A Bose condensate, subject to periodic modulation of the two-body interactions, was recently observed to emit matter-wave jets resembling fireworks [Nature (London) 551, 356 (2017)]. In this Letter, combining experiment with numerical simulation, we demonstrate that these “Bose fireworks” represent a late stage in a complex time evolution of the driven condensate. We identify a “density wave” stage which precedes jet emission and results from the interference of matter waves. The density waves self-organize and self-amplify without breaking long range translational symmetry. This density wave structure deterministically establishes the template for the subsequent patterns of the emitted jets. Moreover, our simulations, in good agreement with experiment, address an apparent asymmetry in the jet pattern, and show that it is fully consistent with momentum conservation.

Twisted light carrying orbital angular momentum (OAM) provides an additional degree of freedom for modern optics and an emerging resource for both classical and quantum information technologies. Its inherently infinite dimensions can potentially be exploited by using mode multiplexing to enhance data capacity for sustaining the unprecedented growth in big data and internet traffic and can be encoded to build large-scale quantum computing machines in high-dimensional Hilbert space. While the emission of twisted light from the surface of integrated devices to free space has been widely investigated, the transmission and processing inside a photonic chip remain to be addressed. Here, we present the first laser-direct-written waveguide being capable of supporting OAM modes and experimentally demonstrate a faithful mapping of twisted light into and out of a photonic chip. The states ${\mathrm{OAM}}_0$, ${\mathrm{OAM}}_{-1}$, ${\mathrm{OAM}}_{+1}$, and their superpositions can transmit through the photonic chip with a total efficiency up to 60% with minimal crosstalk. In addition, we present the transmission of quantum twisted light states of single photons and measure the output states with single-photon imaging. Our results may add OAM as a new degree of freedom to be transmitted and manipulated in a photonic chip for high-capacity communication and high-dimensional quantum information processing.

We report on the first realization of heteronuclear dipolar quantum mixtures of highly magnetic erbium and dysprosium atoms. With a versatile experimental setup, we demonstrate binary Bose-Einstein condensation in five different Er-Dy isotope combinations, as well as one Er-Dy Bose-Fermi mixture. Finally, we present first studies of the interspecies interaction between the two species for one mixture.

We study the long-range interaction of a single ion with a highly excited ultracold Rydberg atom and report on the direct observation of an ion-induced Rydberg excitation blockade mediated over tens of micrometer distances. Our hybrid ion-atom system is directly produced from an ultracold atomic ensemble via near-threshold photoionization of a single Rydberg excitation, employing a two-photon scheme that is specifically suited for generating a very low-energy ion. The ion’s motion is precisely controlled by small electric fields, which allows us to analyze the blockade mechanism for a range of principal quantum numbers. Finally, we explore the capability of the ion as a high-sensitivity, single-atom-based electric field sensor. The observed ion-Rydberg-atom interaction is of current interest for entanglement generation or studies of ultracold chemistry in hybrid ion-atom systems.

Quantum fluids of light are a photonic counterpart to atomic Bose gases and are attracting increasing interest for probing many-body physics quantum phenomena such as superfluidity. Two different configurations are commonly used: the confined geometry where a nonlinear material is fixed inside an optical cavity and the propagating geometry where the propagation direction plays the role of an effective time for the system. The observation of the dispersion relation for elementary excitations in a photon fluid has proved to be a difficult task in both configurations with few experimental realizations. Here, we propose and implement a general method for measuring the excitations spectrum in a fluid of light, based on a group velocity measurement. We observe a Bogoliubov-like dispersion with a speed of sound scaling as the square root of the fluid density. This Letter demonstrates that a nonlinear system based on an atomic vapor pumped near resonance is a versatile and highly tunable platform to study quantum fluids of light.

We use the strong intrinsic nonlinearity of a microwave superconducting qubit with a 4 GHz transition frequency to directly detect and control the energy of a micromechanical oscillator vibrating at 25 MHz. The qubit and the oscillator are coupled electrostatically at a rate of approximately $2\pi \times 22\mathrm{MHz}$. In this far off-resonant regime, the qubit frequency is shifted by 0.52 MHz per oscillator phonon, or about 14% of the 3.7 MHz qubit linewidth. The qubit behaves as a vibrational energy detector and from its line shape we extract the phonon number distribution of the oscillator. We manipulate this distribution by driving number state sensitive sideband transitions and creating profoundly nonthermal states. Finally, by driving the lower frequency sideband transition, we cool the oscillator and increase its ground state population up to $0.48\pm 0.13$, close to a factor of 8 above its value at thermal equilibrium. These results demonstrate a new class of electromechanics experiments that are a promising strategy for quantum nondemolition measurements and nonclassical state preparation.

