We report the storage and retrieval of single photons, via a quantum memory, in the optical phonons of a room-temperature bulk diamond. The THz-bandwidth heralded photons are generated by spontaneous parametric down-conversion and mapped to phonons via a Raman transition, stored for a variable delay, and released on demand. The second-order correlation of the memory output is $g^{(2)}(0)=0.65\pm 0.07$, demonstrating a preservation of nonclassical photon statistics throughout storage and retrieval. The memory is low noise, high speed and broadly tunable; it therefore promises to be a versatile light-matter interface for local quantum processing applications.

Quantum entanglement, a key resource for quantum information science, is inherent in a solid. It has been recently shown that entanglement between a single optical photon and a single spin qubit in a solid is generated via spontaneous emission. However, entanglement generation by measurement is rather essential for quantum operations. We here show that the physics behind the entangled emission can be time reversed to demonstrate entangled absorption mediated by an inherent spin-orbit entanglement in a single nitrogen vacancy center in diamond. Optical arbitrary spin state preparation and complete spin state tomography reveal the fidelity of the entangled absorption to be 95%. With the entangled emission and absorption of a photon, materials can be spontaneously entangled or swap their quantum state based on the quantum teleportation scheme.

We consider the observation of diffuse halos of light around the discs of spiral galaxies, as a probe of the interaction cross section between dark matter (DM) and photons. Using the galaxy M101 as an example, we show that for a scattering cross section at the level of ${10}^{-23}(m/\mathrm{GeV}){\mathrm{cm}}^2$ or greater dark matter in the halo will scatter light out from the more luminous center of the disc to larger radii, contributing to an effective increased surface brightness at the edges of the observed area on the sky. This allows us to set an upper limit on the DM-photon cross section using data from the Dragonfly instrument. We then show how to improve this constraint, and the potential for discovery, by combining the radial profile of DM-photon scattering with measurements at multiple wavelengths. Observation of diffuse light presents a new and potentially powerful way to probe the interactions of dark matter with photons, a way that is complementary to existing searches.

The unprecedented light curves of the Kepler space telescope document how the brightness of some stars pulsates at primary and secondary frequencies whose ratios are near the golden mean, the most irrational number. A nonlinear dynamical system driven by an irrational ratio of frequencies generically exhibits a strange but nonchaotic attractor. For Kepler’s “golden” stars, we present evidence of the first observation of strange nonchaotic dynamics in nature outside the laboratory. This discovery could aid the classification and detailed modeling of variable stars.

An analysis is conducted of the multipartite entanglement for Gaussian states generated by the parametric down-conversion of a femtosecond frequency comb. Using a recently introduced method for constructing optimal entanglement criteria, a family of tests is formulated for mode decompositions that extends beyond the traditional bipartition analyses. A numerical optimization over this family is performed to achieve maximal significance of entanglement verification. For experimentally prepared 4-, 6-, and 10-mode states, full entanglement is certified for all of the 14, 202, and 115 974 possible nontrivial partitions, respectively.

The electric dipole moments of ${({\mathrm{H}}_2\mathrm{O})}_n\mathrm{DCl}$ ($n=3–9$) clusters have been measured by the beam-deflection method. Reflecting the (dynamical) charge distribution within the system, the dipole moment contributes information about the microscopic structure of nanoscale solvation. The addition of a DCl molecule to a water cluster results in a strongly enhanced susceptibility. There is evidence for a noticeable rise in the dipole moment occurring at $n\approx 5–6$. This size is consistent with predictions for the onset of ionic dissociation. Additionally, a molecular-dynamics model suggests that even with a nominally bound impurity an enhanced dipole moment can arise due to the thermal and zero-point motion of the proton and the water molecules. The experimental measurements and the calculations draw attention to the importance of fluctuations in defining the polarity of water-based nanoclusters and generally to the essential role played by motional effects in determining the response of fluxional nanoscale systems under realistic conditions.

Using a quantum circuit model we derive the maximal ability to distinguish which of several candidate Hamiltonians describe an open quantum system. This theory, in particular, provides the maximum information retrievable from continuous quantum measurement records, available when a quantum system is perturbatively coupled to a broadband quantized environment.

