Carrying out fault-tolerant topological quantum computation using non-Abelian anyons (e.g., Majorana zero modes) is currently an important goal of worldwide experimental efforts. However, the Gottesman-Knill theorem [1] holds that if a system can only perform a certain subset of available quantum operations (i.e., operations from the Clifford group) in addition to the preparation and detection of qubit states in the computational basis, then that system is insufficient for universal quantum computation. Indeed, any measurement results in such a system could be reproduced within a local hidden variable theory, so there is no need for a quantum-mechanical explanation and therefore no possibility of quantum speedup [2]. Unfortunately, Clifford operations are precisely the ones available through braiding and measurement in systems supporting non-Abelian Majorana zero modes, which are otherwise an excellent candidate for topologically protected quantum computation. In order to move beyond the classically simulable subspace, an additional phase gate is required. This phase gate allows the system to violate the Bell-like Clauser-Horne-Shimony-Holt (CHSH) inequality that would constrain a local hidden variable theory. In this article, we introduce a new type of phase gate for the already-existing semiconductor-based Majorana wire systems and demonstrate how this phase gate may be benchmarked using CHSH measurements. We present an experimentally feasible schematic for such an experiment using a “measurement-only” approach that bypasses the need for explicit Majorana braiding. This approach may be scaled beyond the two-qubit system necessary for CHSH violations, leading to a well-defined platform for universal fault-tolerant quantum computation using Majorana zero modes.

The Seebeck coefficient $S$ of the cuprate superconductor ${\mathrm{La}}_{2-x}{\mathrm{Sr}}_x{\mathrm{CuO}}_4$ (LSCO) was measured in magnetic fields large enough to access the normal state at low temperatures, for a range of Sr concentrations from $x=0.07$ to $x=0.15$. For $x=0.11$, 0.12, 0.125, and 0.13, $S/T$ decreases upon cooling to become negative at low temperatures. The same behavior is observed in the Hall coefficient $R_{\mathrm{H}}(T)$. In analogy with other hole-doped cuprates at similar hole concentrations $p$, the negative $S$ and $R_{\mathrm{H}}$ show that the Fermi surface of LSCO undergoes a reconstruction caused by the onset of charge-density-wave modulations. Such modulations have indeed been detected in LSCO by x-ray diffraction in precisely the same doping range. Our data show that in LSCO this Fermi-surface reconstruction is confined to $0.085<p<0.15$. We argue that in the field-induced normal state of LSCO, charge-density-wave order ends at a critical doping $p_{\mathrm{CDW}}=0.15\pm 0.005$, well below the pseudogap critical doping $p^{\star }\simeq 0.19$.

The electron-phonon coupling and the corresponding energy exchange are investigated experimentally and by ab initio theory in nonequilibrium states of the free-electron metal aluminium. The temporal evolution of the atomic mean-squared displacement in laser-excited thin freestanding films is monitored by femtosecond electron diffraction. The electron-phonon coupling strength is obtained for a range of electronic and lattice temperatures from density functional theory molecular dynamics simulations. The electron-phonon coupling parameter extracted from the experimental data in the framework of a two-temperature model (TTM) deviates significantly from the ab initio values. We introduce a nonthermal lattice model (NLM) for describing nonthermal phonon distributions as a sum of thermal distributions of the three phonon branches. The contributions of individual phonon branches to the electron-phonon coupling are considered independently and found to be dominated by longitudinal acoustic phonons. Using all material parameters from first-principles calculations except the phonon-phonon coupling strength, the prediction of the energy transfer from electrons to phonons by the NLM is in excellent agreement with time-resolved diffraction data. Our results suggest that the TTM is insufficient for describing the microscopic energy flow even for simple metals like aluminium and that the determination of the electron-phonon coupling constant from time-resolved experiments by means of the TTM leads to incorrect values. In contrast, the NLM describing transient phonon populations by three parameters appears to be a sufficient model for quantitatively describing electron-lattice equilibration in aluminium. We discuss the general applicability of the NLM and provide a criterion for the suitability of the two-temperature approximation for other metals.

