Antiferromagnetic materials feature intrinsic ultrafast spin dynamics, making them ideal candidates for future magnonic devices operating at THz frequencies. A major focus of current research is the investigation of optical methods for the efficient generation of coherent magnons in antiferromagnetic insulators. In magnetic lattices endowed with orbital angular momentum, spin-orbit coupling enables spin dynamics through the resonant excitation of low-energy electric dipoles such as phonons and orbital resonances which interact with spins. However, in magnetic systems with zero orbital angular momentum, microscopic pathways for the resonant and low-energy optical excitation of coherent spin dynamics are lacking. Here, we consider experimentally the relative merits of electronic and vibrational excitations for the optical control of zero orbital angular momentum magnets, focusing on a limit case: the antiferromagnet manganese phosphorous trisulfide (${\mathrm{MnPS}}_3$), constituted by orbital singlet ${\mathrm{Mn}}^{2+}$ ions. We study the correlation of spins with two types of excitations within its band gap: a bound electron orbital excitation from the singlet orbital ground state of ${\mathrm{Mn}}^{2+}$ into an orbital triplet state, which causes coherent spin precession, and a vibrational excitation of the crystal field that causes thermal spin disorder. Our findings cast orbital transitions as key targets for magnetic control in insulators constituted by magnetic centers of zero orbital angular momentum.

We study the diffusion of particles confined close to a single wall and in double-wall planar channel geometries where the local diffusivities depend on the distance to the boundaries. Displacement parallel to the walls is Brownian as characterized by its variance, but it is non-Gaussian having a nonzero fourth cumulant. Establishing a link with Taylor dispersion, we calculate the fourth cumulant and the tails of the displacement distribution for general diffusivity tensors along with potentials generated by either the walls or externally, for instance, gravity. Experimental and numerical studies of the motion of a colloid in the direction parallel to the wall give measured fourth cumulants which are correctly predicted by our theory. Interestingly, contrary to models of Brownian-yet-non-Gaussian diffusion, the tails of the displacement distribution are shown to be Gaussian rather than exponential. All together, our results provide additional tests and constraints for the inference of force maps and local transport properties near surfaces.

The long theorized two-dimensional allotrope of SiC has remained elusive amid the exploration of graphenelike honeycomb structured monolayers. It is anticipated to possess a large direct band gap (2.5 eV), ambient stability, and chemical versatility. While $s{p}^2$ bonding between silicon and carbon is energetically favorable, only disordered nanoflakes have been reported to date. Here we demonstrate large-area, bottom-up synthesis of monocrystalline, epitaxial monolayer honeycomb SiC atop ultrathin transition metal carbide films on SiC substrates. We find the 2D phase of SiC to be almost planar and stable at high temperatures, up to $1200°\mathrm{C}$ in vacuum. Interactions between the 2D-SiC and the transition metal carbide surface result in a Dirac-like feature in the electronic band structure, which in the case of a TaC substrate is strongly spin-split. Our findings represent the first step towards routine and tailored synthesis of 2D-SiC monolayers, and this novel heteroepitaxial system may find diverse applications ranging from photovoltaics to topological superconductivity.

The electron magnetic moment, $-\mu /{\mu }_B=g/2=1.00115965218059(13)$ [0.13 ppt], is determined 2.2 times more accurately than the value that stood for fourteen years. The most precisely determined property of an elementary particle tests the most precise prediction of the standard model (SM) to 1 part in ${10}^{12}$. The test would improve an order of magnitude if the uncertainty from discrepant measurements of the fine structure constant $\alpha$ is eliminated since the SM prediction is a function of $\alpha$. The new measurement and SM theory together predict ${\alpha }^{-1}=137.035999166(15)$ [0.11 ppb] with an uncertainty 10 times smaller than the current disagreement between measured $\alpha$ values.

The Majorana Demonstrator searched for neutrinoless double-$\beta$ decay ($0\nu \beta \beta$) of ${}^{76}\mathrm{Ge}$ using modular arrays of high-purity Ge detectors operated in vacuum cryostats in a low-background shield. The arrays operated with up to 40.4 kg of detectors (27.2 kg enriched to $\sim 88\%$ in ${}^{76}\mathrm{Ge}$). From these measurements, the Demonstrator has accumulated 64.5 kg yr of enriched active exposure. With a world-leading energy resolution of 2.52 keV FWHM at the 2039 keV $Q_{\beta \beta }$ (0.12%), we set a half-life limit of $0\nu \beta \beta$ in ${}^{76}\mathrm{Ge}$ at $T_{1/2}>8.3\times {10}^{25}\mathrm{yr}$ (90% C.L.). This provides a range of upper limits on $m_{\beta \beta }$ of (113–269) meV (90% C.L.), depending on the choice of nuclear matrix elements.

