The liquid-to-solid phase transition is a complex process that is difficult to investigate experimentally with sufficient spatial and temporal resolution. A key aspect of the transition is the formation of a critical seed of the crystalline phase in a supercooled liquid, that is, a liquid in a metastable state below the melting temperature. This stochastic process is commonly described within the framework of classical nucleation theory, but accurate tests of the theory in atomic and molecular liquids are challenging. Here, we employ femtosecond x-ray diffraction from microscopic liquid jets to study crystal nucleation in supercooled liquids of the rare gases argon and krypton. Our results provide stringent limits to the validity of classical nucleation theory in atomic liquids, and offer the long-sought possibility of testing nonclassical extensions of the theory.

The disorder operator is often designed to reveal the conformal field theory (CFT) information in quantum many-body systems. By using large-scale quantum Monte Carlo simulation, we study the scaling behavior of disorder operators on the boundary in the two-dimensional Heisenberg model on the square-octagon lattice with gapless topological edge state. In the Affleck-Kennedy-Lieb-Tasaki phase, the disorder operator is shown to hold the perimeter scaling with a logarithmic term associated with the Luttinger liquid parameter $K$. This effective Luttinger liquid parameter $K$ reflects the low-energy physics and CFT for $(1+1)\mathrm{D}$ boundary. At bulk critical point, the effective $K$ is suppressed but it keeps finite value, indicating the coupling between the gapless edge state and bulk fluctuation. The logarithmic term numerically captures this coupling picture, which reveals the $(1+1)\mathrm{D}$ $\mathrm{SU}(2{)}_1$ CFT and $(2+1)\mathrm{D}$ $O(3)$ CFT at boundary criticality. Our Letter paves a new way to study the exotic boundary state and boundary criticality.

In this Letter, we propose an exotic quantum state that does not order at zero temperature in a Rydberg atom array with antiblockade mechanism. By performing an unbiased large-scale quantum Monte Carlo simulation, we investigate a minimal model with facilitated excitation in a disorder-free system. At zero temperature, this model exhibits a heterogeneous structure of liquid and glass mixture. This state, dubbed quantum slush state, features a quasi-long-range order with an algebraic decay for its correlation function, and is different from most well-established quantum phases of matter.

Emitter dephasing is one of the key issues in the performance of solid-state single-photon sources. Among the various sources of dephasing, acoustic phonons play a central role in adding decoherence to the single-photon emission. Here, we demonstrate that it is possible to tune and engineer the coherence of photons emitted from a single ${\mathrm{WSe}}_2$ monolayer quantum dot via selectively coupling it to a spectral cavity resonance. We utilize an open cavity to demonstrate spectral enhancement, leveling, and suppression of the highly asymmetric phonon sideband, finding excellent agreement with a microscopic description of the exciton-phonon dephasing in a truly two-dimensional system. Moreover, the impact of cavity tuning on the dephasing is directly assessed via optical interferometry, which points out the capability to utilize light-matter coupling to steer and design dephasing and coherence of quantum emitters in atomically thin crystals.

When two active Brownian particles collide, they slide along each other until they can continue their free motion. For persistence lengths much larger than the particle diameter, the directors do not change, but the collision can be modeled as producing a net displacement on the particles compared to their free motion in the absence of the encounter. With these elements, a Boltzmann-Enskog-like kinetic theory is built. A linear stability analysis of the homogeneous state predicts a density instability resulting from the effective velocity reduction of tagged particles predicted by the theory.

We analyze the flow physics inside the body cavity and downstream the deep-sea glass sponge Euplectella aspergillum. We provide evidence that the helical skeletal motifs of the sponge give rise to a rich fluid dynamic field, allowing the organism to scavenge flow from the bottom of the sea and promoting a spontaneous, organized vertical flow within its body cavity toward the osculum. Our analysis points at a functional adaptation of the organism, which can passively divert flow through the osculum in unfavorable, low ambient currents, with no need for active pumping, with potential repercussions in functional ecology, as well as the design of chemical reactors, air-treatment units, and civil and aeronaval structures.

Low temperature phase separation in mixtures of ${}^3\mathrm{H}\mathrm{e}$ and ${}^4\mathrm{H}\mathrm{e}$ isotopes is a unique property of quantum fluids. Hydrogen has long been considered as another potential quantum liquid and has been predicted to be superfluid at $T\le 1\mathrm{K}$, well below freezing temperature of $\approx 14\mathrm{K}$. Phase separation has also been predicted in mixtures of para-${\mathrm{H}}_2$ and ${\mathrm{D}}_2$ at temperatures $\le 3\mathrm{K}$. To defer the freezing, we produced clusters containing para-${\mathrm{H}}_2$ and ${\mathrm{D}}_2$ at an estimated temperature of $\approx 2\mathrm{K}$ whose state was studied by vibrational Raman spectroscopy. The results indicate that the clusters are liquid and show the phase separation of the isotopes. The phase separation is further corroborated by the quantum molecular dynamics simulation.

