Quantum algorithms use the principles of quantum mechanics, such as, for example, quantum superposition, in order to solve particular problems outperforming standard computation. They are developed for cryptography, searching, optimization, simulation, and solving large systems of linear equations. Here, we implement Grover’s quantum algorithm, proposed to find an element in an unsorted list, using a single nuclear $3/2$ spin carried by a Tb ion sitting in a single molecular magnet transistor. The coherent manipulation of this multilevel quantum system (qudit) is achieved by means of electric fields only. Grover’s search algorithm is implemented by constructing a quantum database via a multilevel Hadamard gate. The Grover sequence then allows us to select each state. The presented method is of universal character and can be implemented in any multilevel quantum system with nonequal spaced energy levels, opening the way to novel quantum search algorithms.

Dynamical properties of self-propelled particles obeying a bounded confidence rule are investigated by means of kinetic theory and agent-based simulations. While memory effects are observed in disordered systems, we show that they also occur in active matter systems. In particular, we find that the system exhibits a giant Kovacs-like memory effect that is much larger than predicted by a generic linear theory. Based on a separation of time scales we develop a nonlinear theory to explain this effect. We apply this theory to driven granular gases and propose further applications to spin glasses.

We demonstrate ultrasensitive measurement of fluctuations in a surface-acoustic-wave (SAW) resonator using a hybrid quantum system consisting of the SAW resonator, a microwave (MW) resonator, and a superconducting qubit. The nonlinearity of the driven qubit induces parametric coupling, which up-converts the excitation in the SAW resonator to that in the MW resonator. Thermal fluctuations of the SAW resonator near the quantum limit are observed in the noise spectroscopy in the MW domain.

The topological state transition has been widely studied based on the quantized topological band invariant such as the Chern number for the system without intense randomness that may break the band structures. We numerically demonstrate the disorder-induced state transition in the photonic topological systems for the first time. Instead of applying the ill-defined topological band invariant in a disordered system, we utilize an empirical parameter to unambiguously illustrate the state transition of the topological metamaterials. Before the state transition, we observe a robust surface state with well-confined electromagnetic waves propagating unidirectionally, immune to the disorder from permittivity fluctuation up to 60% of the original value. During the transition, a hybrid state composed of a quasiunidirectional surface mode and intensively localized hot spots is established, a result of the competition between the topological protection and Anderson localization.

Glass films created by vapor-depositing molecules onto a substrate can exhibit properties similar to those of ordinary glasses aged for thousands of years. It is believed that enhanced surface mobility is the mechanism that allows vapor deposition to create such exceptional glasses, but it is unclear how this effect is related to the final state of the film. Here we use molecular dynamics simulations to model vapor deposition and an efficient Monte Carlo algorithm to determine the deposition rate needed to create ultrastable glassy films. We obtain a scaling relation that quantitatively captures the efficiency gain of vapor deposition over bulk annealing, and demonstrates that surface relaxation plays the same role in the formation of vapor-deposited glasses as bulk relaxation does in ordinary glass formation.

Robust quantum computation requires encoding delicate quantum information into degrees of freedom that are hard for the environment to change. Quantum encodings have been demonstrated in many physical systems by observing and correcting storage errors, but applications require not just storing information; we must accurately compute even with faulty operations. The theory of fault-tolerant quantum computing illuminates a way forward by providing a foundation and collection of techniques for limiting the spread of errors. Here we implement one of the smallest quantum codes in a five-qubit superconducting transmon device and demonstrate fault-tolerant state preparation. We characterize the resulting code words through quantum process tomography and study the free evolution of the logical observables. Our results are consistent with fault-tolerant state preparation in a protected qubit subspace.

Searches for invisible Higgs decays at the Large Hadron Collider constrain dark matter Higgs-portal models, where dark matter interacts with the standard model fields via the Higgs boson. While these searches complement dark matter direct-detection experiments, a comparison of the two limits depends on the coupling of the Higgs boson to the nucleons forming the direct-detection nuclear target, typically parametrized in a single quantity $f_N$. We evaluate $f_N$ using recent phenomenological and lattice-QCD calculations, and include for the first time the coupling of the Higgs boson to two nucleons via pion-exchange currents. We observe a partial cancellation for Higgs-portal models that makes the two-nucleon contribution anomalously small. Our results, summarized as $f_N=0.308(18)$, show that the uncertainty of the Higgs-nucleon coupling has been vastly overestimated in the past. The improved limits highlight that state-of-the-art nuclear physics input is key to fully exploiting experimental searches.