We present an analytical approach for bond percolation on multiplex networks and use it to determine the expected size of the giant connected component and the value of the critical bond occupation probability in these networks. We advocate the relevance of these tools to the modeling of multilayer robustness and contribute to the debate on whether any benefit is to be yielded from studying a full multiplex structure as opposed to its monoplex projection, especially in the seemingly irrelevant case of a bond occupation probability that does not depend on the layer. Although we find that in many cases the predictions of our theory for multiplex networks coincide with previously derived results for monoplex networks, we also uncover the remarkable result that for a certain class of multiplex networks, well described by our theory, new critical phenomena occur as multiple percolation phase transitions are present. We provide an instance of this phenomenon in a multiplex network constructed from London rail and European air transportation data sets.

In force sensing, optomechanics, and quantum motion experiments, it is typically advantageous to create lightweight, compliant mechanical elements with the lowest possible force noise. Here, we report the fabrication and characterization of high-aspect-ratio, nanogram-scale ${\mathrm{Si}}_3{\mathrm{N}}_4$ “trampolines” having quality factors above $4\times {10}^7$ and ringdown times exceeding 5 min (mHz linewidth). These devices exhibit thermally limited force noise sensitivities below $20\mathrm{aN}/{\mathrm{Hz}}^{1/2}$ at room temperature, which is the lowest among solid-state mechanical sensors. We also characterize the suitability of these devices for high-finesse cavity readout and optomechanics applications, finding no evidence of surface or bulk optical losses from the processed nitride in a cavity achieving finesse 40,000. These parameters provide access to a single-photon cooperativity $C_0\sim 8$ in the resolved-sideband limit, wherein a variety of outstanding optomechanics goals become feasible.

Power-law dwell times have been observed for molecular motors in living cells, but the origins of these trapped states are not known. We introduce a minimal model of motors moving on a two-dimensional network of filaments, and simulations of its dynamics exhibit statistics comparable to those observed experimentally. Analysis of the model trajectories, as well as experimental particle tracking data, reveals a state in which motors cycle unproductively at junctions of three or more filaments. We formulate a master equation for these junction dynamics and show that the time required to escape from this vortexlike state can account for the power-law dwell times. We identify trends in the dynamics with the motor valency for further experimental validation. We demonstrate that these trends exist in individual trajectories of myosin II on an actin network. We discuss how cells could regulate intracellular transport and, in turn, biological function by controlling their cytoskeletal network structures locally.

In complex systems, the network of interactions we observe between systems components is the aggregate of the interactions that occur through different mechanisms or layers. Recent studies reveal that the existence of multiple interaction layers can have a dramatic impact in the dynamical processes occurring on these systems. However, these studies assume that the interactions between systems components in each one of the layers are known, while typically for real-world systems we do not have that information. Here, we address the issue of uncovering the different interaction layers from aggregate data by introducing multilayer stochastic block models (SBMs), a generalization of single-layer SBMs that considers different mechanisms of layer aggregation. First, we find the complete probabilistic solution to the problem of finding the optimal multilayer SBM for a given aggregate-observed network. Because this solution is computationally intractable, we propose an approximation that enables us to verify that multilayer SBMs are more predictive of network structure in real-world complex systems.

Quantum fluctuations of the gravitational field in the early Universe, amplified by inflation, produce a primordial gravitational-wave background across a broad frequency band. We derive constraints on the spectrum of this gravitational radiation, and hence on theories of the early Universe, by combining experiments that cover 29 orders of magnitude in frequency. These include Planck observations of cosmic microwave background temperature and polarization power spectra and lensing, together with baryon acoustic oscillations and big bang nucleosynthesis measurements, as well as new pulsar timing array and ground-based interferometer limits. While individual experiments constrain the gravitational-wave energy density in specific frequency bands, the combination of experiments allows us to constrain cosmological parameters, including the inflationary spectral index $n_t$ and the tensor-to-scalar ratio $r$. Results from individual experiments include the most stringent nanohertz limit of the primordial background to date from the Parkes Pulsar Timing Array, ${\mathrm{\Omega }}_{\mathrm{GW}}(f)<2.3\times {10}^{-10}$. Observations of the cosmic microwave background alone limit the gravitational-wave spectral index at 95% confidence to $n_t\lesssim 5$ for a tensor-to-scalar ratio of $r=0.11$. However, the combination of all the above experiments limits $n_t<0.36$. Future Advanced LIGO observations are expected to further constrain $n_t<0.34$ by 2020. When cosmic microwave background experiments detect a nonzero $r$, our results will imply even more stringent constraints on $n_t$ and, hence, theories of the early Universe.

