Polar dielectrics with low crystal symmetry and sharp phonon resonances can support hyperbolic shear polaritons, which are highly confined surface modes with frequency-dependent optical axes and asymmetric dissipation features. So far, these modes have been observed only in bulk natural materials at midinfrared frequencies, with properties limited by available crystal geometries and phonon resonance strength. Here, we introduce hyperbolic shear metasurfaces, which are ultrathin engineered surfaces supporting hyperbolic surface modes with symmetry-tailored axial dispersion and loss redistribution that can maximally enhance light-matter interactions. By engineering effective shear phenomena in these engineered surfaces, we demonstrate geometry-controlled, ultraconfined, low-loss hyperbolic surface waves with broadband Purcell enhancements applicable across a broad range of the electromagnetic spectrum.

Solid-state spin qubits are promising candidates for quantum information processing, but controlled interactions and entanglement in large, multiqubit systems are currently difficult to achieve. We describe a method for programmable control of multiqubit spin systems, in which individual nitrogen-vacancy (NV) centers in diamond nanopillars are coupled to magnetically functionalized silicon nitride mechanical resonators in a scanning probe configuration. Qubits can be entangled via interactions with nanomechanical resonators while programmable connectivity is realized via mechanical transport of qubits in nanopillars. To demonstrate the feasibility of this approach, we characterize both the mechanical properties and the magnetic field gradients around the micromagnet placed on the nanobeam resonator. We demonstrate coherent manipulation of a spin qubit in the proximity of a transported micromagnet by utilizing nuclear spin memory and use the NV center to detect the time-varying magnetic field from the oscillating micromagnet, extracting a spin-mechanical coupling of 7.7(9) Hz. With realistic improvements, the high-cooperativity regime can be reached, offering a new avenue toward scalable quantum information processing with spin qubits.

We report on the coherent excitation of the ultranarrow ${}^1{S}_0–{}^3{P}_2$ magnetic quadrupole transition in ${}^{88}\mathrm{Sr}$. By confining atoms in a state insensitive optical lattice, we achieve excitation fractions of 97(1)% and observe linewidths as narrow as 58(1) Hz. With Ramsey spectroscopy, we find coherence times of 14(1) ms, which can be extended to 266(36) ms using a spin-echo sequence. We determine the lifetime of the ${}^3{P}_2$ level for spontaneous emission of magnetic quadrupole radiation to be 110(31) min, confirming long-standing theoretical predictions. These results establish an additional clock transition in strontium and pave the way for applications of the metastable ${}^3{P}_2$ state in quantum computing and quantum simulations.

An elongated object can be rotated around one of its short axes, like a propeller, or around its long axis, like a spinning top. Using optically levitated nanoparticles, short-axis rotation and libration have been systematically investigated in several recent studies. Notably, short-axis rotational degrees of freedom have been cooled to millikelvin temperatures and driven into gigahertz rotational speeds. However, controlled long-axis spinning has so far remained an unrealized goal. Here, we demonstrate controlled long-axis spinning of an optically levitated nanodumbbell with spinning rates exceeding 1 GHz. We show that the damping rate in high vacuum can be as low as a few millihertz. Our results open up applications in inertial torque sensing and studies of rotational quantum interference.

A unitary Fermi gas in an isotropic harmonic trap is predicted to show scale and conformal symmetry that have important consequences in its thermodynamic and dynamical properties. By experimentally realizing a unitary Fermi gas in an isotropic harmonic trap, we demonstrate its universal expansion dynamics along each direction and at different temperatures. We show that as a consequence of SO(2,1) symmetry, the measured release energy is equal to that of the trapping energy. We further observe the breathing mode with an oscillation frequency twice the trapping frequency and a small damping rate, providing the evidence of SO(2,1) symmetry. In addition, away from resonance when scale invariance is broken, we determine the effective exponent $\gamma$ that relates the chemical potential and average density along the BEC-BCS crossover, which qualitatively agrees with the mean field predictions. This Letter opens the possibility of studying nonequilibrium dynamics in a conformal invariant system in the future.