Reliable manipulation of non-Abelian Ising anyons supported by Kitaev spin liquids may enable intrinsically fault-tolerant quantum computation. Here, we introduce a standalone scheme for both generating and detecting individual Ising anyons using tunable gate voltages in a heterostructure containing a non-Abelian Kitaev spin liquid and a monolayer semiconductor. The key ingredients of our setup are a Kondo coupling to stabilize an Ising anyon in the spin liquid around each electron in the semiconductor, and a large charging energy to allow control over the electron numbers in distinct gate-defined regions of the semiconductor. In particular, a single Ising anyon can be generated at a disk-shaped region by gate tuning its electron number to one, while it can be interferometrically detected by measuring the electrical conductance of a ring-shaped region around it whose electron number is allowed to fluctuate between zero and one. We provide concrete experimental guidelines for implementing our proposal in promising candidate materials like $\alpha \text{−}{\mathrm{RuCl}}_3$.

In order to determine the structural relaxation time of a polymer glass during deformation, a strain rate switching experiment is performed in the steady-state plastic flow regime. A lightly cross-linked poly(methylmethacrylate) glass was utilized and, simultaneously, the segmental motion in the glass was quantified using an optical probe reorientation method. After the strain rate switch, a nonmonotonic stress response is observed, consistent with previous work. The correlation time for segmental motion, in contrast, monotonically evolves toward a new steady state, providing an unambiguous measurement of the structural relaxation time during deformation, which is found to be approximately equal to the segmental correlation time. The Chen-Schweizer model qualitatively predicts the changes in the segmental correlation time and the observed nonmonotonic stress response. In addition, our experiments are reasonably consistent with the material time assumption used in polymer deformation modeling; in this approach, the response of a polymer glass to a large deformation is described by combining a linear-response model with a time-dependent segmental correlation time.

A fully homomorphic encryption system enables computation on encrypted data without the necessity for prior decryption. This facilitates the seamless establishment of a secure quantum channel, bridging the server and client components, and thereby providing the client with secure access to the server’s substantial computational capacity for executing quantum operations. However, traditional homomorphic encryption systems lack scalability, programmability, and stability. In this Letter, we experimentally demonstrate a proof-of-concept implementation of a homomorphic encryption scheme on a compact quantum chip, verifying the feasibility of using photonic chips for quantum homomorphic encryption. Our work not only provides a solution for circuit expansion, addressing the longstanding challenge of scalability while significantly reducing the size of quantum network infrastructure, but also lays the groundwork for the development of highly sophisticated quantum fully homomorphic encryption systems.

The Electron-Ion Collider (EIC), to be constructed at Brookhaven National Laboratory, will collide polarized high-energy electron beams with hadron beams, achieving luminosities of up to $1.0\times {10}^{34}{\mathrm{cm}}^{-2}{\mathrm{s}}^{-1}$ in the center-of-mass energy range of 20–140 GeV. To achieve such high luminosity, the EIC will employ small and flat beams at the interaction point. In the hadron storage ring of the EIC, the ratio of horizontal to vertical emittances is approximately $11:1$. In contrast, in previous or existing hadron colliders, the horizontal and vertical emittances are typically similar or closely matched. At the Relativistic Heavy Ion Collider (RHIC), we experimentally demonstrated a large transverse emittance ratio of $11:1$ with gold ion beams at a particle energy of 100 GeV per nucleon, thanks to stochastic cooling and fine decoupling. Furthermore, we demonstrated collisions with flat beams, featuring a transverse beam size ratio of $3:1$ for the first time at the RHIC.

Chiral crystals and molecules were recently predicted to form an intriguing platform for unconventional orbital physics. Here, we report the observation of chirality-driven orbital textures in the bulk electronic structure of CoSi, a prototype member of the cubic B20 family of chiral crystals. Using circular dichroism in soft x-ray angle-resolved photoemission, we demonstrate the formation of a bulk orbital-angular-momentum texture and monopolelike orbital-momentum locking that depends on crystal handedness. We introduce the intrinsic chiral circular dichroism, $ic\mathrm{CD}$, as a differential photoemission observable and a natural probe of chiral electron states. Our findings render chiral crystals promising for spin-orbitronics applications.

Stacking ferroelectricity (SFE) has been discovered in a wide range of van der Waals materials and holds promise for applications, including photovoltaics and high-density memory devices. We show that the microscopic origin of out-of-plane stacking ferroelectric polarization can be generally understood as a consequence of a nontrivial Berry phase borne out of an effective Su-Schrieffer-Heeger model description with broken sublattice symmetry, thus elucidating the quantum-geometric origin of polarization in the extremely nonperiodic bilayer limit. Our theory applies to known stacking ferroelectrics such as bilayer transition-metal dichalcogenides in $3R$ and $T_{\mathrm{d}}$ phases, as well as general $AB$-stacked honeycomb bilayers with staggered sublattice potential. Our explanatory and self-consistent framework based on the quantum-geometric perspective establishes quantitative understanding of out-of-plane SFE materials beyond symmetry principles.