We propose a non-Hermitian generalization of the correspondence between the spectral flow and the topological charges of band crossing points (Berry-Chern monopoles). A class of non-Hermitian Hamiltonians that display a complex-valued spectral flow is built by deforming an Hermitian model while preserving its analytical index. We relate those spectral flows to a generalized Chern number that we show to be equal to that of the Hermitian case, provided a line gap exists. We demonstrate the homotopic invariance of both the non-Hermitian Chern number and the spectral flow index, making explicit their topological nature. In the absence of a line gap, our system still displays a spectral flow whose topology can be captured by exploiting an emergent pseudo-Hermitian symmetry.

Superradiance occurs when a collection of atoms exhibits a cooperative, spontaneous emission of photons at a rate that exceeds that of its component parts. Here, we reveal a similar phenomenon in a hydrodynamic system consisting of a pair of vibrationally excited cavities, coupled through their common wave field, that spontaneously emit droplets via interfacial fracture. We show that the droplet emission rate of two coupled cavities is higher than the emission rate of two isolated cavities. Moreover, the amplified emission rate varies sinusoidally with distance between the cavities, as is characteristic of superradiance. We thus present a hydrodynamic phenomenon that captures several essential features of superradiance in optical systems.

Quantum entanglement is an indispensable resource for implementing quantum information processing. The scale of quantum entanglement directly determines its quantum information processing capability. Therefore, it is of great importance to generate ultra-large-scale (ULS) quantum entanglement for the development of quantum information science and technology. Many efforts have been made to increase the scale of quantum entanglement. Recently, time-domain multiplexing has been introduced into continuous-variable (CV) quantum systems to greatly enlarge the scale of quantum entanglement. In this Letter, based on a time-delayed quantum interferometer, we theoretically propose and experimentally demonstrate a scheme for generating an ULS CV deterministic entanglement containing $2\times 20400$ optical modes. In addition, such ULS entanglement contains 81 596 squeezed modes. Our results provide a new platform for implementing ULS CV quantum information processing.

Ultracompact objects with light rings (LRs) but without an event horizon could mimic black holes (BHs) in their strong gravity phenomenology. But are such objects dynamically viable? Stationary and axisymmetric ultracompact objects that can form from smooth, quasi-Minkowski initial data must have at least one stable LR, which has been argued to trigger a spacetime instability; but its development and fate have been unknown. Using fully nonlinear numerical evolutions of ultracompact bosonic stars free of any other known instabilities and introducing a novel adiabatic effective potential technique, we confirm the LRs triggered instability, identifying two possible fates: migration to nonultracompact configurations or collapse to BHs. In concrete examples we show that typical migration (collapse) timescales are not larger than $\sim {10}^3$ light-crossing times, unless the stable LR potential well is very shallow. Our results show that the LR instability is effective in destroying horizonless ultracompact objects that could be plausible BH imitators.

The COHERENT Collaboration searched for scalar dark matter particles produced at the Spallation Neutron Source with masses between 1 and $220\mathrm{MeV}/{\mathrm{c}}^2$ using a CsI[Na] scintillation detector sensitive to nuclear recoils above $9{\mathrm{keV}}_{\mathrm{nr}}$. No evidence for dark matter is found and we thus place limits on allowed parameter space. With this low-threshold detector, we are sensitive to coherent elastic scattering between dark matter and nuclei. The cross section for this process is orders of magnitude higher than for other processes historically used for accelerator-based direct-detection searches so that our small, 14.6 kg detector significantly improves on past constraints. At peak sensitivity, we reject the flux consistent with the cosmologically observed dark-matter concentration for all coupling constants ${\alpha }_D<0.64$, assuming a scalar dark-matter particle. We also calculate the sensitivity of future COHERENT detectors to dark-matter signals which will ambitiously test multiple dark-matter spin scenarios.