We study possible quantum $U(1)$ spin liquids in three dimensions with time-reversal symmetry. We find a total of seven families of such $U(1)$ spin liquids, distinguished by the properties of their emergent electric or magnetic charges. We show how these spin liquids are related to each other. Two of these classes admit nontrivial protected surface states which we describe. We show how to access all of the seven spin liquids through slave particle (parton) constructions. We also provide intuitive loop gas descriptions of their ground-state wave functions. One of these phases is the “topological Mott insulator,” conventionally described as a topological insulator of an emergent fermionic “spinon.” We show that this phase admits a remarkable dual description as a topological insulator of emergent fermionic magnetic monopoles. This results in a new (possibly natural) surface phase for the topological Mott insulator and a new slave particle construction. We describe some of the continuous quantum phase transitions between the different $U(1)$ spin liquids. Each of these seven families of states admits a finer distinction in terms of their surface properties, which we determine by combining these spin liquids with symmetry-protected topological phases. We discuss lessons for materials such as pyrochlore quantum spin ices which may harbor a $U(1)$ spin liquid. We suggest the topological Mott insulator as a possible ground state in some range of parameters for the quantum spin ice Hamiltonian.

Three-dimensional orientational order in systems whose ground states possess nonzero gradients typically exhibits linelike structures or defects: $\lambda$ lines in cholesterics or Skyrmion tubes in ferromagnets, for example. Here, we show that such lines can be identified as a set of natural geometric singularities in a unit vector field, the generalization of the umbilic points of a surface. We characterize these lines in terms of the natural vector bundles that the order defines and show that they give a way to localize and identify Skyrmion distortions in chiral materials—in particular, that they supply a natural representative of the Poincaré dual of the cocycle describing the topology. Their global structure leads to the definition of a self-linking number and helicity integral which relates the linking of umbilic lines to the Hopf invariant of the texture.

We propose and study the use of photon-mediated interactions for the generation of long-range steady-state entanglement between $N$ atoms. Through the judicious use of coherent drives and the placement of the atoms in a network of cavity QED systems, a balance between their unitary and dissipative dynamics can be precisely engineered to stabilize a long-range correlated state of qubits in the steady state. We discuss the general theory behind such a scheme and present an example of how it can be used to drive a register of $N$ atoms to a generalized $W$ state and how the entanglement can be sustained indefinitely. The achievable steady-state fidelities for entanglement and its scaling with the number of qubits are discussed for presently existing superconducting quantum circuits. While the protocol is primarily discussed for a superconducting circuit architecture, it is ideally realized in any cavity QED platform that permits controllable delivery of coherent electromagnetic radiation to specified locations.

The quantized lateral motional states and the spin states of electrons trapped on the surface of superfluid helium have been proposed as basic building blocks of a scalable quantum computer. Circuit quantum electrodynamics allows strong dipole coupling between electrons and a high-$Q$ superconducting microwave resonator, enabling such sensitive detection and manipulation of electron degrees of freedom. Here, we present the first realization of a hybrid circuit in which a large number of electrons are trapped on the surface of superfluid helium inside a coplanar waveguide resonator. The high finesse of the resonator allows us to observe large dispersive shifts that are many times the linewidth and make fast and sensitive measurements on the collective vibrational modes of the electron ensemble, as well as the superfluid helium film underneath. Furthermore, a large ensemble coupling is observed in the dispersive regime during experiment, and it shows excellent agreement with our numeric model. The coupling strength of the ensemble to the cavity is found to be $\approx 1\mathrm{MHz}$ per electron, indicating the feasibility of achieving single electron strong coupling.

