using the tie-line gradient as a reporter for the stoichiometry of polymers in the condensate, we determine a G3BP1-to-poly(A) RNA molar ratio of $1:0.003–0.015$ in the dense phase. Our framework for measuring tie-line gradients opens up a route for the characterization of interaction types and compositions in ternary phase-separation systems.

Persistent currents in annular geometries have played an important role in disclosing the quantum phase coherence of superconductors and mesoscopic electronic systems. Ultracold atomic gases in multiply connected traps also exhibit long-lived supercurrents and have attracted much interest both for fundamental studies of superfluid dynamics and as prototypes for atomtronics circuits. Here, we report on the realization of supercurrents in homogeneous, tunable fermionic rings. We gain exquisite, rapid control over quantized persistent currents in all regimes of the BCS-BEC crossover through a universal phase-imprinting technique, attaining on-demand circulations $w$ as high as 9. High-fidelity readout of the superfluid circulation state is achieved by exploiting an interferometric protocol, which also yields local information about the superfluid phase around the ring. In the absence of externally introduced perturbations, we find the induced metastable supercurrents to be as long-lived as the atomic sample. Conversely, we trigger and inspect the supercurrent decay by inserting a single small obstacle within the ring. For circulations higher than a critical value, the quantized current is observed to dissipate via the emission of vortices, i.e., quantized phase slips, which we directly image, in good agreement with numerical simulations. The critical circulation at which the superflow becomes unstable is found to depend starkly on the interaction strength, taking its maximum value for the unitary Fermi gas. Our results demonstrate fast and accurate control of quantized collective excitations in a macroscopic quantum system and establish strongly interacting fermionic superfluids as excellent candidates for atomtronics applications.

Extreme ultraviolet light delivering radiation with a wavelength shorter than approximately 100 nm is now available from solid-state sources. However, despite exceptional progress, efficient focusing of extreme ultraviolet photons to their ultimate diffraction limit remains a formidable challenge because of the precision of the focusing by curved, optical surfaces. Here we integrate coherent short-wavelength high-order harmonics from a MgO crystal, with a high-numerical-aperture, nanostructured, focusing element etched onto the surface of the crystal itself. We focus extreme ultraviolet light, seventh harmonic of an 800-nm laser, with a zone plate of numerical aperture 0.35, down to a waist radius of 150 nm, with 18% focusing efficiency. The estimated intensity approaches ${10}^7\mathrm{W}/{\mathrm{cm}}^2$. Future developments may demonstrate nanoscale laser ablation and miniaturization of extreme ultraviolet coherent sources on a chip.

Tensor-network (TN) states are efficient parametric representations of ground states of local quantum Hamiltonians extensively used in numerical simulations. Employing TN Ansatz states directly on a quantum simulator can potentially offer an exponential computational advantage over purely numerical simulation. We implement a quantum-encoded TN Ansatz state using a variational quantum eigensolver on an ion-trap quantum computer that approximates the ground states of the extended Su-Schrieffer-Heeger model. The generated states are characterized by estimating the topological invariants, verifying their topological order. Our TN encoding as a trapped-ion circuit employs only single-site optical pulses—the native operations naturally available on the platform. We reduce nearest-neighbor crosstalk by selecting different magnetic sublevels with well-separated transition frequencies to encode the qubits in neighboring ions.

Electronic properties of superatomic crystals have not been sufficiently explored due to the versatility of their building units; moreover, their interunit couplings are even poorly understood. Here, we present a joint experiment-theory investigation of a rationally designed layered superatomic crystal of ${\mathrm{Au}}_6{\mathrm{Te}}_{12}{\mathrm{Se}}_8$ (ATS) cubes stacked by noncovalent intercube quasibonds. We find a sequential-emerged anisotropic triple-cube charge density wave (TCCDW) and polarized metallic states below 120 K, as revealed via scanning tunneling microscopy and spectroscopy, angle-resolved photoemission spectroscopy, transport measurement, Raman spectra, and density-functional theory. The polarized states are locked in an antiparallel configuration, which is required for maintaining the inversion symmetry of the center cube in the TCCDW. The antipolar metallic states are thus interweaved by the CDW and the polarized metallic states, and primarily ascribed to electronic effects via theoretical calculations. This work not only demonstrates a microscopic picture of the interweaved CDW and polarized charge orders in the superatomic crystal of ATS, but also sheds light on expanding the existing category of quantum materials to noncovalent solids.