When small bubbles rupture in a contaminated water source, the resulting liquid jet breaks up into droplets that can aerosolize solid particulates such as bacteria, viruses, and microplastics. Particles collected on the bubble surface have the potential to become highly concentrated in the jet drops, dramatically increasing their impact. It has been assumed that only particles small enough to fit within a thin microlayer surrounding the bubble can be transported into its influential top jet drop. Yet here, we demonstrate that not only can larger particles be transported into this jet drop, but also that these particles can exceed previous enrichment measurements. Through experiments and simulations, we identify the prerupture location of the liquid that develops into the top jet drop and model how interfacial rearrangement combines with the bubble size, particle size, and the angular distribution of particles on the bubble surface to set the particle enrichment.

We report on an elementary quantum network of two atomic ions separated by 230 m. The ions are trapped in different buildings and connected with 520(2) m of optical fiber. At each network node, the electronic state of an ion is entangled with the polarization state of a single cavity photon; subsequent to interference of the photons at a beam splitter, photon detection heralds entanglement between the two ions. Fidelities of up to $(88.0+2.2-4.7)\%$ are achieved with respect to a maximally entangled Bell state, with a success probability of $4\times {10}^{-5}$. We analyze the routes to improve these metrics, paving the way for long-distance networks of entangled quantum processors.

The KamLAND-Zen experiment has provided stringent constraints on the neutrinoless double-beta ($0\nu \beta \beta$) decay half-life in ${}^{136}\mathrm{Xe}$ using a xenon-loaded liquid scintillator. We report an improved search using an upgraded detector with almost double the amount of xenon and an ultralow radioactivity container, corresponding to an exposure of 970 kg yr of ${}^{136}\mathrm{Xe}$. These new data provide valuable insight into backgrounds, especially from cosmic muon spallation of xenon, and have required the use of novel background rejection techniques. We obtain a lower limit for the $0\nu \beta \beta$ decay half-life of $T_{1/2}^{0\nu }>2.3\times {10}^{26}\mathrm{yr}$ at 90% C.L., corresponding to upper limits on the effective Majorana neutrino mass of 36–156 meV using commonly adopted nuclear matrix element calculations.

Homophily, the tendency of humans to attract each other when sharing similar features, traits, or opinions, has been identified as one of the main driving forces behind the formation of structured societies. Here we ask to what extent homophily can explain the formation of social groups, particularly their size distribution. We propose a spin-glass-inspired framework of self-assembly, where opinions are represented as multidimensional spins that dynamically self-assemble into groups; individuals within a group tend to share similar opinions (intragroup homophily), and opinions between individuals belonging to different groups tend to be different (intergroup heterophily). We compute the associated nontrivial phase diagram by solving a self-consistency equation for “magnetization” (combined average opinion). Below a critical temperature, there exist two stable phases: one ordered with nonzero magnetization and large clusters, the other disordered with zero magnetization and no clusters. The system exhibits a first-order transition to the disordered phase. We analytically derive the group-size distribution that successfully matches empirical group-size distributions from online communities.

Biological functions in living systems are closely related to their geometries and morphologies. Toroidal structures, which widely exist in nature, present interesting features containing positive, zero, and negative Gaussian curvatures within one system. Such varying curvatures would significantly affect the growing or dehydrating morphogenesis, as observed in various intricate patterns in abundant biological structures. To understand the underlying morphoelastic mechanism and to determine the crucial factors that govern the patterning in toroidal structures, we develop a core-shell model and derive a scaling law to characterize growth- or dehydration-induced instability patterns. We find that the eventual patterns are mainly determined by two dimensionless parameters that are composed of stiffness and curvature of the system. Moreover, we construct a phase diagram showing the multiphase wrinkling pattern selection in various toroidal structures in terms of these two parameters, which is confirmed by our experimental observations. Physical insights into the multiphase transitions and existence of bistable modes are further provided by identifying hysteresis loops and the Maxwell equal-energy conditions. The universal law for morphology selection on core shell structures with varying curvatures can fundamentally explain and precisely predict wrinkling patterns of diverse toroidal structures, which may also provide a platform to design morphology-related functional surfaces.

When light scatters off a sphere, it produces a rich Mie spectrum full of overlapping resonances. Single resonances can be explained with a quantum analogy and result in Fano profiles. However, the full spectrum is so complex that recognizable patterns have not been found, and is only understood by comparing to numerical simulations. Here we show the directional Mie spectrum of evaporating water droplets arranged in consecutive Fano Combs. We then fully explain it by expanding the quantum analogy. This turns the droplet into an “optical atom" with angular momentum, tunneling, and excited states.