Deterministic chaos permits a precise notion of a “perfect measurement” as one that, when obtained repeatedly, captures all of the information created by the system’s evolution with minimal redundancy. Finding an optimal measurement is challenging and has generally required intimate knowledge of the dynamics in the few cases where it has been done. We establish an equivalence between a perfect measurement and a variant of the information bottleneck. As a consequence, we can employ machine learning to optimize measurement processes that efficiently extract information from trajectory data. We obtain approximately optimal measurements for multiple chaotic maps and lay the necessary groundwork for efficient information extraction from general time series.

We present a new nucleosynthesis process that may take place on neutron-rich ejecta experiencing an intensive neutrino flux. The nucleosynthesis proceeds similarly to the standard $r$ process, a sequence of neutron captures and beta decays with, however, charged-current neutrino absorption reactions on nuclei operating much faster than beta decays. Once neutron-capture reactions freeze out the produced $r$ process, neutron-rich nuclei undergo a fast conversion of neutrons into protons and are pushed even beyond the $\beta$ stability line, producing the neutron-deficient $p$ nuclei. This scenario, which we denote as the $\nu r$ process, provides an alternative channel for the production of $p$ nuclei and the short-lived nucleus ${}^{92}\mathrm{Nb}$. We discuss the necessary conditions posed on the astrophysical site for the $\nu r$ process to be realized in nature. While these conditions are not fulfilled by current neutrino-hydrodynamic models of $r$-process sites, future models, including more complex physics and a larger variety of outflow conditions, may achieve the necessary conditions in some regions of the ejecta.

Recent experimental developments in multimode nonlinear photonic circuits (MMNPCs), have motivated the development of an optical thermodynamic theory that describes the equilibrium properties of an initial beam excitation. However, a nonequilibrium transport theory for these systems, when they are in contact with thermal reservoirs, is still terra incognita. Here, by combining Landauer and kinematics formalisms we develop a universal one-parameter scaling theory that describes the whole transport behavior from the ballistic to the diffusive regime, including both positive and negative optical temperature scenarios. We also derive a photonic version of the Wiedemann-Franz law that connects the thermal and power conductivities. Our work paves the way toward a fundamental understanding of the transport properties of MMNPCs and may be useful for the design of all-optical cooling protocols.

We introduce density imbalanced electron-hole bilayers at a commensurate $2:1$ density ratio as a platform for realizing novel phases of electrons, excitons, and trions. Through the independently tunable carrier densities and interlayer spacing, competition between kinetic energy, intralayer repulsion, and interlayer attraction yields a rich phase diagram. By a combination of theoretical analysis and numerical calculation, we find a variety of strong-coupling phases in different parameter regions, including quantum crystals of electrons, excitons, and trions. We also propose an “electron-exciton supersolid” phase that features electron crystallization and exciton superfluidity simultaneously. The material realization and experimental signature of these phases are discussed in the context of semiconductor transition metal dichalcogenide bilayers.

The realistic interpretation of classical theory assumes that every classical system has well-defined properties, which may be unknown to the observer but are nevertheless part of reality and can, in principle, be revealed by measurements. Here we show that this interpretation can, in principle, be falsified if classical systems coexist with other types of physical systems. To make this point, we construct a toy theory that (i) includes classical theory as a subtheory and (ii) allows classical systems to be entangled with another type of system, called anticlassical. We show that our toy theory allows for the violation of Bell inequalities in two-party scenarios where one of the settings corresponds to a local measurement performed on a classical system alone. Building on this fact, we show that measurement outcomes in classical theory cannot, in general, be regarded as predetermined by the state of an underlying reality.

We present a framework to integrate tensor network (TN) methods with reinforcement learning (RL) for solving dynamical optimization tasks. We consider the RL actor-critic method, a model-free approach for solving RL problems, and introduce TNs as the approximators for its policy and value functions. Our “actor-critic with tensor networks” (ACTeN) method is especially well suited to problems with large and factorizable state and action spaces. As an illustration of the applicability of ACTeN we solve the exponentially hard task of sampling rare trajectories in two paradigmatic stochastic models, the East model of glasses and the asymmetric simple exclusion process, the latter being particularly challenging to other methods due to the absence of detailed balance. With substantial potential for further integration with the vast array of existing RL methods, the approach introduced here is promising both for applications in physics and to multi-agent RL problems more generally.

The demonstration of a topological band inversion constitutes the most elementary proof of a quantum spin Hall insulator (QSHI). On a fundamental level, such an inverted band gap is intrinsically related to the bulk Berry curvature, a gauge-invariant fingerprint of the wave function’s quantum geometric properties in Hilbert space. Intimately tied to orbital angular momentum (OAM), the Berry curvature can be, in principle, extracted from circular dichroism in angle-resolved photoemission spectroscopy (CD-ARPES), were it not for interfering final state photoelectron emission channels that obscure the initial state OAM signature. Here, we outline a full-experimental strategy to avoid such interference artifacts and isolate the clean OAM from the CD-ARPES response. Bench-marking this strategy for the recently discovered atomic monolayer system indenene, we demonstrate its distinct QSHI character and establish CD-ARPES as a scalable bulk probe to experimentally classify the topology of two-dimensional quantum materials with time reversal symmetry.