This Letter exposes a tight connection between the thermodynamic efficiency of information processing and predictive inference. A generalized lower bound on dissipation is derived for partially observable information engines which are allowed to use temperature differences. It is shown that the retention of irrelevant information limits efficiency. A data representation method is derived from optimizing a fundamental physical limit to information processing: minimizing the lower bound on dissipation leads to a compression method that maximally retains relevant, predictive, information. In that sense, predictive inference emerges as the strategy that least precludes energy efficiency.

Constraints play an important role in the entanglement dynamics of many quantum systems. We develop a diagrammatic formalism to exactly evaluate the entanglement spectrum of random pure states in large constrained Hilbert spaces. The resulting spectra may be classified into universal “phases” depending on their singularities. The simplest class of local constraints reveals a nontrivial phase diagram with a Marchenko-Pastur phase which terminates in a critical point with new singularities. We propose a certain quantum defect chain as a microscopic realization of the critical point. The much studied Rydberg-blockaded or Fibonacci chain lies in the Marchenko-Pastur phase with a modified Page correction to the entanglement entropy. Our results predict the entanglement of infinite temperature eigenstates in thermalizing constrained Floquet spin chains, as we confirm numerically.

Radio observations at low frequencies with the low frequency array (LOFAR) start discovering gigantic radio bridges connecting pairs of massive galaxy clusters. These observations probe unexplored mechanisms of in situ particle acceleration that operate on volumes of several ${\mathrm{Mpc}}^3$. Numerical simulations suggest that such bridges are dynamically complex and that weak shocks and super-Alfvénic turbulence can be driven across the entire volume of these regions. In this Letter, we explore, for the first time, the role of second-order Fermi mechanisms for the reacceleration of relativistic electrons interacting with turbulence in these peculiar regions. We assume the turbulent energy flux measured in simulations and adopt a scenario in which relativistic particles scatter with magnetic field lines diffusing in super-Alfvénic turbulence and magnetic fields are amplified by the same turbulence. We show that steep spectrum and volume filling synchrotron emission can be generated in the entire intracluster bridge region, thus providing a natural explanation for radio bridges. Consequently, radio observations have the potential to probe the dissipation of energy on scales larger than galaxy clusters and second-order Fermi mechanisms operating in physical regimes that are still poorly explored. This has a potential impact on several branches of astrophysics and cosmology.

We propose a new collider probe for axionlike particles (ALPs), and more generally for pseudo-Goldstone bosons: nonresonant searches that take advantage of the derivative nature of their interactions with Standard Model particles. ALPs can participate as off shell mediators in the $s$ channel of $2\to 2$ scattering processes at colliders like the LHC. We exemplify the power of this novel type of search by deriving new limits on ALP couplings to gauge bosons via the processes $pp\to ZZ$, $pp\to \gamma \gamma$, and $pp\to jj$ using run 2 CMS public data, probing previously unexplored areas of the ALP parameter space. In addition, we propose future nonresonant searches involving the ALP coupling to other electroweak bosons and/or the Higgs particle.

Spin-orbit-coupled Bose-Einstein condensates (SOBECs) exhibit two new phases of matter, now known as the stripe and plane-wave phases. When two interacting spin components of a SOBEC spatially overlap, density modulations with periodicity given by the spin-orbit coupling strength appear. In equilibrium, these components fully overlap in the miscible stripe phase and overlap only in a domain wall in the immiscible plane-wave phase. Here we probe the density modulation present in any overlapping region with optical Bragg scattering and observe the sudden drop of Bragg scattering as the overlapping region shrinks. Using an atomic analog of the Talbot effect, we demonstrate the existence of long-range coherence between the different spin components in the stripe phase and surprisingly even in the phase-separated plane-wave phase.

