The physics of bound states in the continuum (BICs) allows the design and demonstration of optical resonant structures with large values of the quality factor ($Q$ factor) by employing dielectric structures with low losses. However, BIC is a general wave phenomenon that should be observed in many systems, including the metal-dielectric structures supporting surface plasmon polaritons where optical resonances are hindered by losses. Here we suggest and develop a comprehensive strategy to achieve high-$Q$ resonances in plasmonic metasurfaces by effectively tailoring the resonant modes from local to nonlocal regimes, thus transitioning from quasi-isolated localized resonances to extended resonant modes involving strong interaction among neighboring structure metaunits.

The natural bulk Van der Waals heterostructure compound $6R\text{−}{\mathrm{TaS}}_2$ consists of alternate stacking $1T$- and $1H\text{−}{\mathrm{TaS}}_2$ monolayers, creating a unique system that incorporates charge-density-wave (CDW) order and superconductivity (SC) in distinct monolayers. Here, after confirming that the 2D nature of the lattice is preserved up to 8 GPa in $6R\text{−}{\mathrm{TaS}}_2$, we documented an unusual evolution of CDW and SC by conducting high-pressure electronic transport measurements. Upon compression, we observe a gradual suppression of CDW within the $1T$ layers, while the SC exhibits a dome-shaped behavior that terminates at a critical pressure $P_{\mathrm{c}}$ around 2.9 GPa. By taking account of the fact that the substantial suppression of SC is concomitant with the complete collapse of CDW order at $P_{\mathrm{c}}$, we argue that the $6R\text{−}{\mathrm{TaS}}_2$ behaves like a stack of Josephson junctions and thus the suppressed superconductivity can be attributed to the weakening of Josephson coupling associated with the presence of CDW fluctuations in the $1T$ layers. Furthermore, the SC reversely enhances above $P_{\mathrm{c}}$, implying the development of emergent superconductivity in the $1T$ layers after the melting of $T$-layer CDW orders. These results show that the $6R\text{−}{\mathrm{TaS}}_2$ not only provides a promising platform to explore emergent phenomena but also serves as a model system to study the complex interactions between competing electronic states.

We study the effect of dynamical screening of interactions on the transition temperatures ($T_c$) of exciton condensation in a symmetric bilayer of quadratically dispersing electrons and holes by solving the linearized Eliashberg equations for the anomalous interlayer Green’s functions. We find that $T_c$ is finite for the range of density and layer separations studied, decaying exponentially with interlayer separation. $T_c$ is suppressed well below that predicted by a Hartree Fock mean field theory with unscreened Coulomb interaction, but is above the estimates from the statically screened Coulomb interaction. Furthermore, using a diagrammatic framework, we show that the system is always an exciton condensate at zero temperature but $T_c$ is exponentially small for large interlayer separation.

Characterizing entanglement is central for quantum information science. Special observables which indicate entanglement, so-called entanglement witnesses, are a widely used tool for this task. The construction of these witnesses typically relies on the observation that quantum states with a high fidelity to some entangled target state are entangled, too. We introduce a general method to construct entanglement witnesses based on the Schmidt decomposition of observables. The method works for two-particle and multiparticle systems and is strictly stronger than fidelity-based constructions. The resulting witnesses can also be used to quantify entanglement and to characterize its dimensionality. Finally, we present experimentally relevant examples, where our approach improves entanglement detection significantly.

We experimentally probe the interplay of the quantum switch with the laws of thermodynamics. The quantum switch places two channels in a superposition of orders and may be applied to thermalizing channels. Quantum-switching thermal channels has been shown to give apparent violations of the second law. Central to these apparent violations is how quantum switching channels can increase the capacity to communicate information. We experimentally show this increase and how it is consistent with the laws of thermodynamics, demonstrating how thermodynamic resources are consumed. We use a nuclear magnetic resonance approach with coherently controlled interactions of nuclear spin qubits. We verify an analytical upper bound on the increase in capacity for channels that preserve energy and thermal states, and demonstrate that the bound can be exceeded for an energy-altering channel. We show that the switch can be used to take a thermal state to a state that is not thermal, while consuming free energy associated with the coherence of a control system. The results show how the switch can be incorporated into quantum thermodynamics experiments as an additional resource.

