Background: The probability per unit area for a radioactive nucleus ( d) to capture neutrons across resonance energies—the neutron-capture resonance integral ()—is the largest ever reported [Shusterman et al., Phys. Rev. C 103, 024614 (2021)] with a value of barns. This implies that the neutron-capture cross section is orders of magnitude larger than previously thought at energies relevant to explosive environments applications, such as nuclear astrophysics and radiochemical diagnostics of nuclear devices.
Purpose: These applications require the shape of the capture cross section across a wide energy range which has never been measured before. The unexpectedly large values of both the thermal capture cross section and resonance integral could have a large impact on applications. Thus, the determination of the neutron capture cross sections over a wide energy range is important on both fundamental and applied levels.
Method: A neutron transmission experiment on [Stamatopoulos et al., Phys. Rev. Lett. 134, 112702 (2025)] was performed at the Device for Indirect Capture Experiments on Radionuclides (DICER) at the Los Alamos Neutron Science CEnter (LANSCE), from to 500 eV using the time of flight technique. Any resonances responsible for the large cross section (), will be reflected in the (,tot) cross section. The (,tot) data were used to extract the capture cross section as a function of energy.
Results: The present work revealed a nuclear level in the system at 171 meV above the neutron separation energy and a thermal neutron-capture cross section of 771(31) kb, which is in good agreement with the recently published value [Shusterman et al., Phys. Rev. C 103, 024614 (2021) and Shusterman et al., Nature (London) 565, 328 (2019)]. In contrast, the neutron-capture resonance integral extracted from the present data is 15.21(67) kb and is roughly a factor of 200 smaller than the literature value [Shusterman et al., Phys. Rev. C 103, 024614 (2021)].
Conclusions: The recently reported enormous thermal capture cross section was confirmed and is attributed to a resonance at 171 meV and bound state 174 eV below the neutron separation energy. Our obtained value of the resonance integral is 166 times smaller than reported and that can have a huge impact on applications.