- Open Access
Emergent Gauge Flux in Mixed with Flavor Chemical Potential: Implications for Magnetized U(1) Dirac Spin Liquids
Phys. Rev. X 16, 041029 – Published 30 October, 2026
DOI: https://doi.org/10.1103/yb9y-3t91
Abstract
We design a lattice model of a “mixed” U(1) gauge field coupled to fermions with a flavor chemical potential and solve it with large-scale determinant quantum Monte Carlo simulations. In this mixed construction, dynamical magnetic monopole events are suppressed in the temporal-continuum limit. For zero flavor chemical potential, the model realizes three-dimensional quantum electrodynamics () which has been argued to describe the ground state and low-energy excitations of the Dirac spin liquid phase of quantum antiferromagnets. At finite flavor chemical potential, which corresponds to a Zeeman field perturbing the Dirac spin liquid, we find a “chiral flux” phase which is characterized by the generation of a finite mean emergent gauge flux and, accordingly, the formation of relativistic Landau levels for the Dirac fermions. We use field-theory arguments to argue that in this state a magnetic symmetry is spontaneously broken, leading to a gapless photon mode. Because of spin-flux attachment this mode would contribute to the low-energy longitudinal spin response. We numerically compute longitudinal and transverse spin structure factors which match our continuum and lattice mean-field theory predictions. In a different region of the phase diagram, strong fluctuations of the emergent gauge field give rise to an antiferromagnetically ordered state with gapped Dirac fermions coexisting with a deconfined gauge field. We also find an interesting intermediate phase where the chiral flux phase and the antiferromagnetic phase coexist. We argue that our results pave the way to testable predictions for magnetized Dirac spin liquids in frustrated quantum antiferromagnets.
Physics Subject Headings (PhySH)
Popular Summary
Dirac spin liquids are intriguing states of matter characterized by fractionalized excitations, with their low-energy physics described by a strongly interacting emergent gauge theory. How this fractionalization and the emergent gauge dynamics manifest themselves in response to an external magnetic field has remained challenging. We performed large-scale quantum Monte Carlo simulations and field-theoretic analyses of a quantum lattice model of fermionic spinons subject to an applied flavor chemical potential corresponding to a Zeeman magnetic field. We identified a chiral flux phase, in which the system spontaneously generates a net emergent gauge flux, and neighboring antiferromagnetic and coexisting phases within the global phase diagram. In the chiral flux phase, the spectrum of Dirac spinons is organized into relativistic Landau levels. Our numerical calculations exhibit signatures of a gapless excitation that we argue to be consistent with the photon mode of the emergent gauge field predicted by field theory. Our work provides concrete dynamical spin structure factor predictions, establishing neutron scattering signatures to detect emergent gauge fields and fractionalization in frustrated magnets.
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References (81)
- N. Karthik and R. Narayanan, No evidence for bilinear condensate in parity-invariant three-dimensional QED with massless fermions, Phys. Rev. D 93, 045020 (2016).
- S. Giombi, I. R. Klebanov, and G. Tarnopolsky, Conformal , F-theorem and the -expansion, J. Phys. A 49, 135403 (2016).
- L. Di Pietro and E. Stamou, Scaling dimensions in QED3 from the -expansion, J. High Energy Phys. 12 (2017) 054.
- Y.-C. He, J. Rong, and N. Su, Conformal bootstrap bounds for the Dirac spin liquid and Stiefel liquid, SciPost Phys. 13, 014 (2022).
- M. Hermele, T. Senthil, M. P. A. Fisher, P. A. Lee, N. Nagaosa, and X.-G. Wen, Stability of spin liquids in two dimensions, Phys. Rev. B 70, 214437 (2004).
- M. Hermele, T. Senthil, and M. P. A. Fisher, Algebraic spin liquid as the mother of many competing orders, Phys. Rev. B 72, 104404 (2005).
- Y. Ran, M. Hermele, P. A. Lee, and X.-G. Wen, Projected-wave-function study of the spin- Heisenberg model on the kagomé lattice, Phys. Rev. Lett. 98, 117205 (2007).