The large-scale organization of the genome inside the cell nucleus is critical for the cell’s function. Chromatin—the functional form of DNA in cells—serves as a template for active nuclear processes such as transcription, replication, and DNA repair. Chromatin’s spatial organization directly affects its accessibility by ATP-powered enzymes, e.g., RNA polymerase II in the case of transcription. In differentiated cells, chromatin is spatially segregated into compartments—euchromatin and heterochromatin—the former being largely transcriptionally active and loosely packed, the latter containing mostly silent genes and densely compacted. The euchromatin-heterochromatin segregation is crucial for proper genomic function, yet the physical principles behind it are far from understood. Here, we model the nucleus as filled with hydrodynamically interacting active Zimm chains—chromosomes—and investigate how large heterochromatic regions form and segregate from euchromatin through their complex interactions. Each chromosome presents a block copolymer composed of heterochromatic blocks, capable of cross-linking that increases chromatin’s local compaction, and euchromatic blocks, subjected to stochastic force dipoles that capture the microscopic stresses exerted by nuclear ATPases. These active stresses lead to a dynamic self-organization of the genome, with its coherent motions driving some mixing of chromosome territories as well as large-scale heterochromatic segregation through cross-linking of distant genomic regions. We study the stresses and flows that arise in the nucleus during the heterochromatic segregation and identify their signatures in Hi-C proximity maps. Our results reveal the fundamental role of active mechanical processes and hydrodynamic interactions in the kinetics of chromatin compartmentalization and in the emergent large-scale organization of the nucleus.

The relationship between many-body interactions and dimensionality is integral to numerous emergent quantum phenomena. A striking example is the Bose gas, which upon confinement to one dimension (1D) obeys an infinite set of conservation laws, prohibiting thermalization and constraining dynamics. In our experiment, we demonstrate that such a 1D behavior can extend much further into the dimensional crossover toward 3D than expected. Starting from a weakly interacting Bose gas trapped in a highly elongated potential, we perform a quench to instigate the dynamics of a single density mode. Employing the theory of generalized hydrodynamics, we identify the dominant relaxation mechanism as the 1D dephasing of the relevant collective excitations of the system, the rapidities. Surprisingly, the dephasing remains dominant even for temperatures far exceeding conventional limits of one dimensionality where thermalization should occur. We attribute our observations to an emergent Pauli blocking of transverse excitations caused by the rapidities assuming fermionic statistics, despite the gas being purely bosonic. Thus, our study suggests that 1D physics is less fragile than previously thought, as it can persist even in the presence of significant perturbations. More broadly, by employing the exact Bethe ansatz solutions of the many-body system, we facilitate an interpretation of how the emergent macroscopic behavior arises from the microscopic interactions.

Because electrons and ions form a coupled system, it is a priori clear that the dynamics of the lattice should reflect symmetry breaking within the electronic degrees of freedom. Recently, this has been clearly evidenced for the case of time-reversal and mirror symmetry breaking by observations of a large phononic thermal Hall effect in many strongly correlated electronic materials. However, the mechanism by which time-reversal breaking and chirality is communicated to the lattice is far from evident. In this paper, we discuss how this occurs via many-body scattering of phonons by collective modes: a consequence of non-Gaussian correlations of the latter modes. We derive fundamental new results for such skew (i.e., chiral) scattering and the consequent thermal Hall conductivity. We emphasize that these results apply to any collective variables in any phase of matter: electronic, magnetic, or neither; highly fluctuating and correlated, or not. As a proof of principle, we compute general formulas for the above quantities for ordered antiferromagnets. From the latter, we obtain the scaling behavior of the phonon thermal Hall effect in clean antiferromagnets. The calculations show several different regimes and give quantitative estimates of similar order to that seen in recent experiments.