Magnets with chiral crystal structures and helical spin structures have recently attracted much attention as potential spin-electronics materials, but their relatively low magnetic-ordering temperatures are a disadvantage. While cobalt has long been recognized as an element that promotes high-temperature magnetic ordering, most Co-rich alloys are achiral and exhibit collinear rather than helimagnetic order. Crystallographically, the B20-ordered compound CoSi is an exception due to its chiral structure, but it does not exhibit any kind of magnetic order. Here, we use nonequilibrium processing to produce B20-ordered ${\mathrm{Co}}_{1+x}{\mathrm{Si}}_{1-x}$ with a maximum Co solubility of $x=0.043$. Above a critical excess-Co content ($x_c=0.028$), the alloys are magnetically ordered, and for $x=0.043$, a critical temperature $T_c=328\mathrm{K}$ is obtained, the highest among all B20-type magnets. The crystal structure of the alloy supports spin spirals caused by Dzyaloshinskii-Moriya interactions, and from magnetic measurements we estimate that the spirals have a periodicity of about 17 nm. Our density-functional calculations explain the combination of high magnetic-ordering temperature and short periodicity in terms of a quantum phase transition where excess-cobalt spins are coupled through the host matrix.

Terahertz lights are usually generated through the optical rectification process within a femtosecond laser pulse in noncentrosymmetric materials. Here, we report a new generation mechanism of terahertz lights based upon a photoinduced phase transition, in which an electronic structure is rapidly changed by a photoirradiation. When a ferroelectric organic molecular compound, tetrathiafulvalene-$p$-chloranil, is excited by a femtosecond laser pulse, the ionic-to-neutral transition is driven and simultaneously a strong terahertz radiation is produced. By analyzing the terahertz electric-field waveforms and their dependence on the polarization direction of the incident laser pulse, we demonstrate that the terahertz radiation originates from the ultrafast decrease of the spontaneous polarization in the photoinduced ionic-to-neutral transition. The efficiency of the observed terahertz radiation via the photoinduced phase transition mechanism is found to be much higher than that via the optical rectification in the same material and in a typical terahertz emitter, ZnTe.

We report the experimental implementation of discrete-time topological quantum walks of a Bose-Einstein condensate in momentum space. Introducing stroboscopic driving sequences to the generation of a momentum lattice, we show that the dynamics of atoms along the lattice is effectively governed by a periodically driven Su-Schrieffer-Heeger model, which is equivalent to a discrete-time topological quantum walk. We directly measure the underlying topological invariants through time-averaged mean chiral displacements, which are consistent with our experimental observation of topological phase transitions. We then observe interaction-induced localization in the quantum-walk dynamics, where atoms tend to populate a single momentum-lattice site under interactions that are nonlocal in momentum space. Our experiment opens up the avenue of investigating discrete-time topological quantum walks using cold atoms, where the many-body environment and tunable interactions offer exciting new possibilities.

We improve the test of the gravitational inverse-square law at the submillimeter range by suppressing the vibration of the electrostatic shielding membrane to reduce the disturbance coupled from the residual surface potential. The result shows that, at a 95% confidence level, the gravitational inverse-square law holds ($|\alpha |\le 1$) down to a length scale $\lambda =48\mu \mathrm{m}$. This work establishes the strongest bound on the magnitude $\alpha$ of the Yukawa violation in the range of $40–350\mu \mathrm{m}$, and improves the previous bounds by up to a factor of 3 at the length scale $\lambda \approx 70\mu \mathrm{m}$. Furthermore, the constraints on the power-law potentials are improved by about a factor of 2 for $k=4$ and 5.

The excitation functions for quasielastic scattering of ${}^{22}\mathrm{Ne}+{}^{248}\mathrm{Cm}$, ${}^{26}\mathrm{Mg}+{}^{248}\mathrm{Cm}$, and ${}^{48}\mathrm{Ca}+{}^{238}\mathrm{U}$ are measured using a gas-filled recoil ion separator. The quasielastic barrier distributions are extracted for these systems and are compared with coupled-channel calculations. The results indicate that the barrier distribution is affected dominantly by deformation of the actinide target nuclei, but also by vibrational or rotational excitations of the projectile nuclei, as well as neutron transfer processes before capture. From a comparison between the experimental barrier distributions and the evaporation residue cross sections for Sg ($Z=106$), Hs (108), Cn (112), and Lv (116), it is suggested that the hot fusion reactions take advantage of a compact collision, where the projectile approaches along the short axis of a prolately deformed nucleus. A new method is proposed to estimate the optimum incident energy to synthesize unknown superheavy nuclei using the barrier distribution.