- S. Albayrak, R. S. Erramilli, Z. Li, D. Poland, and Y. Xin, Bootstrapping conformal , Phys. Rev. D 105, 085008 (2022).
- S. M. Chester and S. S. Pufu, Towards bootstrapping QED3, J. High Energy Phys. 08 (2016) 019.
- X.-Y. Song, C. Wang, A. Vishwanath, and Y.-C. He, Unifying description of competing orders in two-dimensional quantum magnets, Nat. Commun. 10, 4254 (2019).
- A. Wietek, S. Capponi, and A. M. Läuchli, Quantum electrodynamics in dimensions as the organizing principle of a triangular lattice antiferromagnet, Phys. Rev. X 14, 021010 (2024).
- Z.-X. Luo, U. F. P. Seifert, and L. Balents, Twisted bilayer U(1) Dirac spin liquids, Phys. Rev. B 106, 144437 (2022).
- G. Nambiar, D. Bulmash, and V. Galitski, Monopole Josephson effects in a Dirac spin liquid, Phys. Rev. Res. 5, 013169 (2023).
- U. F. P. Seifert, J. Willsher, M. Drescher, F. Pollmann, and J. Knolle, Spin-Peierls instability of the U(1) Dirac spin liquid, Nat. Commun. 15, 7110 (2024).
- M. B. Hastings, Dirac structure, RVB, and Goldstone modes in the kagomé antiferromagnet, Phys. Rev. B 63, 014413 (2000).
- Y. Iqbal, F. Becca, and D. Poilblanc, Projected wave function study of spin liquids on the kagome lattice for the spin- quantum Heisenberg antiferromagnet, Phys. Rev. B 84, 020407 (2011).
- Y.-C. He, M. P. Zaletel, M. Oshikawa, and F. Pollmann, Signatures of Dirac cones in a DMRG study of the kagome Heisenberg model, Phys. Rev. X 7, 031020 (2017).
- X. Lu, A. Raikos, M. Song, Z. Li, L. Han, S. Li, S. Capponi, Z. Y. Meng, and C. Zhou, Unraveling the kagome antiferromagnetic model and its materials: An integrated approach, arXiv:2609.11745.
- R. Kaneko, S. Morita, and M. Imada, Gapless spin-liquid phase in an extended spin triangular Heisenberg model, J. Phys. Soc. Jpn. 83, 093707 (2014).
- Z. Zhu and S. R. White, Spin liquid phase of the Heisenberg model on the triangular lattice, Phys. Rev. B 92, 041105 (2015).
- W.-J. Hu, S.-S. Gong, W. Zhu, and D. N. Sheng, Competing spin-liquid states in the spin- Heisenberg model on the triangular lattice, Phys. Rev. B 92, 140403 (2015).
- Y. Iqbal, W.-J. Hu, R. Thomale, D. Poilblanc, and F. Becca, Spin liquid nature in the Heisenberg triangular antiferromagnet, Phys. Rev. B 93, 144411 (2016).
- S.-S. Gong, W. Zhu, J.-X. Zhu, D. N. Sheng, and K. Yang, Global phase diagram and quantum spin liquids in a spin- triangular antiferromagnet, Phys. Rev. B 96, 075116 (2017).
- S. N. Saadatmand and I. P. McCulloch, Detection and characterization of symmetry-broken long-range orders in the spin- triangular Heisenberg model, Phys. Rev. B 96, 075117 (2017).
- S. Hu, W. Zhu, S. Eggert, and Y.-C. He, Dirac spin liquid on the spin- triangular Heisenberg antiferromagnet, Phys. Rev. Lett. 123, 207203 (2019).
- F. Ferrari, J. Willsher, U. F. P. Seifert, R. Valentí, and J. Knolle, Stability of algebraic spin liquids coupled to quantum phonons, Phys. Rev. Res. 7, L042053 (2025).
- F. Ferrari and F. Becca, Dynamical structure factor of the Heisenberg model on the triangular lattice: Magnons, spinons, and gauge fields, Phys. Rev. X 9, 031026 (2019).
- N. E. Sherman, M. Dupont, and J. E. Moore, Spectral function of the Heisenberg model on the triangular lattice, Phys. Rev. B 107, 165146 (2023).