We present a merged-beams study of reactions between ${\mathrm{HD}}^{+}$ ions, stored in the Cryogenic Storage Ring (CSR), and laser-produced ground-term C atoms. The molecular ions are stored for up to 20 s in the extreme vacuum of the CSR, where they have time to relax radiatively until they reach their vibrational ground state (within 0.5 s of storage) and rotational states with $J\le 3$ (after 5 s). We combine our experimental studies with quasiclassical trajectory calculations based on two reactive potential energy surfaces. In contrast to previous studies with internally excited ${\mathrm{H}}_2^{+}$ and ${\mathrm{D}}_2^{+}$ ions, our results reveal a pronounced isotope effect, favoring the production of ${\mathrm{CH}}^{+}$ over ${\mathrm{CD}}^{+}$ across all collision energies, and a significant increase in the absolute rate coefficient of the reaction. Our experimental results agree well with our theoretical calculations for vibrationally relaxed ${\mathrm{HD}}^{+}$ ions in their lowest rotational states.

The momentum space Josephson effect describes the supercurrent flow between weakly coupled Bose-Einstein condensates (BECs) at two discrete momentum states. Here, we experimentally observe this exotic phenomenon using a BEC with Raman-induced spin-orbit coupling, where the tunneling between two local band minima is implemented by the momentum kick of an additional optical lattice. A sudden quench of the Raman detuning induces coherent spin-momentum oscillations of the BEC, which is analogous to the ac Josephson effect. We observe both plasma and regular Josephson oscillations in different parameter regimes. The experimental results agree well with the theoretical model and numerical simulation and showcase the important role of nonlinear interactions. We also show that the measurement of the Josephson plasma frequency gives the Bogoliubov zero quasimomentum gap, which determines the mass of the corresponding pseudo-Goldstone mode, a long-sought phenomenon in particle physics. The observation of momentum space Josephson physics offers an exciting platform for quantum simulation and sensing utilizing momentum states as a synthetic degree.

A key method to produce trapped and laser-cooled molecules is the magneto-optical trap (MOT), which is conventionally created using light red detuned from an optical transition. In this work, we report a MOT for CaF molecules created using blue-detuned light. The blue-detuned MOT (BDM) achieves temperatures well below the Doppler limit and provides the highest densities and phase-space densities reported to date in CaF MOTs. Our results suggest that BDMs are likely achievable in many relatively light molecules including polyatomic ones, but our measurements suggest that BDMs will be challenging to realize in substantially heavier molecules due to sub-mK trap depths. In addition to record temperatures and densities, we find that the BDM substantially simplifies and enhances the loading of molecules into optical tweezer arrays, which are a promising platform for quantum simulation and quantum information processing. Notably, the BDM reduces molecular number requirements ninefold compared to a conventional red-detuned MOT, while not requiring additional hardware. Our work therefore substantially simplifies preparing large-scale molecular tweezer arrays, which are a novel platform for simulation of quantum many-body dynamics and quantum information processing with molecular qubits.

Interatomic Coulombic decay (ICD) plays a crucial role in weakly bound complexes exposed to intense or high-energy radiation. So far, neutral or ionic atoms or molecules have been prepared in singly excited electron or hole states that can transfer energy to neighboring centers and cause ionization and radiation damage. Here we demonstrate that a doubly excited atom, despite its extremely short lifetime, can decay by ICD; evidenced by high-resolution photoelectron spectra of He nanodroplets excited to the $2s2p+$ state. We find that ICD proceeds by relaxation into excited ${\mathrm{He}}^{*}{\mathrm{He}}^{+}$ atom-pair states, in agreement with calculations. The ability of inducing ICD by resonant excitation far above the single-ionization threshold opens opportunities for controlling radiation damage to a high degree of element specificity and spectral selectivity.