In order to resolve a recent discrepancy in the half-life of ${}^{60}\mathrm{Fe}$, we performed an independent measurement with a new method that determines the ${}^{60}\mathrm{Fe}$ content of a material relative to ${}^{55}\mathrm{Fe}$ ($t_{1/2}=2.744\mathrm{yr}$) with accelerator mass spectrometry. Our result of $(2.50\pm 0.12)\times {10}^6\mathrm{yr}$ clearly favors the recently reported value $(2.62\pm 0.04)\times {10}^6\mathrm{yr}$, and rules out the older result of $(1.49\pm 0.27)\times {10}^6\mathrm{yr}$. The present weighted mean half-life value of $(2.60\pm 0.05)\times {10}^6\mathrm{yr}$ substantially improves the reliability as an important chronometer for astrophysical applications in the million-year time range. This includes its use as a sensitive probe for studying recent chemical evolution of our Galaxy, the formation of the early Solar System, nucleosynthesis processes in massive stars, and as an indicator of a recent nearby supernova.

This Letter reports the demonstration of laser cooling without spontaneous emission, and thereby addresses a significant controversy. It works by restricting the atom-light interaction to a time short compared to a cycle of absorption followed by natural decay. It is achieved by using the bichromatic force on an atomic transition with a relatively long excited state lifetime and a relatively short cooling time so that spontaneous emission effects are minimized. The observed width of the one-dimensional velocity distribution is reduced by $\times 2$ thereby reducing the “temperature” by $\times 4$. Moreover, our results comprise a compression in phase space because the spatial expansion of the atomic sample is limited. This accomplishment is of interest to direct laser cooling of molecules or in experiments where working space or time is limited.

This Letter presents the first experimental demonstration of the capability to launch shocks of several-hundred Mbar in spherical targets—a milestone for shock ignition [R. Betti et al., Phys. Rev. Lett. 98, 155001 (2007)]. Using the temporal delay between the launching of the strong shock at the outer surface of the spherical target and the time when the shock converges at the center, the shock-launching pressure can be inferred using radiation-hydrodynamic simulations. Peak ablation pressures exceeding 300 Mbar are inferred at absorbed laser intensities of $\sim 3\times {10}^{15}\mathrm{W}/{\mathrm{cm}}^2$. The shock strength is shown to be significantly enhanced by the coupling of suprathermal electrons with a total converted energy of up to 8% of the incident laser energy. At the end of the laser pulse, the shock pressure is estimated to exceed $\sim 1\mathrm{Gbar}$ because of convergence effects.

Optomechanical coupling between a light field and the motion of a cavity mirror via radiation pressure plays an important role for the exploration of macroscopic quantum physics and for the detection of gravitational waves (GWs). It has been used to cool mechanical oscillators into their quantum ground states and has been considered to boost the sensitivity of GW detectors, e.g., via the optical spring effect. Here, we present the experimental characterization of generalized, that is, dispersive and dissipative, optomechanical coupling, with a macroscopic $(1.5\mathrm{mm}{)}^2$-size silicon nitride membrane in a cavity-enhanced Michelson-type interferometer. We report for the first time strong optomechanical cooling based on dissipative coupling, even on cavity resonance, in excellent agreement with theory. Our result will allow for new experimental regimes in macroscopic quantum physics and GW detection.

Free electrons can possess an intrinsic orbital angular momentum, similar to those in an electron cloud, upon free-space propagation. The wave front corresponding to the electron’s wave function forms a helical structure with a number of twists given by the angular speed. Beams with a high number of twists are of particular interest because they carry a high magnetic moment about the propagation axis. Among several different techniques, electron holography seems to be a promising approach to shape a conventional electron beam into a helical form with large values of angular momentum. Here, we propose and manufacture a nanofabricated phase hologram for generating a beam of this kind with an orbital angular momentum up to $200\hslash$. Based on a novel technique the value of orbital angular momentum of the generated beam is measured and then compared with simulations. Our work, apart from the technological achievements, may lead to a way of generating electron beams with a high quanta of magnetic moment along the propagation direction and, thus, may be used in the study of the magnetic properties of materials and for manipulating nanoparticles.

We report an experimental study of superfluid hydrodynamic effects in a one-dimensional polariton fluid flowing along a laterally patterned semiconductor microcavity and hitting a micron-sized engineered defect. At high excitation power, superfluid propagation effects are observed in the polariton dynamics; in particular, a sharp acoustic horizon is formed at the defect position, separating regions of sub- and supersonic flow. Our experimental findings are quantitatively reproduced by theoretical calculations based on a generalized Gross-Pitaevskii equation. Promising perspectives to observe Hawking radiation via photon correlation measurements are illustrated.

It has been conjectured that the velocity of sound in any medium is smaller than the velocity of light in vacuum divided by $\sqrt{3}$. Simple arguments support this bound in nonrelativistic and/or weakly coupled theories. The bound has been demonstrated in several classes of strongly coupled theories with gravity duals and is saturated only in conformal theories. We point out that the existence of neutron stars with masses around two solar masses combined with the knowledge of the equation of state of hadronic matter at “low” densities is in strong tension with this bound.

