The recent demonstration of topological states in antiferromagnets (AFMs) provides an exciting platform for exploring prominent physical phenomena and applications of antiferromagnetic spintronics. A famous example is the AFM topological insulator (TI) state, which, however, was still not observed in two dimensions. Using a tight-binding model and first-principles calculations, we show that, in contrast to previously observed AFM topological insulators in three dimensions, an AFM TI can emerge in two dimensions as a result of a nonsymmorphic symmetry that combines the twofold rotation symmetry and half-lattice translation. Based on the spin Chern number, Wannier charge centers, and gapless edge states analysis, we identify intrinsic AFM $X\mathrm{Mn}Y$ ($X=\mathrm{Sr}$ and Ba, $Y=\mathrm{Sn}$ and Pb) quintuple layers as experimentally feasible examples of predicted topological states with a stable crystal structure and giant magnitude of the nontrivial band gaps, reaching as much as 186 meV for SrMnPb, thereby promoting these systems as promising candidates for innovative spintronics applications.

The effect of compression on the magnetic ground state of ${\mathrm{Sr}}_2{\mathrm{IrO}}_4$ is studied with x-ray resonant techniques in the diamond anvil cell. The weak interlayer exchange coupling between square-planar 2D ${\mathrm{IrO}}_2$ layers is readily modified upon compression, with a crossover between magnetic structures around 7 GPa mimicking the effect of an applied magnetic field at ambient pressure. Higher pressures drive an order-disorder magnetic phase transition with no magnetic order detected above 17–20 GPa. The persistence of strong exchange interactions between $J_{\mathrm{eff}}=1/2$ magnetic moments within the insulating ${\mathrm{IrO}}_2$ layers up to at least 35 GPa points to a highly frustrated magnetic state in compressed ${\mathrm{Sr}}_2{\mathrm{IrO}}_4$, opening the door for realization of novel quantum paramagnetic phases driven by extended $5d$ orbitals with entangled spin and orbital degrees of freedom.

The rotational diffusive motion of a self-propelled, attractive spherical colloid immersed in a solution of self-avoiding polymers is studied by mesoscale hydrodynamic simulations. A drastic enhancement of the rotational diffusion by more than an order of magnitude in the presence of activity is obtained. The amplification is a consequence of two effects, a decrease of the amount of adsorbed polymers by active motion and an asymmetric encounter with polymers on the squirmer surface, which yields an additional torque and random noise for the rotational motion. Our simulations suggest a way to control the rotational dynamics of squirmer-type microswimmers by the degree of polymer adsorption and system heterogeneity.

We study the quantum fluctuations in a one-dimensional Bose-Einstein condensate realizing an analogous acoustic black hole. The taking into account of evanescent channels and of zero modes makes it possible to accurately reproduce recent experimental measurements of the density correlation function. We discuss the determination of Hawking temperature and show that in our model the analogous radiation presents some significant departure from thermality.

We study fluctuations of interfaces in the Kardar-Parisi-Zhang (KPZ) universality class with curved initial conditions. By simulations of a cluster growth model and experiments with liquid-crystal turbulence, we determine the universal scaling functions that describe the height distribution and the spatial correlation of the interfaces growing outward from a ring. The scaling functions, controlled by a single dimensionless time parameter, show crossover from the statistical properties of the flat interfaces to those of the circular interfaces. Moreover, employing the KPZ variational formula to describe the case of the ring initial condition, we find that the formula, which we numerically evaluate, reproduces the numerical and experimental results precisely without adjustable parameters. This demonstrates that precise numerical evaluation of the variational formula is possible at all, and underlines the practical importance of the formula, which is able to predict the one-point distribution of KPZ interfaces for general initial conditions.

Polar molecules in superpositions of rotational states exhibit long-range dipolar interactions, but maintaining their coherence in a trapped sample is a challenge. We present calculations that show many laser-coolable molecules have convenient rotational transitions that are exceptionally insensitive to magnetic fields. We verify this experimentally for CaF where we find a transition with sensitivity below $5\mathrm{Hz}{\mathrm{G}}^{-1}$ and use it to demonstrate a rotational coherence time of 6.4(8) ms in a magnetic trap. Simulations suggest it is feasible to extend this to more than 1 s using a smaller cloud in a biased magnetic trap.

Graphite is known to transform into diamond under dynamic compression or under combined high pressure and high temperature, either by a concerted mechanism or by a nucleation mechanism. However, these mechanisms fail to explain the recently reported discovery of diamond formation during ambient temperature compression combined with shear stress. Here we report a new transition pathway for graphite to diamond under compression combined with shear, based on results from both theoretical simulations and advanced experiments. In contrast to the known model for thermally activated diamond formation under pressure, the shear-induced diamond formation takes place during the decompression process via structural transitions. At a high pressure with large shear, graphite transforms into ultrastrong $s{p}^3$ phases whose structures depend on the degree of shear stress. These metastable $s{p}^3$ phases transform into either diamond or graphite upon decompression. Our results explain several recent experimental observations of low-temperature diamond formation. They also emphasize the importance of shear stress for diamond formation, providing new insight into the graphite-diamond transformation mechanism.