Attoclock provides a powerful tool for probing the ultrafast electron dynamics in strong laser fields. However, this technique has remained restricted to single electron or sequential double ionized electron dynamics. Here, we propose a novel attoclock scheme with a polarization-gated few-cycle laser pulse and demonstrate its application in timing the correlated-electron emission in strong field double ionization of argon. Our experimental measurements reveal that the correlated-electron emission occurs mainly through two channels with time differences of $234\pm 22$ as and $1043\pm 73$ as, respectively. Classical model calculations well reproduce the experimental results and deepen our understanding of ultrafast electron correlation dynamics.

We present the new concept of photonic alloy as a nonperiodic topological material. By mixing nonmagnetized and magnetized rods in a nonperiodic 2D photonic crystal configuration, we realized photonic alloys in the microwave regime. Our experimental findings reveal that the photonic alloy sustains nonreciprocal chiral edge states even at very low concentration of magnetized rods. The nontrivial topology and the associated edge states of these nonperiodic systems can be characterized by the winding of the reflection phase. Our results indicate that the threshold concentrations for the investigated system within the first nontrivial band gap to exhibit topological behavior approach zero in the thermodynamic limit for substitutional alloys, while the threshold remains nonzero for interstitial alloys. At low concentration, the system exhibits an inhomogeneous structure characterized by isolated patches of nonpercolating magnetic domains that are spaced far apart within a topologically trivial photonic crystal. Surprisingly, the system manifests chiral edge states despite a local breakdown of time-reversal symmetry rather than a global one. Photonic alloys represent a new category of disordered topological materials, offering exciting opportunities for exploring topological materials with adjustable gaps.

Recent experimental developments in multimode nonlinear photonic circuits (MMNPCs), have motivated the development of an optical thermodynamic theory that describes the equilibrium properties of an initial beam excitation. However, a nonequilibrium transport theory for these systems, when they are in contact with thermal reservoirs, is still terra incognita. Here, by combining Landauer and kinematics formalisms we develop a universal one-parameter scaling theory that describes the whole transport behavior from the ballistic to the diffusive regime, including both positive and negative optical temperature scenarios. We also derive a photonic version of the Wiedemann-Franz law that connects the thermal and power conductivities. Our work paves the way toward a fundamental understanding of the transport properties of MMNPCs and may be useful for the design of all-optical cooling protocols.

The ability to tailor with a high accuracy the intersite connectivity in a lattice is a crucial tool for realizing novel topological phases of matter. Here, we report the experimental realization of photonic dimer chains with long-range hopping terms of arbitrary strength and phase, providing a rich generalization of the Su-Schrieffer-Heeger model which, in its conventional form, is limited to nearest-neighbor couplings only. Our experiment is based on a synthetic dimension scheme involving the frequency modes of an optical fiber loop platform. This setup provides direct access to both the band dispersion and the geometry of the Bloch wave functions throughout the entire Brillouin zone allowing us to extract the winding number for any possible configuration. Finally, we highlight a topological phase transition solely driven by a time-reversal-breaking synthetic gauge field associated with the phase of the long-range hopping, providing a route for engineering topological bands in photonic lattices belonging to the AIII symmetry class.

Increasing accuracy of the theory and experiment of the $n=2$ ${}^3\mathrm{P}$ fine structure of helium has allowed for increasingly precise tests of quantum electrodynamics (QED), determinations of the fine-structure constant $\alpha$, and limitations on possible beyond the standard model physics. Here we present a 2 ppb measurement of the $J=1$ to $J=0$ interval. The measurement is performed using frequency-offset separated-oscillatory fields. Our result of 29 616 955 018(60) Hz represents a landmark for helium fine-structure measurements, and, for the first time, will allow for a 1-ppb determination of the fine-structure constant when QED theory for the interval is improved.

