Controlling the polarization state of electromagnetic radiation enables the investigation of fundamental symmetry properties of matter through chiroptical processes. Over the past decades, many strategies have been developed to reveal structural or dynamical information about chiral molecules with high sensitivity, from the microwave to the extreme ultraviolet range. Most schemes employ circularly or elliptically polarized radiation, and more sophisticated configurations involve, for instance, light pulses with time-varying polarization states. All these schemes share a common property—the polarization state of light is always considered as constant over one optical cycle. In this study, we focus on the optical cycle in order to resolve and control a subcyle chiroptical process. We engineer an electric field whose instantaneous chirality can be controlled within the optical cycle, by combining two phase-locked orthogonally polarized fundamental and second harmonic fields. While the composite field has zero net ellipticity, it shows an instantaneous optical chirality which can be controlled via the two-color delay. We theoretically and experimentally investigate the photoionization of chiral molecules with this controlled chiral field. We find that electrons are preferentially ejected forward or backward relative to the laser propagation direction depending on the molecular handedness, similarly to the well-established photoelectron circular dichroism process. However, since the instantaneous chirality switches sign from one half-cycle to the next, electrons ionized from two consecutive half-cycles of the laser show opposite forward-backward asymmetries. This chiral signal, the enantiosensitive subcycle antisymmetric response gated by electric-field rotation, provides a unique insight into the influence of instantaneous chirality in the dynamical photoionization process. More generally, our results demonstrate the important role of subcycle polarization shaping of electric fields as a new route to study and manipulate chiroptical processes.

We establish a lower bound on the asymptotic secret key rate of continuous-variable quantum key distribution with a discrete modulation of coherent states. The bound is valid against collective attacks and is obtained by formulating the problem as a semidefinite program. We illustrate our general approach with the quadrature-phase-shift-keying modulation scheme and show that distances over 100 km are achievable for realistic values of noise. We also discuss the application to more complex quadrature-amplitude-modulation schemes. This result opens the way to establishing the full security of continuous-variable protocols with a discrete modulation, and thereby to the large-scale deployment of these protocols for quantum key distribution.

Despite the importance of fluid flow for transporting and organizing populations, few laboratory systems exist to systematically investigate the impact of advection on their spatial evolutionary dynamics. To address this problem, we study the morphology and genetic spatial structure of microbial colonies growing on the surface of a nutrient-laden fluid ${10}^4$ to ${10}^5$ times more viscous than water in Petri dishes; the extreme but finite viscosity inhibits undesired thermal convection and allows populations to effectively live at the air-liquid interface due to capillary forces. We discover that S. cerevisiae (baker’s yeast) growing on a viscous liquid behave like “active matter”: They metabolically generate fluid flows many times larger than their unperturbed colony expansion speed, and that flow, in turn, can dramatically impact their colony morphology and spatial population genetics. We show that yeast cells generate fluid flows by consuming surrounding nutrients and decreasing the local substrate density, leading to misaligned fluid pressure and density contours, which ultimately generates vorticity via a thresholdless baroclinic instability. Numerical simulations with experimentally measured parameters demonstrate that an intense vortex ring is produced below the colony’s edge. As the viscosity of the substrate is lowered and the self-induced flow intensifies, we observe three distinct morphologies: At the highest viscosity, cell proliferation and movement produces compact circular colonies with, however, a stretched regime of exponential expansion; intermediate viscosities give rise to compact colonies with “fingers” that are usually monoclonal and then break into smaller cell clusters; at the lowest viscosity, the expanding colony fractures into many genetically diverse, mutually repelling, islandlike fragments that can colonize an entire 94-mm-diameter Petri dish within 36 hours. We propose a simple phenomenological model that predicts the early colony dynamics. Our results provide rich opportunities to study the interplay between fluid flow and spatial population genetics for future investigations.

We resolve phonon number states in the spectrum of a superconducting qubit coupled to a multimode acoustic cavity. Crucial to this resolution is the sharp frequency dependence in the qubit-phonon interaction engineered by coupling the qubit to surface acoustic waves in two locations separated by $\sim 40$ acoustic wavelengths. In analogy to double-slit diffraction, the resulting interference generates high-contrast frequency structure in the qubit-phonon interaction. We observe this frequency structure both in the coupling rate to multiple cavity modes and in the qubit spontaneous emission rate into unconfined modes. We use this sharp frequency structure to resolve single phonons by tuning the qubit to a frequency of destructive interference where all acoustic interactions are dispersive. By exciting several detuned yet strongly coupled phononic modes and measuring the resulting qubit spectrum, we observe that, for two modes, the device enters the strong dispersive regime where single phonons are spectrally resolved.