Motivated by the prediction of fractonic topological defects in a quantum crystal, we utilize a reformulated elasticity duality to derive a description of a fracton phase in terms of coupled vector U(1) gauge theories. The fracton order and restricted mobility emerge as a result of an unusual Gauss law where electric field lines of one gauge field act as sources of charge for others. At low energies this vector gauge theory reduces to the previously studied fractonic symmetric tensor gauge theory. We construct the corresponding lattice model and a number of generalizations, which realize fracton phases via a condensation of stringlike excitations built out of charged particles, analogous to the $p$-string condensation mechanism of the gapped $X$-cube fracton phase.

Suppose that Alice and Bob are located in distant laboratories, which are connected by an ideal quantum channel. Suppose further that they share many copies of a quantum state ${\rho }_{ABE}$, such that Alice possesses the $A$ systems and Bob the $BE$ systems. In our model, there is an identifiable part of Bob’s laboratory that is insecure: a third party named Eve has infiltrated Bob’s laboratory and gained control of the $E$ systems. Alice, knowing this, would like use their shared state and the ideal quantum channel to communicate a message in such a way that Bob, who has access to the whole of his laboratory ($BE$ systems), can decode it, while Eve, who has access only to a sector of Bob’s laboratory ($E$ systems) and the ideal quantum channel connecting Alice to Bob, cannot learn anything about Alice’s transmitted message. We call this task the conditional one-time pad, and in this Letter, we prove that the optimal rate of secret communication for this task is equal to the conditional quantum mutual information $I(A;B|E)$ of their shared state. We thus give the conditional quantum mutual information an operational meaning that is different from those given in prior works, via state redistribution, conditional erasure, or state deconstruction. We also generalize the model and method in several ways, one of which is a secret-sharing task, i.e., the case in which Alice’s message should be secure from someone possessing only the $AB$ or $AE$ systems, but should be decodable by someone possessing all systems $A$, $B$, and $E$.

The local stability of a weakly dissipative heat engine is analyzed and linked to an energetic multi-objective optimization perspective. This constitutes a novel issue in the unified study of cyclic energy converters, opening the perspective to the possibility that stability favors self-optimization of thermodynamic quantities including efficiency, power and entropy generation. To this end, a dynamics simulating the restitution forces, which mimics a harmonic potential, bringing the system back to the steady state is analyzed. It is shown that relaxation trajectories are not arbitrary but driven by the improvement of several energetic functions. Insights provided by the statistical behavior of consecutive random perturbations show that the irreversible behavior works as an attractor for the energetics of the system, while the endoreversible limit acts as an upper bound and the Pareto front as a global attractor. Fluctuations around the operation regime reveal a difference between the behavior coming from fast and slow relaxation trajectories: while the former are associated to an energetic self-optimization evolution, the latter are ascribed to better performances. The self-optimization induced by stability and the possible use of instabilities in the operation regime to improve the energetic performance might usher into new useful perspectives in the control of variables for real engines.

Four-dimensional gauge theories with matter can have regions in parameter space, often dubbed conformal windows, where they flow in the infrared to nontrivial conformal field theories. It has been conjectured that conformality can be lost because of merging of two nearby fixed points that move into the complex plane, and that a walking dynamics governed by scaling dimensions of operators defined at such complex fixed points can occur. We find controlled, parametrically weakly coupled, and ultraviolet-complete 4D gauge theories that explicitly realize this scenario. We show how the walking dynamics is controlled by the coupling of a double-trace operator that crosses marginality. The walking regime ends when the renormalization group flow of this coupling leads to a (weak) first-order phase transition with Coleman-Weinberg symmetry breaking. A light dilatonlike scalar particle appears in the spectrum, but it is not parametrically lighter than the other excitations.

We report the trapping of ultracold neutral Rb atoms and ${\mathrm{Ba}}^{+}$ ions in a common optical potential in absence of any radio frequency (rf) fields. We prepare ${\mathrm{Ba}}^{+}$ at $370\mu \mathrm{K}$ and demonstrate efficient sympathetic cooling by $100\mu \mathrm{K}$ after one collision. Our approach is currently limited by the Rb density and related three-body losses, but it overcomes the fundamental limitation in rf traps set by rf-driven, micromotion-induced heating. It is applicable to a wide range of ion-atom species, and may enable novel ultracold chemistry experiments and complex many-body dynamics.