Accurate calculation of spectral line broadening is important for many hot, dense plasma applications. However, calculated line widths have significantly underestimated measured widths for $\mathrm{\Delta }n=0$ lines of Li-like ions, which is known as the isolated-line problem. In this Letter, scrutinization of the line-width derivation reveals that the commonly used expression neglects a potentially important contribution from electron-capture. Line-width calculations including this process are performed with two independent codes, both of which removed the discrepancies at temperatures below 10 eV. The revised calculations also suggest the remaining discrepancy scales more strongly with electron temperature than the atomic number as was previously suggested.

Several types of experiments showed the existence of negative methane ions ${\mathrm{CH}}_4^{-}$ over a period of 50 years but the nature of this elusive species remains unknown. A benchmark study has shown that the experimentally observed species cannot be described by the attachment of an electron in the doublet ground state of ${\mathrm{CH}}_4^{-}$. Here we find ${\mathrm{CH}}_4^{-}$ as being a metastable species in its lowest quartet spin state, a ${\mathrm{CH}}_2^{-}:{\mathrm{H}}_2$ exciplex with three open shells lying ca. 10 eV above the methane singlet ground state but slightly below the dissociation fragments. The formation of charged high-spin exciplexes is a novel mechanism to explain small molecular anions with implications in a plethora of basic and applied research fields.

Oxygen reactivity plays a key role in the performance of ceria-based catalysts. Aberration-corrected transmission electron microscopy and molecular dynamics simulations were used to study the oxygen atom diffusion in ceria under activated conditions. Reactive oxygen atom and its real-time diffusion were visualized. The interplay between cerium and oxygen atoms originating from a Coulomb interaction was revealed by the out-of-plane buckling of cerium atoms associated with oxygen transport. Anisotropic oxygen atom diffusion that depends on crystal orientations was discovered, demonstrating a preferential [001] crystallographic diffusion pathway. These findings reveal prospects for applications of anisotropic orientation-relevant fluorite-structured oxides.

Inverse problems are encountered in many domains of physics, with analytic continuation of the imaginary Green’s function into the real frequency domain being a particularly important example. However, the analytic continuation problem is ill defined and currently no analytic transformation for solving it is known. We present a general framework for building an artificial neural network (ANN) that solves this task with a supervised learning approach. Application of the ANN approach to quantum Monte Carlo calculations and simulated Green’s function data demonstrates its high accuracy. By comparing with the commonly used maximum entropy approach, we show that our method can reach the same level of accuracy for low-noise input data, while performing significantly better when the noise strength increases. The computational cost of the proposed neural network approach is reduced by almost three orders of magnitude compared to the maximum entropy method.

Creating a transmon qubit using semiconductor-superconductor hybrid materials not only provides electrostatic control of the qubit frequency, it also allows parts of the circuit to be electrically connected and disconnected in situ by operating a semiconductor region of the device as a field-effect transistor. Here, we exploit this feature to compare in the same device characteristics of the qubit, such as frequency and relaxation time, with related transport properties such as critical supercurrent and normal-state resistance. Gradually opening the field-effect transistor to the monitoring circuit allows the influence of weak-to-strong dc monitoring of a “live” qubit to be measured. A model of this influence yields excellent agreement with experiment, demonstrating a relaxation rate mediated by a gate-controlled environmental coupling.

Disorder is more the rule than the exception in natural and synthetic materials. Nonetheless, wave propagation within inhomogeneously disordered materials has received scant attention. We combine microwave experiments and theory to find the spatial variation of generic wave propagation quantities in inhomogeneously disordered materials. We demonstrate that wave statistics within samples of any dimension are independent of the detailed structure of a material and depend only on the net strengths of distributed scattering and reflection between the observation point and each of the boundaries.

Monte Carlo simulations, fully constrained by experimental parameters, are found to agree well with a measured phase diagram of aqueous dispersions of nanoparticles with a moderate size polydispersity over a broad range of salt concentrations, $c_s$, and volume fractions, $\varphi$. Upon increasing $\varphi$, the colloids freeze first into coexisting compact solids then into a body centered cubic phase (bcc) before they melt into a glass forming liquid. The surprising stability of the bcc solid at high $\varphi$ and $c_s$ is explained by the interaction (charge) polydispersity and vibrational entropy.