We report on self-induced switchings between multiple distinct space-time patterns in the dynamics of a spatially extended excitable system. These switchings between low-amplitude oscillations, nonlinear waves, and extreme events strongly resemble a random process, although the system is deterministic. We show that a chaotic saddle—which contains all the patterns as well as channel-like structures that mediate the transitions between them—is the backbone of such a pattern-switching dynamics. Our analyses indicate that essential ingredients for the observed phenomena are that the system behaves like an inhomogeneous oscillatory medium that is capable of self-generating spatially localized excitations and that is dominated by short-range connections but also features long-range connections. With our findings, we present an alternative to the well-known ways to obtain self-induced pattern switching, namely, noise-induced attractor hopping, heteroclinic orbits, and adaptation to an external signal. This alternative way can be expected to improve our understanding of pattern switchings in spatially extended natural dynamical systems like the brain and the heart.

The metal-insulator transition has been a subject of intense research since Mott first proposed that the metallic behavior of interacting electrons could turn to an insulating one as electron correlations increase. Here, we consider electrons with massless Dirac-like dispersion in two spatial dimensions, described by the Hubbard models on two geometrically different lattices, and perform numerically exact calculations on unprecedentedly large systems that, combined with a careful finite-size scaling analysis, allow us to explore the quantum critical behavior in the vicinity of the interaction-driven metal-insulator transition. Thereby, we find that the transition is continuous, and we determine the quantum criticality for the corresponding universality class, which is described in the continuous limit by the Gross-Neveu model, a model extensively studied in quantum field theory. Furthermore, we discuss a fluctuation-driven scenario for the metal-insulator transition in the interacting Dirac electrons: The metal-insulator transition is triggered only by the vanishing of the quasiparticle weight, not by the Dirac Fermi velocity, which instead remains finite near the transition. This important feature cannot be captured by a simple mean-field or Gutzwiller-type approximate picture but is rather consistent with the low-energy behavior of the Gross-Neveu model.

Progress of silicon-based technology is nearing its physical limit, as the minimum feature size of components is reaching a mere 10 nm. The resistive switching behavior of transition metal oxides and the associated memristor device is emerging as a competitive technology for next-generation electronics. Significant progress has already been made in the past decade, and devices are beginning to hit the market; however, this progress has mainly been the result of empirical trial and error. Hence, gaining theoretical insight is of the essence. In the present work, we report the striking result of a connection between the resistive switching and shock-wave formation, a classic topic of nonlinear dynamics. We argue that the profile of oxygen vacancies that migrate during the commutation forms a shock wave that propagates through a highly resistive region of the device. We validate the scenario by means of model simulations and experiments in a manganese-oxide-based memristor device, and we extend our theory to the case of binary oxides. The shock-wave scenario brings unprecedented physical insight and enables us to rationalize the process of oxygen-vacancy-driven resistive change with direct implications for a key technological aspect—the commutation speed.

In ${\mathrm{ABO}}_3$ perovskites, oxygen octahedron rotations are common structural distortions that can promote large ferroelectricity in ${\text{BiFeO}}_3$ with an $R3c$ structure [1] but suppress ferroelectricity in ${\text{CaTiO}}_3$ with a $Pbnm$ symmetry [2]. For many ${\text{CaTiO}}_3$-like perovskites, the ${\text{BiFeO}}_3$ structure is a metastable phase. Here, we report the stabilization of the highly polar ${\text{BiFeO}}_3$-like phase of ${\text{CaTiO}}_3$ in a ${\text{BaTiO}}_3/{\text{CaTiO}}_3$ superlattice grown on a ${\text{SrTiO}}_3$ substrate. The stabilization is realized by a reconstruction of oxygen octahedron rotations at the interface from the pattern of nonpolar bulk ${\text{CaTiO}}_3$ to a different pattern that is characteristic of a ${\text{BiFeO}}_3$ phase. The reconstruction is interpreted through a combination of amplitude-contrast sub-0.1-nm high-resolution transmission electron microscopy and first-principles theories of the structure, energetics, and polarization of the superlattice and its constituents. We further predict a number of new artificial ferroelectric materials demonstrating that nonpolar perovskites can be turned into ferroelectrics via this interface mechanism. Therefore, a large number of perovskites with the ${\text{CaTiO}}_3$ structure type, which include many magnetic representatives, are now good candidates as novel highly polar multiferroic materials [3].