Quasiparticles and collective modes are two fundamental aspects that characterize quantum matter in addition to its ground-state features. For example, the low-energy physics for Fermi-liquid phase in He-III is featured not only by fermionic quasiparticles near the chemical potential but also by fruitful collective modes in the long-wave limit, including several different sound waves that can propagate through it under different circumstances. On the other hand, it is very difficult for sound waves to be carried by electron liquid in ordinary metals due to the fact that long-range Coulomb interaction among electrons will generate a plasmon gap for ordinary electron density oscillation and thus prohibits the propagation of sound waves through it. In the present paper, we propose a unique type of acoustic collective mode in Weyl semimetals under magnetic field called chiral zero sound. Chiral zero sound can be stabilized under the so-called “chiral limit,” where the intravalley scattering time is much shorter than the intervalley one and propagates only along an external magnetic field for Weyl semimetals with multiple pairs of Weyl points. The sound velocity of chiral zero sound is proportional to the field strength in the weak field limit, whereas it oscillates dramatically in the strong field limit, generating an entirely new mechanism for quantum oscillations through the dynamics of neutral bosonic excitation, which may manifest itself in the thermal conductivity measurements under magnetic field.

Spattering has been a problem in metal processing involving high-power lasers, like laser welding, machining, and recently, additive manufacturing. Limited by the capabilities of in situ diagnostic techniques, typically imaging with visible light or laboratory x-ray sources, a comprehensive understanding of the laser-spattering phenomenon, particularly the extremely fast spatters, has not been achieved yet. Here, using MHz single-pulse synchrotron-x-ray imaging, we probe the spattering behavior of Ti-6Al-4V with micrometer spatial resolution and subnanosecond temporal resolution. Combining direct experimental observations, quantitative image analysis, as well as numerical simulations, our study unravels a novel mechanism of laser spattering: The bulk explosion of a tonguelike protrusion forming on the front keyhole wall leads to the ligamentation of molten metal at the keyhole rims and the subsequent spattering. Our study confirms the critical role of melt and vapor flow in the laser-spattering process and opens a door to manufacturing spatter- and defect-free metal parts via precise control of keyhole dynamics.

We explore the interplay of electron-electron correlations and spin-orbit coupling in the model Fermi liquid ${\mathrm{Sr}}_2{\mathrm{RuO}}_4$ using laser-based angle-resolved photoemission spectroscopy. Our precise measurement of the Fermi surface confirms the importance of spin-orbit coupling in this material and reveals that its effective value is enhanced by a factor of about 2, due to electronic correlations. The self-energies for the $\beta$ and $\gamma$ sheets are found to display significant angular dependence. By taking into account the multi-orbital composition of quasiparticle states, we determine self-energies associated with each orbital component directly from the experimental data. This analysis demonstrates that the perceived angular dependence does not imply momentum-dependent many-body effects but arises from a substantial orbital mixing induced by spin-orbit coupling. A comparison to single-site dynamical mean-field theory further supports the notion of dominantly local orbital self-energies and provides strong evidence for an electronic origin of the observed nonlinear frequency dependence of the self-energies, leading to “kinks” in the quasiparticle dispersion of ${\mathrm{Sr}}_2{\mathrm{RuO}}_4$.

We introduce a new class of states for bosonic quantum fields which extend tensor network states to the continuum and generalize continuous matrix product states to spatial dimensions $d\ge 2$. By construction, they are Euclidean invariant and are genuine continuum limits of discrete tensor network states. Admitting both a functional integral and an operator representation, they share the important properties of their discrete counterparts: expressiveness, invariance under gauge transformations, simple rescaling flow, and compact expressions for the $N$-point functions of local observables. While we discuss mostly the continuous tensor network states extending projected entangled-pair states, we propose a generalization bearing similarities with the continuum multiscale entanglement renormalization ansatz.

We demonstrate full quantum state control of two species of single atoms using optical tweezers and assemble the atoms into a molecule. Our demonstration includes 3D ground-state cooling of a single atom (Cs) in an optical tweezer, transport by several microns with minimal heating, and merging with a single Na atom. Subsequently, both atoms occupy the simultaneous motional ground state with 61(4)% probability. This realizes a sample of exactly two cotrapped atoms near the phase-space-density limit of one, and allows for efficient stimulated-Raman transfer of a pair of atoms into a molecular bound state of the triplet electronic ground potential $a^3{\mathrm{\Sigma }}^{+}$. The results are key steps toward coherent creation of single ultracold molecules for future exploration of quantum simulation and quantum information processing.