Two-dimensional topological insulators (2D TIs) are a highly desired quantum phase but few materials have demonstrated clear signatures of a 2D TI state. It has been predicted that 2D TIs can be created from thin films of three-dimensional TIs by reducing the film thickness until the surface states hybridize. Here, we employ this technique to report the first observation of a 2D TI state in epitaxial thin films of cadmium arsenide, a prototype Dirac semimetal in bulk form. Using magnetotransport measurements with electrostatic gating, we observe a Landau level spectrum and quantum Hall effect that are in excellent agreement with those of an ideal 2D TI. Specifically, we observe a crossing of the zeroth Landau levels at a critical magnetic field. We show that the film thickness can be used to tune the critical magnetic field. Moreover, a larger change in film thickness causes a transition from a 2D TI to a 2D trivial insulator, just as predicted by theory. The high degree of tunability available in epitaxial cadmium arsenide heterostructures can thus be used to fine-tune the 2D TI, which is essential for future topological devices.

Bell nonlocality and Kochen-Specker contextuality are two remarkable nonclassical features of quantum theory, related to strong correlations between outcomes of measurements performed on quantum systems. Both phenomena can be witnessed by the violation of certain inequalities, the simplest and most important of which are the Clauser-Horne-Shimony-Holt (CHSH) and the Klyachko-Can-Binicioğlu-Shumovski (KCBS), for Bell nonlocality and Kochen-Specker contextuality, respectively. It has been shown that, using the most common interpretation of Bell scenarios, quantum systems cannot violate both inequalities concomitantly, thus suggesting a monogamous relation between the two phenomena. In this Letter, we show that the joint consideration of the CHSH and KCBS inequalities naturally calls for the so-called generalized Bell scenarios, which, contrary to the previous results, allows for joint violation of them. In fact, this result is not a special feature of such inequalities: We provide very strong evidence that there is no monogamy between nonlocality and contextuality in any scenario where both phenomena can be observed. We also implement a photonic experiment to test the synchronous violation of both CHSH and KCBS inequalities. Our results agree with the theoretical predictions, thereby providing experimental proof of the coexistence of Bell nonlocality and contextuality in the simplest scenario, and lead to novel possibilities where both concepts could be jointly employed for quantum information processing protocols.

Convection in radial force fields is a fundamental process behind weather on Earth and the Sun, as well as magnetic dynamo action in both. Until now, benchtop experiments have been unable to study convection in radial force fields due to the inability to generate radial forces of sufficient strength. Recently, it has been appreciated that sound, when averaged over many cycles, exerts a force on density gradients in the gas it travels through. The acoustic radiation pressure on thermal gradients draws cooler gas to regions with large time-averaged acoustic velocity and can be modeled as an effective acoustic gravity. We have constructed a system which generates a high amplitude, spherically symmetric acoustic wave in a rotating spherical bulb containing weakly ionized sulfur gas. Without sound, the gas stratifies itself into an initial state with the warmest gas near the center of the bulb, and the coolest gas near the bulb surface. When the sound is initiated, the acoustic radiation pressure is not balanced and a convective instability is triggered. With high speed videography, we observe the initial shape and growth rate of the most unstable mode at various acoustic amplitudes. Acoustic and rotational forces both contribute to the detailed mode shape, which changes qualitatively at low amplitudes where acoustic forces no longer surpass rotational ones everywhere in the bulb.

Flat bands (FBs), presenting a strongly interacting quantum system, have drawn increasing interest recently. However, experimental growth and synthesis of FB materials have been challenging and have remained elusive for the ideal form of monolayer materials where the FB arises from destructive quantum interference as predicted in 2D lattice models. Here, we report surface growth of a self-assembled monolayer of 2D hydrogen-bond (H-bond) organic frameworks (HOFs) of 1,3,5-tris(4-hydroxyphenyl)benzene (THPB) on Au(111) substrate and the observation of FB. High-resolution scanning tunneling microscopy or spectroscopy shows mesoscale, highly ordered, and uniform THPB HOF domains, while angle-resolved photoemission spectroscopy highlights a FB over the whole Brillouin zone. Density-functional-theory calculations and analyses reveal that the observed topological FB arises from a hidden electronic breathing-kagome lattice without atomically breathing bonds. Our findings demonstrate that self-assembly of HOFs provides a viable approach for synthesis of 2D organic topological materials, paving the way to explore many-body quantum states of topological FBs.