- M. Drescher, L. Vanderstraeten, R. Moessner, and F. Pollmann, Dynamical signatures of symmetry-broken and liquid phases in an Heisenberg antiferromagnet on the triangular lattice, Phys. Rev. B 108, L220401 (2023).
- J. Willsher and J. Knolle, Dynamics and stability of U(1) spin liquids beyond mean-field theory: Triangular-lattice Heisenberg model, arXiv:2503.13831.
- Y. Ran, W.-H. Ko, P. A. Lee, and X.-G. Wen, Spontaneous spin ordering of a Dirac spin liquid in a magnetic field, Phys. Rev. Lett. 102, 047205 (2009).
- T. T. Dumitrescu, P. Niro, and R. Thorngren, Symmetry breaking from monopole condensation in , arXiv:2410.05366.
- X. Y. Xu, Y. Qi, L. Zhang, F. F. Assaad, C. Xu, and Z. Y. Meng, Monte Carlo study of lattice compact quantum electrodynamics with fermionic matter: The parent state of quantum phases, Phys. Rev. X 9, 021022 (2019).
- W. Wang, D.-C. Lu, X. Y. Xu, Y.-Z. You, and Z. Y. Meng, Dynamics of compact quantum electrodynamics at large fermion flavor, Phys. Rev. B 100, 085123 (2019).
- L. Janssen, W. Wang, M. M. Scherer, Z. Y. Meng, and X. Y. Xu, Confinement transition in the -Gross-Neveu-XY universality class, Phys. Rev. B 101, 235118 (2020).
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/yb9y-3t91 for details of the lattice mean-field and continuum field-theory calculations, DQMC and SAC methods, and supplementary results, which includes Ref. [37].
- I. S. Gradshteyn, I. M. Ryzhik, D. Zwillinger, and V. Moll, Table of Integrals, Series, and Products, 8th ed. (Academic Press, Amsterdam, 2015).
- G. Pan and Z. Y. Meng, The sign problem in quantum Monte Carlo simulations, in Encyclopedia of Condensed Matter Physics (Second Edition), edited by T. Chakraborty (Academic Press, Oxford, 2024), pp. 879–893, 10.1016/B978-0-323-90800-9.00095-0.
- R. Blankenbecler, D. Scalapino, and R. Sugar, Monte Carlo calculations of coupled boson-fermion systems. I, Phys. Rev. D 24, 2278 (1981).
- F. F. Assaad and H. G. Evertz, World-line and determinantal quantum Monte Carlo methods for spins, phonons and electrons, in Computational Many-Particle Physics, Lecture Notes in Physics, edited by H. Fehske, R. Schneider, and A. Weiße (Springer, Berlin, Heidelberg, 2008), Vol. 739, pp. 277–356, 10.1007/978-3-540-74686-7_10.
- X. Y. Xu, Z. Hong Liu, G. Pan, Y. Qi, K. Sun, and Z. Y. Meng, Revealing fermionic quantum criticality from new Monte Carlo techniques, J. Phys. Condens. Matter 31, 463001 (2019).
- F. F. Assaad, M. Bercx, F. Goth, A. Götz, J. S. Hofmann, E. Huffman, Z. Liu, F. P. Toldin, J. S. E. Portela, and J. Schwab, The ALF (Algorithms for Lattice Fermions) project release 2.0. Documentation for the auxiliary-field quantum Monte Carlo code, SciPost Phys. Codebases 1 (2022).
- W. Jiang, Y. Liu, A. Klein, Y. Wang, K. Sun, A. V. Chubukov, and Z. Y. Meng, Monte Carlo study of the pseudogap and superconductivity emerging from quantum magnetic fluctuations, Nat. Commun. 13, 2655 (2022).
- E. Fradkin, Field Theories of Condensed Matter Physics, 2nd ed. (Cambridge University Press, Cambridge, 2013).
- A. Zee, Quantum Field Theory in a Nutshell, 2nd ed. (Princeton University Press, Princeton, NJ, 2010).
- D. R. Hofstadter, Energy levels and wave functions of Bloch electrons in rational and irrational magnetic fields, Phys. Rev. B 14, 2239 (1976).