By combining theory and experiments, we demonstrate that dipolar quantum gases of both ${}^{166}\mathrm{Er}$ and ${}^{164}\mathrm{Dy}$ support a state with supersolid properties, where a spontaneous density modulation and a global phase coherence coexist. This paradoxical state occurs in a well-defined parameter range, separating the phases of a regular Bose-Einstein condensate and of an insulating droplet array, and is rooted in the roton mode softening, on the one side, and in the stabilization driven by quantum fluctuations, on the other side. Here, we identify the parameter regime for each of the three phases. In the experiment, we rely on a detailed analysis of the interference patterns resulting from the free expansion of the gas, quantifying both its density modulation and its global phase coherence. Reaching the phases via a slow interaction tuning, starting from a stable condensate, we observe that ${}^{166}\mathrm{Er}$ and ${}^{164}\mathrm{Dy}$ exhibit a striking difference in the lifetime of the supersolid properties, due to the different atom loss rates in the two systems. Indeed, while in ${}^{166}\mathrm{Er}$ the supersolid behavior survives only a few tens of milliseconds, we observe coherent density modulations for more than 150 ms in ${}^{164}\mathrm{Dy}$. Building on this long lifetime, we demonstrate an alternative path to reach the supersolid regime, relying solely on evaporative cooling starting from a thermal gas.

Quantum simulations with ultracold atoms typically create atomic wave functions with structures at optical length scales, where direct imaging suffers from the diffraction limit. In analogy to advances in optical microscopy for biological applications, we use a nonlinear atomic response to surpass the diffraction limit. Exploiting quantum interference, we demonstrate imaging with superresolution of $\lambda /50$ and excellent temporal resolution of 500 ns. We characterize our microscope’s performance by measuring the ensemble-averaged probability density of atoms within the unit cells of an optical lattice and observe the dynamics of atoms excited into motion. This approach can be readily applied to image any atomic or molecular system, as long as it hosts a three-level system.

Superresolution microscopy has revolutionized the fields of chemistry and biology by resolving features at the molecular level. In atomic physics, such a scheme can be applied to resolve the atomic density distribution beyond the diffraction limit and to perform quantum control. Here we demonstrate superresolution imaging based on the nonlinear response of atoms to an optical pumping pulse. With this technique, the atomic density distribution can be imaged with a full-width-at-half-maximum resolution of 32(4) nm and a localization precision below 500 pm. The short optical pumping pulse of $1.4\mu \mathrm{s}$ enables us to resolve fast atomic dynamics within a single lattice site. A by-product of our scheme is the emergence of moiré patterns on the atomic cloud, which we show to be immensely magnified images of the atomic density in the lattice.

We study theoretically and experimentally the emergence of supersolid properties in a dipolar Bose-Einstein condensate. The theory reveals a ground state phase diagram with three distinct regimes—a regular Bose-Einstein condensate and incoherent and coherent arrays of quantum droplets. The coherent droplets are connected by a background condensate, which leads—in addition to the periodic density modulation—to a robust phase coherence throughout the whole system. We further theoretically demonstrate that we are able to dynamically approach the ground state in our experiment and that its lifetime is limited only by three-body losses. Experimentally we probe and confirm the signatures of the phase diagram by observing the in situ density modulation as well as the phase coherence using matter wave interference.

Recent research has led to the discovery of fundamental new phenomena in network synchronization, including chimera states, explosive synchronization, and asymmetry-induced synchronization. Each of these phenomena has thus far been observed only in systems designed to exhibit that one phenomenon, which raises the questions of whether they are mutually compatible and, if so, under what conditions they co-occur. Here, we introduce a class of remarkably simple oscillator networks that concurrently exhibit all of these phenomena. The dynamical units consist of pairs of nonidentical phase oscillators, which we refer to as Janus oscillators by analogy with Janus particles and the mythological figure from which their name is derived. In contrast to previous studies, these networks exhibit (i) explosive synchronization with identical oscillators; (ii) extreme multistability of chimera states, including traveling, intermittent, and bouncing chimeras; and (iii) asymmetry-induced synchronization in which synchronization is promoted by random oscillator heterogeneity. These networks also exhibit the previously unobserved possibility of inverted synchronization transitions, in which a transition to a more synchronous state is induced by a reduction rather than an increase in the coupling strength. These various phenomena are shown to emerge under rather parsimonious conditions and even in locally connected ring topologies, which has the potential to facilitate their use to control and manipulate synchronization in experiments.

We perform microwave spectroscopy of Andreev states in superconducting weak links tailored in an InAs-Al (core-full shell) epitaxially grown nanowire. The spectra present distinctive features with bundles of four lines crossing when the superconducting phase difference across the weak link is 0 or $\pi$. We interpret these features as arising from zero-field spin-split Andreev states. A simple analytical model, which takes into account the Rashba spin-orbit interaction in a nanowire containing several transverse subbands, explains these features and their evolution with magnetic field. Our results show that the spin degree of freedom is addressable in Josephson junctions and constitute a first step towards its manipulation.