Coherent control of reactive atomic and molecular collision processes remains elusive experimentally due to quantum interference-based requirements. Here, with insights from symmetry conditions, a viable method for controlling Penning and associative ionization in atomic collisions is proposed. Computational applications to ${\mathrm{He}}^{*}({}^{3}S)\text{−}\mathrm{Li}({}^{2}S)$ and ${\mathrm{Ne}}^{*}({}^3{P}_2)\text{−}\mathrm{Ar}({}^1{S}_0)$ show extensive control over the ionization processes under experimentally feasible conditions.

For decades, improved theory and experiment of the $n=2$ ${}^{3}P$ fine structure of helium have allowed for increasingly precise tests of quantum electrodynamics, determinations of the fine-structure constant $\alpha$, and limitations on possible beyond-the-standard-model physics. Here we use the new frequency-offset separated-oscillatory-fields technique to measure the $2{}^3{P}_2\to 2{}^3{P}_1$ interval. Our result of 2 291 176 590(25) Hz represents a major step forward in precision for helium fine-structure measurements.

Processes that break molecular bonds are typically observed with molecules occupying a mixture of quantum states and successfully described with quasiclassical models, while a few studies have explored the distinctly quantum mechanical low-energy regime. Here, we use photodissociation of diatomic strontium molecules to demonstrate the crossover from the ultracold, quantum regime where photofragment angular distributions strongly depend on the kinetic energy to the quasiclassical regime. Using time-of-flight imaging for photodissociation channels with millikelvin reaction barriers, we explore photofragment energies in the 0.1–300 mK range experimentally and up to 3 K theoretically, and discuss the energy scale at which the crossover occurs. We find that the effects of quantum statistics can persist to high photodissociation energies.

We demonstrate a clear similarity between attoclock offset angles and Rutherford scattering angles taking the Keldysh tunneling width as the impact parameter and the vector potential of the driving pulse as the asymptotic velocity. This simple model is tested against the solution of the time-dependent Schrödinger equation using hydrogenic and screened (Yukawa) potentials of equal binding energy. We observe a smooth transition from a hydrogenic to “hard-zero” intensity dependence of the offset angle with variation of the Yukawa screening parameter. Additionally, we make a comparison with the attoclock offset angles for various noble gases obtained with the classical-trajectory Monte Carlo method. In all cases we find a close correspondence between the model predictions and numerical calculations. This suggests a largely Coulombic origin of the attoclock offset angle and casts further doubt on its interpretation in terms of a finite tunneling time.

The “trilobite”-type of molecule, predicted in 2000 and observed experimentally in 2015, arises when a Rydberg electron exerts a weak attractive force on a neutral ground state atom. Such molecules have bond lengths exceeding 100 nm. The ultralong-range chemical bond between the two atoms is a nonperturbative linear combination of the many degenerate electronic states associated with high principal quantum numbers, and the resulting electron probability distribution closely resembles a fossil trilobite from antiquity. We show how to coherently engineer this same long-range orbital through a sequence of electric and magnetic field pulses even when the ground-state atom is not present and propose several methods to observe the resulting orbital. The existence of such a ghost chemical bond in which an electron reaches out from one atom to a nonexistent second atom is a consequence of the high level degeneracy.

Measuring inelastic rates with partial-wave resolution requires temperatures close to a Kelvin or below, even for the lightest molecule. In a recent experiment, Perreault, Mukherjee, and Zare [Nat. Chem. 10, 561 (2018).] studied collisional relaxation of excited HD molecules in the $v=1$, $j=2$ state by para- and ortho-${\mathrm{H}}_2$ at a temperature of about 1 K, extracting the angular distribution of scattered HD in the $v=1$, $j=0$ state. By state preparation of the HD molecules, control of the angular distribution of scattered HD was demonstrated. Here, we report a first-principles simulation of that experiment which enables us to attribute the main features of the observed angular distribution to a single $L=2$ partial-wave shape resonance. Our results demonstrate important stereodynamical insights that can be gained when numerically exact quantum scattering calculations are combined with experimental results in the few-partial-wave regime.