We report the first dark matter search results from XENON1T, a $\sim 2000\text{−}\mathrm{kg}$-target-mass dual-phase (liquid-gas) xenon time projection chamber in operation at the Laboratori Nazionali del Gran Sasso in Italy and the first ton-scale detector of this kind. The blinded search used 34.2 live days of data acquired between November 2016 and January 2017. Inside the $(1042\pm 12)\text{−}\mathrm{kg}$ fiducial mass and in the $[5,40]{\mathrm{keV}}_{\mathrm{nr}}$ energy range of interest for weakly interacting massive particle (WIMP) dark matter searches, the electronic recoil background was $(1.93\pm 0.25)\times {10}^{-4}\mathrm{events}/(\mathrm{kg}\times \mathrm{day}\times {\mathrm{keV}}_{\mathrm{ee}})$, the lowest ever achieved in such a dark matter detector. A profile likelihood analysis shows that the data are consistent with the background-only hypothesis. We derive the most stringent exclusion limits on the spin-independent WIMP-nucleon interaction cross section for WIMP masses above $10\mathrm{GeV}/c^2$, with a minimum of $7.7\times {10}^{-47}{\mathrm{cm}}^2$ for $35\text{−}\mathrm{GeV}/c^2$ WIMPs at 90% C.L.

We report a new search for weakly interacting massive particles (WIMPs) using the combined low background data sets acquired in 2016 and 2017 from the PandaX-II experiment in China. The latest data set contains a new exposure of 77.1 live days, with the background reduced to a level of $0.8\times {10}^{-3}\mathrm{evt}/\mathrm{kg}/\mathrm{day}$, improved by a factor of 2.5 in comparison to the previous run in 2016. No excess events are found above the expected background. With a total exposure of $5.4\times {10}^4\mathrm{kg}\mathrm{day}$, the most stringent upper limit on the spin-independent WIMP-nucleon cross section is set for a WIMP with mass larger than $100\mathrm{GeV}/c^2$, with the lowest 90% C.L. exclusion at $8.6\times {10}^{-47}{\mathrm{cm}}^2$ at $40\mathrm{GeV}/c^2$.

The spin-flip tunneling rates are measured in GaAs-based double quantum dots by time-resolved charge detection. Such processes occur in the Pauli spin blockade regime with two electrons occupying the double quantum dot. Ways are presented for tuning the spin-flip tunneling rate, which on the one hand gives access to measuring the Rashba and Dresselhaus spin-orbit coefficients. On the other hand, they make it possible to turn on and off the effect of spin-orbit interaction with a high on/off ratio. The tuning is accomplished by choosing the alignment of the tunneling direction with respect to the crystallographic axes, as well as by choosing the orientation of the external magnetic field with respect to the spin-orbit magnetic field. Spin lifetimes of 10 s are achieved at a tunneling rate close to 1 kHz.

We report transport studies of Mn-doped ${\mathrm{Bi}}_2{\mathrm{Te}}_3$ topological insulator (TI) films with an accurately controlled thickness grown by molecular beam epitaxy. We find that films thicker than five quintuple layers (QLs) exhibit the usual anomalous Hall effect for magnetic TIs. When the thickness is reduced to four QLs, however, characteristic features associated with the topological Hall effect (THE) emerge. More surprisingly, the THE vanishes again when the film thickness is further reduced to three QLs. Theoretical calculations demonstrate that the coupling between the top and bottom surface states at the dimensional crossover regime stabilizes the magnetic Skyrmion structure that is responsible for the THE.

Polarized neutron scattering experiments reveal that type-II multiferroics allow for controlling the spin chirality by external electric fields even in the absence of long-range multiferroic order. In the two prototype compounds ${\mathrm{TbMnO}}_3$ and ${\mathrm{MnWO}}_4$, chiral magnetism associated with soft overdamped electromagnons can be observed above the long-range multiferroic transition temperature $T_{\mathrm{MF}}$, and it is possible to control it through an electric field. While ${\mathrm{MnWO}}_4$ exhibits chiral correlations only in a tiny temperature interval above $T_{\mathrm{MF}}$, in ${\mathrm{TbMnO}}_3$ chiral magnetism can be observed over several kelvin up to the lock-in transition, which is well separated from $T_{\mathrm{MF}}$.

Multistability is an inseparable feature of many physical, chemical, and biological systems which are driven far from equilibrium. In these nonequilibrium systems, stochastic dynamics often induces switching between distinct states on emergent time scales; for example, bistable switching is a natural feature of noisy, spatially extended systems that consist of bistable elements. Nevertheless, here we present experimental evidence that bistable elements are not required for the global bistability of a system. We observe temporal switching between a crystalline, condensed state and a gaslike, excited state in a spatially extended, quasi-two-dimensional system of charged microparticles. Accompanying numerical simulations show that conservative forces, damping, and stochastic noise are sufficient to prevent steady-state equilibrium, leading to switching between the two states over a range of time scales, from seconds to hours.

Microwave transitions between the ortho and para states of the ${\mathrm{S}}_2{\mathrm{Cl}}_2$ molecule in a free isolated condition are observed for the first time. In the theoretical treatment, we derive eigenfunctions of an effective Hamiltonian including the ortho-para interaction to calculate the intensities and frequencies of forbidden ortho-para transitions in the cm-wave region and pick up some promising candidates for the spectroscopic detection. In the experiment, transitions of the ${\mathrm{S}}_2{\mathrm{Cl}}_2$ molecule under a supersonic jet condition are observed with a Fourier transform microwave spectrometer. Seven hyperfine resolved rotational transitions including the lowest rotational level are detected as the ortho-para transitions at the predicted frequencies within the experimental errors. The observed intensities are about ${10}^{-3}$ times the allowed transitions, which are consistent with the predictions based on the intensity-borrowing model. This result suggests that the ortho-para conversion of this molecule occurs in a few thousand years through spontaneous emission even in a circumstance where molecular collisions occur rarely like in interstellar space.