Solid-state impurity spins with optical control are currently investigated for quantum networks and repeaters. Among these, rare-earth-ion doped crystals are promising as quantum memories for light, with potentially long storage time, high multimode capacity, and high bandwidth. However, with spins there is often a tradeoff between bandwidth, which favors electronic spin, and memory time, which favors nuclear spins. Here, we present optical storage experiments using highly hybridized electron-nuclear hyperfine states in ${{}^{171}\mathrm{Yb}}^{3+}:{\mathrm{Y}}_2{\mathrm{SiO}}_5$, where the hybridization can potentially offer both long storage time and high bandwidth. We reach a storage time of 1.2 ms and an optical storage bandwidth of 10 MHz that is currently only limited by the Rabi frequency of the optical control pulses. The memory efficiency in this proof-of-principle demonstration was about 3%. The experiment constitutes the first optical storage using spin states in any rare-earth ion with electronic spin. These results pave the way for rare-earth based quantum memories with high bandwidth, long storage time, and high multimode capacity, a key resource for quantum repeaters.

Topological nodal-line semimetals with exotic quantum properties are characterized by symmetry-protected line-contact bulk band crossings in the momentum space. However, in most of identified topological nodal-line compounds, these topological nontrivial nodal lines are enclosed by complicated topological trivial states at the Fermi energy ($E_F$), which would perplex their identification and hinder further applications. Utilizing angle-resolved photoemission spectroscopy and first-principles calculations, we provide compelling evidence for the existence of Dirac nodal-line fermions in the monoclinic semimetal ${\mathrm{SrAs}}_3$, which possesses a simple nodal loop in the vicinity of $E_F$ without the distraction from complicated trivial Fermi surfaces. Our calculations revealed that two bands with opposite parities were inverted around $Y$ near $E_F$, resulting in the single nodal loop at the $\mathrm{\Gamma }\text{−}Y\text{−}S$ plane with a negligible spin-orbit coupling effect. The band crossings were tracked experimentally and the complete nodal loop was identified quantitatively, which provide a critical experimental support for the existence of nodal-line fermions in the ${\mathrm{CaP}}_3$ family of materials. Hosting simple topological nontrivial bulk electronic states around $E_F$ and without complication from the trivial states, ${\mathrm{SrAs}}_3$ is expected to be a potential platform for topological quantum state investigation and applications.

We consider conditions for the existence of boundary modes in non-Hermitian systems with edges of arbitrary codimension. Through a universal formulation of formation criteria for boundary modes in terms of local Green’s functions, we outline a generic perspective on the appearance of such modes and generate corresponding dispersion relations. In the process, we explain the skin effect in both topological and nontopological systems, exhaustively generalizing bulk-boundary correspondence to different types of non-Hermitian gap conditions, a prominent distinguishing feature of such systems. Indeed, we expose a direct relation between the presence of a point gap invariant and the appearance of skin modes when this gap is trivialized by an edge. This correspondence is established via a doubled Green’s function, inspired by doubled Hamiltonian methods used to classify Floquet and, more recently, non-Hermitian topological phases. Our work constitutes a general tool, as well as a unifying perspective for this rapidly evolving field. Indeed, as a concrete application we find that our method can expose novel non-Hermitian topological regimes beyond the reach of previous methods.

Using microtransient absorption spectroscopy, we show that the dynamical form of exciton-exciton annihilation in atomically thin black phosphorous can be made to switch between time varying 1D scattering and time-independent 2D scattering. At low carrier densities, anisotropy drives the 1D behavior, but as the photoexcitation density approaches the exciton saturation limit, the 2D nature of exciton-exciton scattering takes over. Furthermore, lowering the temperature provides a handle on the ultrafast timescale at which the 1D to 2D transition occurs. We understand our results quantitatively using a diffusion based model of exciton-exciton scattering.

We investigate the quasiparticle dynamics in the prototypical heavy fermion ${\mathrm{CeCoIn}}_5$ using ultrafast optical pump-probe spectroscopy. Our results indicate that this material system undergoes hybridization fluctuations before the establishment of heavy electron coherence, as the temperature decreases from $\sim 120\mathrm{K}$ ($T^{†}$) to $\sim 55\mathrm{K}$ ($T^{*}$). We reveal that the anomalous coherent phonon softening and damping reduction below $T^{*}$ are directly associated with the emergence of collective hybridization. We also discover a distinct collective mode with an energy of $\sim 8\mathrm{meV}$, which may be experimental evidence of the predicted unconventional density wave. Our findings provide important information for understanding the hybridization dynamics in heavy fermion systems.

We report that trivalent cobalt hexammine cations decrease the persistence length, stretching modulus, helical density, and size of plectonemes formed under torque of DNA but increase those of RNA. Divalent magnesium cations, however, decrease the persistence lengths, contour lengths, and sizes of plectonemes while increasing the helical densities of both DNA and RNA. The experimental results are explained by different binding modes of the cations on DNA and RNA in our all-atom molecular dynamics simulations. The significant variations of the helical densities and structures of DNA and RNA duplexes induced by high-valent cations may affect interactions of the duplexes with proteins.