Diffusion-controlled annihilation : Coalescence, fragmentation, and collapse of nonidentical -particle islands submerged in the -particle sea
Boris M. Shipilevsky
Phys. Rev. E 106, 054206 (2022) - Published 9 November, 2022
We present a systematic analysis of diffusion-controlled interaction and collapse of two nonidentical spatially separated -dimensional -particle islands in the -particle sea at propagation of the sharp reaction front at equal species diffusivities. We show that at a sufficiently large initial distance between the centers of islands and a relatively large initial ratio of island-to-sea concentrations, the evolution dynamics of the island-sea-island system demonstrates remarkable universality and, depending on the system dimension, is determined unambiguously by two dimensionless parameters and , where and are the initial particle numbers in the larger and smaller of the islands, respectively, and is the initial number of sea particles in the volume . We find that at each fixed , there are threshold values and that depend on the dimension and separate the domains of individual death of each of the islands , coalescence and subsequent fragmentation (division) of a two-centered island , and collapse of a single-centered island formed by coalescence . We demonstrate that regardless of , the trajectories of the island centers are determined unambiguously by the parameter , and we reveal a detailed picture of the evolution of islands and front trajectories with an increase in , focusing on the scaling laws of evolution at the final collapse stage and in the vicinity of starting coalescence and fragmentation points.