Exotic magnetic textures emerging from the subtle interplay between thermodynamic and topological fluctuation have attracted intense interest due to their potential applications in spintronic devices. Recent advances in electron microscopy enable the imaging of random photogenerated individual skyrmions. However, their deterministic and dynamical manipulation is hampered by the chaotic nature of such fluctuations and the intrinsically irreversible switching between different minima in the magnetic energy landscape. Here, we demonstrate a method to coherently control the rotation of a skyrmion crystal by discrete amounts at speeds which are much faster than previously observed. By employing circularly polarized femtosecond laser pulses with an energy below the band gap of the Mott insulator ${\mathrm{Cu}}_2{\mathrm{OSeO}}_3$, we excite a collective magnon mode via the inverse Faraday effect. This triggers coherent magnetic oscillations that directly control the rotation of a skyrmion crystal imaged by cryo-Lorentz transmission electron microscopy. The manipulation of topological order via ultrafast laser pulses shown here can be used to engineer fast spin-based logical devices.

The exploration of quantum spin liquids (QSLs) has been guided by different approaches including the resonating valence bond (RVB) picture, deconfined lattice gauge theories, and the Kitaev model. More recently, a spin-liquid ground state was numerically established on the ruby lattice, inspired by the Rydberg blockade mechanism. Here, we unify these varied approaches in a single parent Hamiltonian, in which local fluctuations of anyons stabilize deconfinement. The parent Hamiltonian is defined on kagomé triangles—each hosting four RVB-like states—and includes only Ising interactions and single-site transverse fields. In the weak-field limit, the ruby spin liquid and exactly soluble kagomé dimer models are recovered, while the strong-field limit reduces to the Kitaev honeycomb model, thereby unifying three seemingly different approaches to QSLs. We similarly obtain the chiral Yao-Kivelson model, the honeycomb toric code, and a new spin-1 quadrupolar Kitaev model. The last is shown to be in a QSL phase by a nonlocal mapping to the kagomé Ising antiferromagnet. We demonstrate various applications of our framework, including (a) an adiabatic deformation of the ruby lattice model to the exactly soluble kagomé dimer model, conclusively establishing the QSL phase in the former and (b) demystifying the dynamical protocol for measuring off-diagonal strings in the Rydberg implementation of the ruby lattice spin liquid. More generally, we find an intimate connection between Kitaev couplings and the repulsive interactions used for emergent dimer models. For instance, we show how a spin-$1/2$ $XXZ$ model on the ruby lattice encodes a Kitaev honeycomb model, providing a new route toward realizing the latter in cold-atom or solid-state systems.

We combine the swap Monte Carlo algorithm to long multi-CPU molecular dynamics simulations to analyze the equilibrium relaxation dynamics of model supercooled liquids over a time window covering 10 orders of magnitude for temperatures down to the experimental glass transition temperature $T_g$. The analysis of several time correlation functions coupled to spatiotemporal resolution of particle motion allow us to elucidate the nature of the equilibrium dynamics in deeply supercooled liquids. We find that structural relaxation starts at early times in rare localized regions characterized by a waiting-time distribution that develops a power law near $T_g$. At longer times, relaxation events accumulate with increasing probability in these regions as $T_g$ is approached. This accumulation leads to a power-law growth of the linear extension of relaxed domains with time with a large, temperature-dependent dynamic exponent. Past the average relaxation time, unrelaxed domains slowly shrink with time due to relaxation events happening at their boundaries. Our results provide a complete microscopic description of the particle motion responsible for key experimental signatures of glassy dynamics, from the shape and temperature evolution of relaxation spectra to the core features of dynamic heterogeneity. They also provide a microscopic basis to understand the emergence of dynamic facilitation in deeply supercooled liquids and allow us to critically reassess theoretical descriptions of the glass transition.