- L. Balents and O. A. Starykh, Collective spinon spin wave in a magnetized U(1) spin liquid, Phys. Rev. B 101, 020401 (2020).
- M. Agarwal, O. A. Starykh, D. A. Pesin, and E. G. Mishchenko, Collective spin oscillations in a magnetized graphene sheet, Phys. Rev. B 109, 224302 (2024).
- C. Chen, Y. Da Liao, C. Zhou, G. Pan, Z. Y. Meng, and Y. Qi, Universal collective Larmor-Silin mode emerging in magnetized correlated Dirac fermions, Phys. Rev. B 110, L121112 (2024).
- A. W. Sandvik, Stochastic method for analytic continuation of quantum Monte Carlo data, Phys. Rev. B 57, 10287 (1998).
- K. S. D. Beach, Identifying the maximum entropy method as a special limit of stochastic analytic continuation, arXiv:cond-mat/0403055.
- O. F. Syljuåsen, Using the average spectrum method to extract dynamics from quantum Monte Carlo simulations, Phys. Rev. B 78, 174429 (2008).
- A. W. Sandvik, Constrained sampling method for analytic continuation, Phys. Rev. E 94, 063308 (2016).
- H. Shao, Y. Q. Qin, S. Capponi, S. Chesi, Z. Y. Meng, and A. W. Sandvik, Nearly deconfined spinon excitations in the square-lattice spin- Heisenberg antiferromagnet, Phys. Rev. X 7, 041072 (2017).
- C. Zhou, Z. Yan, H.-Q. Wu, K. Sun, O. A. Starykh, and Z. Y. Meng, Amplitude mode in quantum magnets via dimensional crossover, Phys. Rev. Lett. 126, 227201 (2021).
- G.-Y. Sun, Y.-C. Wang, C. Fang, Y. Qi, M. Cheng, and Z. Y. Meng, Dynamical signature of symmetry fractionalization in frustrated magnets, Phys. Rev. Lett. 121, 077201 (2018).
- C.-J. Huang, Y. Deng, Y. Wan, and Z. Y. Meng, Dynamics of topological excitations in a model quantum spin ice, Phys. Rev. Lett. 120, 167202 (2018).
- Y.-C. Wang, M. Cheng, W. Witczak-Krempa, and Z. Y. Meng, Fractionalized conductivity and emergent self-duality near topological phase transitions, Nat. Commun. 12, 5347 (2021).
- N. Ma, G.-Y. Sun, Y.-Z. You, C. Xu, A. Vishwanath, A. W. Sandvik, and Z. Y. Meng, Dynamical signature of fractionalization at a deconfined quantum critical point, Phys. Rev. B 98, 174421 (2018).
- C. Huang, N. Parthenios, M. Ulybyshev, X. Zhang, F. F. Assaad, L. Classen, and Z. Y. Meng, Angle-tuned Gross-Neveu quantum criticality in twisted bilayer graphene, Nat. Commun. 16, 7176 (2025).
- O. F. Syljuåsen, Numerical evidence for unstable magnons at high fields in the Heisenberg antiferromagnet on the square lattice, Phys. Rev. B 78, 180413 (2008).
- A. Lüscher and A. M. Läuchli, Exact diagonalization study of the antiferromagnetic spin- Heisenberg model on the square lattice in a magnetic field, Phys. Rev. B 79, 195102 (2009).
- M. Mourigal, M. E. Zhitomirsky, and A. L. Chernyshev, Field-induced decay dynamics in square-lattice antiferromagnets, Phys. Rev. B 82, 144402 (2010).
- K. Feng, C. Chen, and Z. Y. Meng, Scalable hybrid quantum Monte Carlo simulation of gauge field coupled to fermions on GPU, SciPost Phys. 20, 060 (2026).
- W. O. Wang, U. F. P. Seifert, O. A. Starykh, and L. Balents, Chirality and quasi-long-range order in finite-flux Gutzwiller states for magnetized frustrated magnets, Phys. Rev. Lett. 137, 076701 (2026).