We demonstrate experimentally an efficient electron axicon lens using a magnetic vortex. We show that naturally occurring magnetic vortices with circular magnetic moment distributions in a soft-magnetic thin film create conical phase shifts for fast electrons. Such radially symmetric linear phase ramps are equivalent to ideal light optical axicons. We apply this lens to generate efficient nondiffracting electron Bessel beams, which we observe experimentally in through-focus Lorentz images as well as in propagated off-axis electron holograms. This highlights the potential for using magnetic nanostructures as highly efficient and flexible phase plates for crafting desired electron beam shapes.

We present a free-space interferometer to observe two-particle interference of a pair of atoms with entangled momenta. The source of atom pairs is a Bose-Einstein condensate subject to a dynamical instability, and the interferometer is realized using Bragg diffraction on optical lattices, in the spirit of our recent Hong-Ou-Mandel experiment. We report on an observation ruling out the possibility of a purely mixed state at the input of the interferometer. We explain how our current setup can be extended to enable a test of a Bell inequality on momentum observables.

It is commonly assumed that surface plasmon-polariton (SPP) excitations on a metal-dielectric interface decay exponentially inside the metallic sample. Here, we show that in a wide spectral interval the SPP field decays much slower, being inversely proportional to the distance to the interface modified by an additional logarithmic factor. This dependence differs from the standard anomalous skin effect and is provisionally referred to as superanomalous. Its origin is the nonlocality and the logarithmic singularity of the dielectric permittivity in metals. This type of decay is pronounced for SPP modes of higher frequencies, but it is suppressed for light waves.

The cosmic unidentified infrared emission (UIE) band phenomenon is generally considered as indicative of free-flying polycyclic aromatic hydrocarbon molecules in space. However, a coherent explanation of emission spectral band patterns depending on astrophysical source is yet to be resolved under this attribution. Meanwhile astronomers have restored the alternative origin as due to amorphous carbon particles, but assigning spectral patterns to specific structural elements of particles is equally challenging. Here we report a physical principle in which inclusion of nonplanar structural defects in aromatic core molecular structures ($\pi$ domains) induces spectral patterns typical of the phenomenon. We show that defects in model $\pi$ domains modulate the electronic-vibration coupling that activates the delocalized $\pi$-electron contribution to aromatic vibrational modes. The modulation naturally disperses $\mathrm{C}=\mathrm{C}$ stretch modes in band patterns that readily resemble the UIE bands in the elusive $6–9\mu \mathrm{m}$ range. The electron-vibration interaction mechanics governing the defect-induced band patterns underscores the importance of $\pi$ delocalization in the emergence of UIE bands. We discuss the global UIE band regularity of this range as compatible with an emission from the delocalized $s{p}^2$ phase, as $\pi$ domains, confined in disordered carbon mixed-phase aggregates.

The separation of isotopes in space and time by gas-surface atomic diffraction is presented as a new means for isotopic enrichment. A supersonic beam of natural abundance neon is scattered from a periodic surface of methyl-terminated silicon, with the ${}^{20}\mathrm{Ne}$ and ${}^{22}\mathrm{Ne}$ isotopes scattering into unique diffraction channels. Under the experimental conditions presented in this Letter, a single pass yields an enrichment factor $3.50\pm 0.30$ for the less abundant isotope, ${}^{22}\mathrm{Ne}$, with extension to multiple passes easily envisioned. The velocity distribution of the incident beam is demonstrated to be the determining factor in the degree of separation between the isotopes’ diffraction peaks. In cases where there is incomplete angular separation, the difference in arrival times of the two isotopes at a given scattered angle can be exploited to achieve complete temporal separation of the isotopes. This study explores the novel application of supersonic molecular beam studies as a viable candidate for separation of isotopes without the need for ionization or laser excitation.

Electron correlation in graphene is unique because of the interplay between the Dirac cone dispersion of $\pi$ electrons and long-range Coulomb interaction. Because of the zero density of states at Fermi level, the random phase approximation predicts no metallic screening at long distance and low energy, so one might expect that graphene should be a poorly screened system. However, empirically graphene is a weakly interacting semimetal, which leads to the question of how electron correlations take place in graphene at different length scales. We address this question by computing the equal time and dynamic structure factor $S(\mathit{q})$ and $S(\mathit{q},\omega )$ of freestanding graphene using ab initio fixed-node diffusion Monte Carlo simulations and the random phase approximation. We find that the $\sigma$ electrons contribute strongly to $S(\mathit{q},\omega )$ for relevant experimental values of $\omega$ even at distances up to around 80 Å. These findings illustrate how the emergent physics from underlying Coulomb interactions results in the observed weakly correlated semimetal.