We report optical trapping of laser-cooled molecules at sufficient density to observe molecule-molecule collisions for the first time in a bulk gas. SrF molecules from a red-detuned magneto-optical trap (MOT) are compressed and cooled in a blue-detuned MOT. Roughly 30% of these molecules are loaded into an optical dipole trap with peak number density $n_0\approx 3\times {10}^{10}{\mathrm{cm}}^{-3}$ and temperature $T\approx 40\mathrm{\mu }\mathrm{K}$. We observe two-body loss with rate coefficient $\beta ={2.7}_{-0.8}^{+1.2}\times {10}^{-10}{\mathrm{cm}}^3{\mathrm{s}}^{-1}$. Achieving this density and temperature opens a path to evaporative cooling towards quantum degeneracy of laser-cooled molecules.

In ${\mathrm{CO}}_2$-rich atmospheres that are always exposed to ionizing radiation (e.g., Venus and Mars), every fragmentation process can significantly impact the inventory of moieties present in these environments. Nevertheless, the production of ${\mathrm{O}}_2^{+}$ ions as a direct result of ${\mathrm{CO}}_2$ fragmentation has never been quantified so far. Since molecular oxygen is considered as a potential trace of living organisms, nonbiotic pathways for its production must be known. In this work, ${\mathrm{O}}_2^{+}$ coming from ${\mathrm{CO}}_2$ fragmentation by electron impact is unambiguously identified and measured in absolute scale.

We propose and experimentally demonstrate the generation of enhanced optical springs using the optical Kerr effect. A nonlinear optical crystal is inserted into a Fabry-Perot cavity with a movable mirror, and a chain of second-order nonlinear optical effects in the phase-mismatched condition induces the Kerr effect. The optical spring constant is enhanced by a factor of $1.6\pm 0.1$ over linear theory. To our knowledge, this is the first realization of optomechanical coupling enhancement using a nonlinear optical effect, which has been theoretically investigated to overcome the performance limitations of linear optomechanical systems. The tunable nonlinearity of demonstrated system has a wide range of potential applications, from observing gravitational waves emitted by binary neutron star postmerger remnants to cooling macroscopic oscillators to their quantum ground state.

Uninhibited control of the complex spatiotemporal quantum wave function of a single photon has so far remained elusive even though it can dramatically increase the encoding flexibility and thus the information capacity of a photonic quantum link. By fusing temporal waveform generation in an atomic ensemble and spatial single-photon shaping, we hereby demonstrate for the first time complete spatiotemporal control of a propagation invariant $(2+1)\text{D}$ Airy single-photon optical bullet. These correlated photons are not only self-accelerating and impervious to spreading as their classical counterparts, but can be concealed and revealed in the presence of strong classical stray light.

An integrated quantum light source is increasingly desirable in large-scale quantum information processing. Despite recent remarkable advances, a new material platform is constantly being explored for the fully on-chip integration of quantum light generation, active and passive manipulation, and detection. Here, for the first time, we demonstrate a gallium nitride (GaN) microring based quantum light generation in the telecom C-band, which has potential toward the monolithic integration of quantum light source. In our demonstration, the GaN microring has a free spectral range of 330 GHz and a near-zero anomalous dispersion region of over 100 nm. The generation of energy-time entangled photon pair is demonstrated with a typical raw two-photon interference visibility of $95.5\pm 6.5\%$, which is further configured to generate a heralded single photon with a typical heralded second-order autocorrelation $g_H^{(2)}(0)$ of $0.045\pm 0.001$. Our results pave the way for developing a chip-scale quantum photonic circuit.

A levitated nanomechanical oscillator under ultrahigh vacuum is highly isolated from its environment. It has been predicted that this isolation leads to very low mechanical dissipation rates. However, a gap persists between predictions and experimental data. Here, we levitate a silica nanoparticle in a linear Paul trap at room temperature, at pressures as low as $7\times {10}^{-11}\mathrm{mbar}$. We measure a dissipation rate of $2\pi \times 69(22)\mathrm{nHz}$, corresponding to a quality factor exceeding ${10}^{10}$, more than 2 orders of magnitude higher than previously shown. A study of the pressure dependence of the particle’s damping and heating rates provides insight into the relevant dissipation mechanisms.