We upper bound and lower bound the optimal precision with which one can estimate an unknown Hamiltonian parameter via measurements of Gibbs thermal states with a known temperature. The bounds depend on the uncertainty in the Hamiltonian term that contains the parameter and on the term’s degree of noncommutativity with the full Hamiltonian: higher uncertainty and commuting operators lead to better precision. We apply the bounds to show that there exist entangled thermal states such that the parameter can be estimated with an error that decreases faster than $1/\sqrt{n}$, beating the standard quantum limit. This result governs Hamiltonians where an unknown scalar parameter (e.g., a component of a magnetic field) is coupled locally and identically to $n$ qubit sensors. In the high-temperature regime, our bounds allow for pinpointing the optimal estimation error, up to a constant prefactor. Our bounds generalize to joint estimations of multiple parameters. In this setting, we recover the high-temperature sample scaling derived previously via techniques based on quantum state discrimination and coding theory. In an application, we show that noncommuting conserved quantities hinder the estimation of chemical potentials.

We report on an experimental simulation of the spin-1 Heisenberg model with composite bosons in a one-dimensional chain based on the two-component Bose-Hubbard model. Exploiting our site- and spin-resolved quantum gas microscope, we observed faster superexchange dynamics of the spin-1 system compared to its spin-$1/2$ counterpart, which is attributed to the enhancement effect of multi-bosons. We further probed the nonequilibrium spin dynamics driven by the superexchange and single-ion anisotropy terms, unveiling the linear expansion of the spin-spin correlations, which is limited by the Lieb-Robinson bound. Based on the superexchange process, we prepared and verified the entangled qutrits pairs with these composite spin-1 bosons, potentially being applied in qutrit-based quantum information processing.

Realizing precise control over multiquanta emission is crucial for quantum information processing, especially when integrated with advanced techniques of manipulating quantum states. Here, by spinning the resonator to induce the Sagnac effect, we can obtain nonreciprocal photon-phonon and photon-magnon super-Rabi oscillations under conditions of optically driving resonance transitions. Opening dissipative channels for such super-Rabi oscillations enables the realization of directional bundle emissions of entangled photon-phonon pairs and photon-magnon pairs by transferring the pure multiquanta state to a bundled multiquanta outside of the system. This nonreciprocal emission is a flexible switch that can be controlled with precision, and simultaneous emissions of different entangled pairs (such as photon-phonon or photon-magnon pairs) can even emerge but in opposite directions by driving the resonator from different directions. This ability to flexibly manipulate the system allows us to achieve directional entangled multiquanta emitters, and has also potential applications for building hybrid quantum networks and on-chip quantum communications.

We show that multi-GeV laser wakefield electron accelerators in meter-scale, low density hydrodynamic plasma waveguides operate in a new nonlinear propagation regime dominated by sustained beating of lowest order modes of the ponderomotively modified channel; this occurs whether or not the injected pulse is linearly matched to the guide. For a continuously doped gas jet, this emergent mode beating effect leads to axially modulated enhancement of ionization injection and a multi-GeV energy spectrum of multiple quasimonoenergetic peaks; the same process in a locally doped jet produces single multi-GeV peaks with $<10\%$ energy spread. A three-stage model of drive laser pulse evolution and ionization injection characterizes the beating effect and explains our experimental results.

The kagome spin ice can host frustrated magnetic excitations by flipping its local spin. Under an inelastic tunneling condition, the tip in a scanning tunneling microscope can flip the local spin, and we apply this technique to kagome metal HoAgGe with a long-range ordered spin ice ground state. Away from defects, we discover a pair of pronounced dips in the local tunneling spectrum at symmetrical bias voltages with negative intensity values, serving as a striking inelastic tunneling signal. This signal disappears above the spin ice formation temperature and has a dependence on the magnetic fields, demonstrating its intimate relation with the spin ice magnetism. We provide a two-level spin-flip model to explain the tunneling dips considering the spin ice magnetism under spin-orbit coupling. Our results uncover a local emergent excitation of spin ice magnetism in a kagome metal, suggesting that local electrical field induced spin flip climbs over a barrier caused by spin-orbital locking.