- R. Bag, S. Xu, N. E. Sherman, L. Yadav, A. I. Kolesnikov, A. A. Podlesnyak, E. S. Choi, I. da Silva, J. E. Moore, and S. Haravifard, Evidence of Dirac quantum spin liquid in , Phys. Rev. Lett. 133, 266703 (2024).
- H. C. H. Wu, F. L. Pratt, B. M. Huddart, D. Chatterjee, P. A. Goddard, J. Singleton, D. Prabhakaran, and S. J. Blundell, Spin dynamics in the Dirac spin liquid , Phys. Rev. Lett. 135, 046704 (2025).
- A. O. Scheie et al., Proximate spin liquid and fractionalization in the triangular antiferromagnet , Nat. Phys. 20, 74 (2024).
- A. O. Scheie, M. Lee, K. Wang, P. Laurell, E. S. Choi, D. Pajerowski, Q. Zhang, J. Ma, H. D. Zhou, S. Lee, C. Huan, S. M. Thomas, M. O. Ajeesh, P. F. S. Rosa, A. Chen, V. S. Zapf, M. Heyl, C. D. Batista, E. Dagotto, J. E. Moore, and D. A. Tennant, Spectrum and low-temperature bulk properties of triangular quantum spin liquid candidate , arXiv:2406.17773.
- Z. Zeng, C. Zhou, H. Zhou, L. Han, R. Chi, K. Li, M. Kofu, K. Nakajima, Y. Wei, W. Zhang, D. G. Mazzone, Z. Y. Meng, and S. Li, Spectral evidence for Dirac spinons in a kagome lattice antiferromagnet, Nat. Phys. 20, 1097 (2024).
- L. Han, Z. Zeng, M. Long, M. Song, C. Zhou, B. Liu, M. Kofu, K. Nakajima, P. Steffens, A. Hiess, Z. Y. Meng, Y. Su, and S. Li, Spin excitations arising from anisotropic Dirac spinons in , Phys. Rev. B 112, 045114 (2025).
- Z. Y. Meng, C. D. Batista, and S. Li, An integrated theoretical and numerical approach to understand modern experiments on quantum magnetism, Nat. Phys. 22, 1189 (2026).
- G. Zheng, Y. Zhu, K.-W. Chen, B. Kang, D. Zhang, K. Jenkins, A. Chan, Z. Zeng, A. Xu, O. A. Valenzuela, J. Blawat, J. Singleton, S. Li, P. A. Lee, and L. Li, Unconventional magnetic oscillations in a kagome Mott insulator, Proc. Natl. Acad. Sci. U.S.A. 122, e2421390122 (2025).
- I. S. Villadiego, Pseudoscalar U(1) spin liquids in , Phys. Rev. B 104, 195149 (2021).
- X.-Y. Song, H. Goldman, and L. Fu, Emergent from half-filled flat Chern bands, Phys. Rev. B 108, 205123 (2023).
- F. Paoletti, D. Guerci, G. Sangiovanni, U. F. P. Seifert, and E. J. König, Topologically enabled superconductivity: Possible implications for rhombohedral graphene, arXiv:2504.13166.
- T. Wang, X.-Y. Song, M. P. Zaletel, and T. Senthil, Emergent at the bosonic Laughlin state to superfluid transition, arXiv:2507.07611.
- T. T. Dumitrescu and J. Maldacena, Comments on in a magnetic field, arXiv:2508.03532.
- A. Keselman, X. Xu, H. Zhang, C. D. Batista, and O. A. Starykh, Magnetization plateaux as a roadmap to quantum spin liquids, Phys. Rev. Lett. 137, 116702 (2026).
- T. Bader, S. Feng, S. Budaraju, F. Becca, J. Knolle, and F. Pollmann, Triangular Heisenberg antiferromagnet in a magnetic field, Phys. Rev. B 113, L241114 (2026).
- C. Chen, U. F. P. Seifert, K. Feng, O. A. Starykh, L. Balents, and Z. Y. Meng, Numerical data for emergent gauge flux in mixed with flavor chemical potential, [Dataset], GitHub repository, https://github.com/baucd/mixed_qed3_cf_data (2026).
