- Open Access
Unified Description of Cuprate Superconductors by Fractionalized Electrons Emerging from Integrated Analyses of Photoemission Spectra and Quasiparticle Interference
Phys. Rev. X 16, 011018 – Published 4 February, 2026
DOI: https://doi.org/10.1103/mww7-32gn
Abstract
Electronic structure of high-temperature superconducting cuprates is studied by analyzing experimental data independently obtained from two complementary spectroscopies: one, quasiparticle interference (QPI) measured by scanning-tunneling microscopy, and the other, angle-resolved photoemission spectroscopy (ARPES). We combine these two sets of data in a unified theoretical analysis. Through explicit calculations of experimentally measurable quantities, we show that a simple two-component fermion model (TCFM) representing electron fractionalization succeeds in reproducing various detailed features of these experimental data: ARPES and QPI data are concomitantly reproduced by the TCFM in full energy and momentum spaces. The measured QPI pattern reveals a signature characteristic of the TCFM, distinct from the conventional single-component prediction, supporting the validity of the electron fractionalization in the cuprates. The integrated analysis also solves the puzzles of ARPES and QPI data that are seemingly inconsistent with each other. The overall success of the TCFM offers a comprehensive understanding of the electronic structure of the cuprates, in particular, the unoccupied side of the spectra, of which momentum-resolved structure has long been unexplored experimentally. We further predict that a characteristic QPI pattern should appear in the unoccupied high-energy part if the fractionalization is at work. We propose that integrated-spectroscopy analyses offer a promising way to explore challenging issues of strongly correlated electron systems.
Physics Subject Headings (PhySH)
- Electrical properties
- Electron-mediated pairing
- Electronic structure
- Fractionalization
- Impurities in superconductors
- Pairing mechanisms
- Pseudogap
- Quasiparticles & collective excitations
- Superconducting gap
- Superconductivity
- High-temperature superconductors
- Strongly correlated systems
- Angle-resolved photoemission spectroscopy
- Green's function methods
- Lattice models in condensed matter
- Scanning tunneling microscopy
- Scanning tunneling spectroscopy
Popular Summary
Unresolved questions surrounding the mechanism of high-temperature superconductivity in cuprates frequently persist because data from various spectroscopic tools are usually analyzed independently, using sometimes conflicting theories. We addressed this challenge by performing integrated analyses of angle-resolved photoemission spectroscopy and scanning-tunneling microscopy data within a single, unified theoretical framework. By comparing raw experimental data directly with calculated measurable quantities rather than conventional theoretical replacements, we demonstrated that a model incorporating electron fractionalization quantitatively explains both sets of measurements. Our findings are supported by a specific signal in the quasiparticle interference phase-reference map that confirms the reality of fractionalized electrons in these materials. This success suggests that wider integrated analyses incorporating data from other complementary probes, such as neutron scattering, x-ray scattering, and optics, will provide a new avenue for resolving the long-standing mysteries of strongly correlated electron systems.
Article Text
Supplemental Material
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