The semiconductor polariton laser promises a new source of coherent light, which, compared to conventional semiconductor photon lasers, has input-energy threshold orders of magnitude lower. However, intensity stability, a defining feature of a coherent state, has remained poor. Intensity noise many times the shot noise of a coherent state has persisted, attributed to multiple mechanisms that are difficult to separate in conventional polariton systems. The large intensity noise, in turn, limits the phase coherence. Thus, the capability of the polariton laser as a source of coherence light is limited. Here, we demonstrate a polariton laser with shot-noise-limited intensity stability, as expected from a fully coherent state. This stability is achieved by using an optical cavity with high mode selectivity to enforce single-mode lasing, suppress condensate depletion, and establish gain saturation. Moreover, the absence of spurious intensity fluctuations enables the measurement of a transition from exponential to Gaussian decay of the phase coherence of the polariton laser. It suggests large self-interaction energies in the polariton condensate, exceeding the laser bandwidth. Such strong interactions are unique to matter-wave lasers and important for nonlinear polariton devices. The results will guide future development of polariton lasers and nonlinear polariton devices.

Today’s narrowest linewidth lasers are limited by mirror motion in the reference optical resonator used to stabilize the laser’s frequency. Recent proposals suggest that superradiant lasers based on narrow dipole-forbidden transitions in cold alkaline earth atoms could offer a way around this limitation. Such lasers operating on transitions with linewidth of order mHz are predicted to achieve output spectra orders of magnitude narrower than any currently existing laser. As a step towards this goal, we demonstrate and study a laser based on the 7.5-kHz linewidth dipole-forbidden ${}^3{P}_1$ to ${}^1{S}_0$ transition in laser-cooled and tightly confined ${}^{88}\mathrm{Sr}$. We can operate this laser in the bad-cavity or superradiant regime, where coherence is primarily stored in the atoms, or continuously tune to the more conventional good-cavity regime, where coherence is primarily stored in the light field. We show that the cold-atom gain medium can be repumped to achieve quasi-steady-state lasing. We also demonstrate up to an order of magnitude suppression in the sensitivity of laser frequency to changes in cavity length, verifying a key feature of the proposed narrow linewidth lasers.

Quantum cryptography holds the promise to establish an information-theoretically secure global network. All field tests of metropolitan-scale quantum networks to date are based on trusted relays. The security critically relies on the accountability of the trusted relays, which will break down if the relay is dishonest or compromised. Here, we construct a measurement-device-independent quantum key distribution (MDIQKD) network in a star topology over a 200-square-kilometer metropolitan area, which is secure against untrustful relays and against all detection attacks. In the field test, our system continuously runs through one week with a secure key rate 10 times larger than previous results. Our results demonstrate that the MDIQKD network, combining the best of both worlds—security and practicality, constitutes an appealing solution to secure metropolitan communications.

Tensor network algorithms provide a suitable route for tackling real-time-dependent problems in lattice gauge theories, enabling the investigation of out-of-equilibrium dynamics. We analyze a U(1) lattice gauge theory in ($1+1$) dimensions in the presence of dynamical matter for different mass and electric-field couplings, a theory akin to quantum electrodynamics in one dimension, which displays string breaking: The confining string between charges can spontaneously break during quench experiments, giving rise to charge-anticharge pairs according to the Schwinger mechanism. We study the real-time spreading of excitations in the system by means of electric-field and particle fluctuations. We determine a dynamical state diagram for string breaking and quantitatively evaluate the time scales for mass production. We also show that the time evolution of the quantum correlations can be detected via bipartite von Neumann entropies, thus demonstrating that the Schwinger mechanism is tightly linked to entanglement spreading. To present a variety of possible applications of this simulation platform, we show how one could follow the real-time scattering processes between mesons and the creation of entanglement during scattering processes. Finally, we test the quality of quantum simulations of these dynamics, quantifying the role of possible imperfections in cold atoms, trapped ions, and superconducting circuit systems. Our results demonstrate how entanglement properties can be used to deepen our understanding of basic phenomena in the real-time dynamics of gauge theories such as string breaking and collisions.