We present measurements of the dynamical structure factor $S(q,\omega )$ of an interacting one-dimensional Fermi gas for small excitation energies. We use the two lowest hyperfine levels of the ${}^6\mathrm{Li}$ atom to form a pseudospin-$1/2$ system whose $s$-wave interactions are tunable via a Feshbach resonance. The atoms are confined to one dimension by a two-dimensional optical lattice. Bragg spectroscopy is used to measure a response of the gas to density (“charge”) mode excitations at a momentum $q$ and frequency $\omega$, as a function of the interaction strength. The spectrum is obtained by varying $\omega$, while the angle between two laser beams determines $q$, which is fixed to be less than the Fermi momentum $k_F$. The measurements agree well with Tomonaga-Luttinger theory.

We report on nondestructive imaging of optically trapped calcium monofluoride molecules using in situ $\mathrm{\Lambda }$-enhanced gray molasses cooling. 200 times more fluorescence is obtained compared to destructive on-resonance imaging, and the trapped molecules remain at a temperature of $20\mu \mathrm{K}$. The achieved number of scattered photons makes possible nondestructive single-shot detection of single molecules with high fidelity.

We demonstrate, theoretically and experimentally, the generation of hexapartite modal entanglement by the optical parametric oscillator (OPO) operating above the oscillation threshold. We show that the OPO generates a rich structure of entanglement among sets of six optical sideband modes interacting through the nonlinear crystal. The class of quantum states thus produced can be controlled by a single parameter, the power of the external laser that pumps the system. Our platform allows for the generation of massive entanglement among many optical modes with well defined but vastly different frequencies, potentially bridging nodes of a multicolor quantum network.

We investigate the minimal Hilbert-space dimension for a system to be synchronized. We first show that qubits cannot be synchronized due to the lack of a limit cycle. Moving to larger spin values, we demonstrate that a single spin 1 can be phase locked to a weak external signal of similar frequency and exhibits all the standard features of the theory of synchronization. Our findings rely on the Husimi $Q$ representation based on spin coherent states which we propose as a tool to obtain a phase portrait.

We observe the unconventional photon blockade effect in quantum dot cavity QED, which, in contrast to the conventional photon blockade, operates in the weak coupling regime. A single quantum dot transition is simultaneously coupled to two orthogonally polarized optical cavity modes, and by careful tuning of the input and output state of polarization, the unconventional photon blockade effect is observed. We find a minimum second-order correlation $g^{(2)}(0)\approx 0.37$, which corresponds to $g^{(2)}(0)\approx 0.005$ when corrected for detector jitter, and observe the expected polarization dependency and photon bunching and antibunching; close by in parameter space, which indicates the abrupt change from phase to amplitude squeezing.

We have observed the unconventional photon blockade effect for microwave photons using two coupled superconducting resonators. As opposed to the conventional blockade, only weakly nonlinear resonators are required. The blockade is revealed through measurements of the second order correlation function $g^{(2)}(t)$ of the microwave field inside one of the two resonators. The lowest measured value of $g^{(2)}(0)$ is 0.4 for a resonator population of approximately ${10}^{-2}$ photons. The time evolution of $g^{(2)}(t)$ exhibits an oscillatory behavior, which is characteristic of the unconventional photon blockade.

We report on rotating an optically trapped silica nanoparticle in vacuum by transferring spin angular momentum of light to the particle’s mechanical angular momentum. At sufficiently low damping, realized at pressures below ${10}^{-5}\mathrm{mbar}$, we observe rotation frequencies of single 100 nm particles exceeding 1 GHz. We find that the steady-state rotation frequency scales linearly with the optical trapping power and inversely with pressure, consistent with theoretical considerations based on conservation of angular momentum. Rapidly changing the polarization of the trapping light allows us to extract the pressure-dependent response time of the particle’s rotational degree of freedom.

Levitated optomechanics has great potential in precision measurements, thermodynamics, macroscopic quantum mechanics, and quantum sensing. Here we synthesize and optically levitate silica nanodumbbells in high vacuum. With a linearly polarized laser, we observe the torsional vibration of an optically levitated nanodumbbell. This levitated nanodumbbell torsion balance is a novel analog of the Cavendish torsion balance, and provides rare opportunities to observe the Casimir torque and probe the quantum nature of gravity as proposed recently. With a circularly polarized laser, we drive a 170-nm-diameter nanodumbbell to rotate beyond 1 GHz, which is the fastest nanomechanical rotor realized to date. Smaller silica nanodumbbells can sustain higher rotation frequencies. Such ultrafast rotation may be used to study material properties and probe vacuum friction.