We show that a small number of intentionally introduced defects can be used as a spectroscopic tool to amplify quasiparticle interference in $2H\text{−}{\mathrm{NbSe}}_2$ that we measure by scanning tunneling spectroscopic imaging. We show, from the momentum and energy dependence of the quasiparticle interference, that Fermi surface nesting is inconsequential to charge density wave formation in $2H\text{−}{\mathrm{NbSe}}_2$. We demonstrate that, by combining quasiparticle interference data with additional knowledge of the quasiparticle band structure from angle resolved photoemission measurements, one can extract the wave vector and energy dependence of the important electronic scattering processes thereby obtaining direct information both about the fermiology and the interactions. In $2H\text{−}{\mathrm{NbSe}}_2$, we use this combination to confirm that the important near-Fermi-surface electronic physics is dominated by the coupling of the quasiparticles to soft mode phonons at a wave vector different from the charge density wave ordering wave vector.

From experimental studies, it is well known that colloidal particles suspended in a near-critical binary solvent exhibit interesting aggregation phenomena, often associated with colloidal phase transitions and assumed to be driven by long-ranged solvent-mediated (SM) interactions (critical Casimir forces), set by the (diverging) correlation length of the solvent. We present the first simulation and theoretical study of an explicit model of a ternary mixture that mimics this situation. Both the effective SM pair interactions and the full ternary phase diagram are determined for Brownian disks suspended in an explicit two-dimensional supercritical binary liquid mixture. Gas-liquid and fluid-solid transitions are observed in a region that extends well away from criticality of the solvent reservoir. We discuss to what extent an effective pair-potential description can account for the phase behavior we observe. Our study provides a fresh perspective on how proximity to the critical point of the solvent reservoir might influence colloidal self-assembly.

At this time, explosive synchronization (ES) of networked oscillators is thought of as being rooted in the setting of specific microscopic correlation features between the natural frequencies of the oscillators and their effective coupling strengths. We show that ES is, in fact, far more general and can occur in adaptive and multilayer networks in the absence of such correlation properties. We first report evidence of ES for single-layer networks where a fraction $f$ of the nodes have links adaptively controlled by a local order parameter, and we then extend the study to a variety of two-layer networks with a fraction $f$ of their nodes coupled with each other by means of dependency links. In the latter case, we give evidence of ES regardless of the differences in the frequency distribution, in the topology of connections between the layers, or both. Finally, we provide a rigorous, analytical treatment to properly ground all of the observed scenarios and to advance the understanding of the actual mechanisms at the basis of ES in real-world systems.

Atrial fibrillation (AF) is the most common abnormal heart rhythm and the single biggest cause of stroke. Ablation, destroying regions of the atria, is applied largely empirically and can be curative but with a disappointing clinical success rate. We design a simple model of activation wave front propagation on an anisotropic structure mimicking the branching network of heart muscle cells. This integration of phenomenological dynamics and pertinent structure shows how AF emerges spontaneously when the transverse cell-to-cell coupling decreases, as occurs with age, beyond a threshold value. We identify critical regions responsible for the initiation and maintenance of AF, the ablation of which terminates AF. The simplicity of the model allows us to calculate analytically the risk of arrhythmia and express the threshold value of transversal cell-to-cell coupling as a function of the model parameters. This threshold value decreases with increasing refractory period by reducing the number of critical regions which can initiate and sustain microreentrant circuits. These biologically testable predictions might inform ablation therapies and arrhythmic risk assessment.

Knots are abundant in globular homopolymers but rare in globular proteins. To shed new light on this long-standing conundrum, we study the influence of sequence on the formation of knots in proteins under native conditions within the framework of the hydrophobic-polar lattice protein model. By employing large-scale Wang-Landau simulations combined with suitable Monte Carlo trial moves we show that even though knots are still abundant on average, sequence introduces large variability in the degree of self-entanglements. Moreover, we are able to design sequences which are either almost always or almost never knotted. Our findings serve as proof of concept that the introduction of just one additional degree of freedom per monomer (in our case sequence) facilitates evolution towards a protein universe in which knots are rare.

Nonlocality enables two parties to win specific games with probabilities strictly higher than allowed by any classical theory. Nevertheless, all known such examples consider games where the two parties have a common interest, since they jointly win or lose the game. The main question we ask here is whether the nonlocal feature of quantum mechanics can offer an advantage in a scenario where the two parties have conflicting interests. We answer this in the affirmative by presenting a simple conflicting interest game, where quantum strategies outperform classical ones. Moreover, we show that our game has a fair quantum equilibrium with higher payoffs for both players than in any fair classical equilibrium. Finally, we play the game using a commercial entangled photon source and demonstrate experimentally the quantum advantage.