Tunable directional scattering is of paramount importance for operation of antennas, routing of light, and design of topologically protected optical states. For visible light scattered on a nanoparticle, the directionality could be provided by the Kerker effect, exploiting the interference of electric and magnetic dipole emission patterns. However, magnetic optical resonances in small sub-100-nm particles are relativistically weak. Here, we predict inelastic scattering with the unexpectedly strong tunable directivity up to 5.25 driven by a trembling of a small particle without any magnetic resonance. The proposed optomechanical Kerker effect originates from the vibration-induced multipole conversion. We also put forward an optomechanical spin-Hall effect, the inelastic polarization-dependent directional scattering. Our results uncover an intrinsically multipolar nature of the interaction between light and mechanical motion and apply to a variety of systems from cold atoms to two-dimensional materials to superconducting qubits. An application for engineering of chiral optomechanical coupling and nonreciprocal transmission at nanoscale is proposed.

The Kuramoto model, originally proposed to model the dynamics of many interacting oscillators, has been used and generalized for a wide range of applications involving the collective behavior of large heterogeneous groups of dynamical units whose states are characterized by a scalar angle variable. One such application in which we are interested is the alignment of orientation vectors among members of a swarm. Despite being commonly used for this purpose, the Kuramoto model can only describe swarms in two dimensions, and hence the results obtained do not apply to the often relevant situation of swarms in three dimensions. Partly based on this motivation, as well as on relevance to the classical, mean-field, zero-temperature Heisenberg model with quenched site disorder, in this paper we study the Kuramoto model generalized to $D$ dimensions. We show that in the important case of three dimensions, as well as for any odd number of dimensions, the $D$-dimensional generalized Kuramoto model for heterogeneous units has dynamics that are remarkably different from the dynamics in two dimensions. In particular, for odd $D$ the transition to coherence occurs discontinuously as the interunit coupling constant $K$ is increased through zero, as opposed to the $D=2$ case (and, as we show, also the case of even $D$) for which the transition to coherence occurs continuously as $K$ increases through a positive critical value $K_c$. We also demonstrate the qualitative applicability of our results to related models constructed specifically to capture swarming and flocking dynamics in three dimensions.

We demonstrate single-shot imaging and narrow-line cooling of individual alkaline-earth atoms in optical tweezers; specifically, strontium trapped in $515.2\text{−}\mathrm{nm}$ light. Our approach enables high-fidelity detection of single atoms by imaging photons from the broad singlet transition while cooling on the narrow intercombination line, and we extend this technique to highly uniform two-dimensional tweezer arrays with 121 sites. Cooling during imaging is based on a previously unobserved narrow-line Sisyphus mechanism, which we predict to be applicable in a wide variety of experimental situations. Further, we demonstrate optically resolved sideband cooling of a single atom to near the motional ground state of a tweezer, which is tuned to a magic-trapping configuration achieved by elliptical polarization. Finally, we present calculations, in agreement with our experimental results, that predict a linear-polarization and polarization-independent magic crossing at 520(2) nm and 500.65(50) nm, respectively. Our results pave the way for a wide range of novel experimental avenues based on individually controlled alkaline-earth atoms in tweezers—from fundamental experiments in atomic physics to quantum computing, simulation, and metrology.

Optical tweezers provide a versatile platform for the manipulation and detection of single atoms. Here, we use optical tweezers to demonstrate a set of tools for the microscopic control of atomic strontium, which has two valence electrons. Compared to the single-valence-electron atoms typically used with tweezers, strontium has a more complex internal state structure with a variety of transition wavelengths and linewidths. We report single-atom loading into an array of subwavelength scale optical tweezers and light-shift-free control of a narrow-linewidth optical transition. We use this transition to perform three-dimensional ground-state cooling and to enable high-fidelity nondestructive imaging of single atoms on subwavelength spatial scales. These capabilities, combined with the rich internal structure of strontium, open new possibilities including tweezer-based metrology, new quantum computing architectures, and new paths to low-entropy many-body physics.

In sight of fundamental thermal limits on further substantial performance improvements of modern digital computational processing units, wave-based analog computation is becoming an enticing alternative. A wave, as it propagates through a carefully tailored medium, performs the desired computational operation. Yet, the necessary designs are so intricate that experimental demonstrations will necessitate further technological advances. Here, we show that, counterintuitively, the carefully tailored medium can be replaced with a random medium, subject to an appropriate shaping of the incident wave front. Using tunable metasurface reflect-arrays, we demonstrate our concept experimentally in a chaotic microwave cavity. We conclude that off-the-shelf wireless communication infrastructure in combination with a simple reflect-array suffices to perform analog computation with Wi-Fi waves reverberating in a room.