We propose a new formalism and an effective computational framework to study self-trapped excitons (STEs) in insulators and semiconductors from first principles. Using the many-body Bethe-Salpeter equation in combination with perturbation theory, we are able to obtain the mode- and momentum-resolved exciton-phonon coupling matrix element in a perturbative scheme and explicitly solve the real space localization of the electron (hole), as well as the lattice distortion. Further, this method allows us to compute the STE potential energy surface and evaluate the STE formation energy and Stokes shift. We demonstrate our approach using two-dimensional magnetic semiconductor chromium trihalides and a wide-gap insulator BeO, the latter of which features dark excitons, and make predictions of their Stokes shift and coherent phonon generation which we hope will spark future experiments such as photoluminescence and transient absorption studies.

We propose a bond-percolation model intended to describe the consumption, and eventual exhaustion, of resources in transport networks. Edges forming minimum-length paths connecting demanded origin-destination nodes are removed if below a certain budget. As pairs of nodes are demanded and edges are removed, the macroscopic connected component of the graph disappears, i.e., the graph undergoes a percolation transition. Here, we study such a shortest-path-percolation transition in homogeneous random graphs where pairs of demanded origin-destination nodes are randomly generated, and fully characterize it by means of finite-size scaling analysis. If budget is finite, the transition is identical to the one of ordinary percolation, where a single giant cluster shrinks as edges are removed from the graph; for infinite budget, the transition becomes more abrupt than the one of ordinary percolation, being characterized by the sudden fragmentation of the giant connected component into a multitude of clusters of similar size.

Learning physical properties of high-dimensional states is crucial for developing quantum technologies but usually consumes an exceedingly large number of samples which are difficult to afford in practice. In this Letter, we use the methodology of quantum metrology to tackle this difficulty, proposing a strategy built upon entangled measurements for dramatically reducing sample complexity. The strategy, whose characteristic feature is symmetrization of observables, is powered by the exploration of symmetric structures of states which are ubiquitous in physics. It is provably optimal under some natural assumption, efficiently implementable in a variety of contexts, and capable of being incorporated into existing methods as a basic building block. We apply the strategy to different scenarios motivated by experiments, demonstrating exponential reductions in sample complexity.

Precision spectroscopy of hyperfine splitting (HFS) is a crucial tool for investigating the structure of nuclei and testing quantum electrodynamics. However, accurate theoretical predictions are hindered by two-photon exchange (TPE) effects. We propose a novel formalism that accounts for nuclear excitations and recoil in TPE, providing a model-independent description of TPE effects on HFS in light ordinary and muonic atoms. Combining our formalism with pionless effective field theory at next-to-next-to-leading order, the predicted TPE effects on HFS are 41.7(4.4) kHz and 0.117(13) meV for the 1S state in deuterium and the 2S state in muonic deuterium. These results align within $1\sigma$ and $1.3\sigma$ from recent measurements and highlight the importance of nuclear structure effects on HFS and indicate the value of more precise measurements in future experiments.

Understanding spin and lattice excitations in a metallic magnetic ordered system forms the basis to unveil the magnetic and lattice exchange couplings and their interactions with itinerant electrons. Kagome lattice antiferromagnet FeGe is interesting because it displays a rare charge density wave (CDW) deep inside the antiferromagnetic ordered phase that interacts with the magnetic order. We use neutron scattering to study the evolution of spin and lattice excitations across the CDW transition $T_{\mathrm{CDW}}$ in FeGe. While spin excitations below $\sim 100\mathrm{meV}$ can be well described by spin waves of a spin-1 Heisenberg Hamiltonian, spin excitations at higher energies are centered around the Brillouin zone boundary and extend up to $\sim 180\mathrm{meV}$ consistent with quasiparticle excitations across spin-polarized electron-hole Fermi surfaces. Furthermore, $c$-axis spin wave dispersion and Fe-Ge optical phonon modes show a clear hardening below $T_{\mathrm{CDW}}$ due to spin-charge-lattice coupling but with no evidence of a phonon Kohn anomaly. By comparing our experimental results with density functional theory calculations in absolute units, we conclude that FeGe is a Hund’s metal in the intermediate correlated regime where magnetism has contributions from both itinerant and localized electrons arising from spin polarized electronic bands near the Fermi level.