We find that laser-induced local melting attracts and deforms grain boundaries in 2D colloidal crystals. When a melted region in contact with the edge of a crystal grain recrystallizes, it deforms the grain boundary—this attraction is driven by the multiplicity of deformed grain boundary configurations. Furthermore, the attraction provides a method to fabricate artificial colloidal crystal grains of arbitrary shape, enabling new experimental studies of grain boundary dynamics and ultimately hinting at a novel approach for fabricating materials with designer microstructures.

We study a bilayer GaAs hole system that hosts two distinct many-body phases at low temperatures and high perpendicular magnetic fields. The higher-density (top) layer develops a Fermi sea of composite fermions (CFs) in its half-filled lowest Landau level, while the lower-density (bottom) layer forms a Wigner crystal (WC) as its filling becomes very small. Owing to the interlayer interaction, the CFs in the top layer feel the periodic Coulomb potential of the WC in the bottom layer. We measure the magnetoresistance of the top layer while changing the bottom-layer density. As the WC layer density increases, the resistance peaks separating the adjacent fractional quantum Hall states in the top layer change nonmonotonically and attain maximum values when the cyclotron orbit of the CFs encloses one WC lattice point. These features disappear at $T=275\mathrm{mK}$ when the WC melts. The observation of such geometric resonance features is unprecedented and surprising as it implies that the CFs retain a well-defined cyclotron orbit and Fermi wave vector even deep in the fractional quantum Hall regime, far from half-filling.

Electrical control of structural and physical properties is a long-sought, but elusive goal of contemporary science and technology. We demonstrate that a combination of strong spin-orbit interactions (SOI) and a canted antiferromagnetic Mott state is sufficient to attain that goal. The antiferromagnetic insulator ${\mathrm{Sr}}_2{\mathrm{IrO}}_4$ provides a model system in which strong SOI lock canted Ir magnetic moments to ${\mathrm{IrO}}_6$ octahedra, causing them to rigidly rotate together. A novel coupling between an applied electrical current and the canting angle reduces the Néel temperature and drives a large, nonlinear lattice expansion that closely tracks the magnetization, increases the electron mobility, and precipitates a unique resistive switching effect. Our observations open new avenues for understanding fundamental physics driven by strong SOI in condensed matter, and provide a new paradigm for functional materials and devices.

X-ray free-electron lasers combine a high pulse power, short pulse length, narrow bandwidth, and high degree of transverse coherence. Any increase in the photon pulse power, while shortening the pulse length, will further push the frontier on several key x-ray free-electron laser applications including single-molecule imaging and novel nonlinear x-ray methods. This Letter shows experimental results at the Linac Coherent Light Source raising its maximum power to more than 300% of the current limit while reducing the photon pulse length to 10 fs. This was achieved by minimizing residual transverse-longitudinal centroid beam offsets and beam yaw and by correcting the dispersion when operating over 6 kA peak current with a longitudinally shaped beam.

The magnetotransport properties of epitaxial films of ${\mathrm{Cd}}_3{\mathrm{As}}_2$, a paradigm three-dimensional Dirac semimetal, are investigated. We show that an energy gap opens in the bulk electronic states of sufficiently thin films and, at low temperatures, carriers residing in surface states dominate the electrical transport. The carriers in these states are sufficiently mobile to give rise to a quantized Hall effect. The sharp quantization demonstrates surface transport that is virtually free of parasitic bulk conduction and paves the way for novel quantum transport studies in this class of topological materials. Our results also demonstrate that heterostructuring approaches can be used to study and engineer quantum states in topological semimetals.

We report strong coupling between light and polaron optical excitations in a doped organic semiconductor microcavity at room temperature. Codepositing ${\mathrm{MoO}}_3$ and the hole transport material 4, $4^{\prime }$-cyclohexylidenebis[$N$, $N$-bis(4-methylphenyl)benzenamine] introduces a large hole density with a narrow linewidth optical transition centered at 1.8 eV and an absorption coefficient exceeding ${10}^4{\mathrm{cm}}^{-1}$. Coupling this transition to a Fabry-Pérot cavity mode yields upper and lower polaron polariton branches that are clearly resolved in angle-dependent reflectivity with a vacuum Rabi splitting $\hslash {\mathrm{\Omega }}_R>0.3\mathrm{eV}$. This result establishes a path to electrically control polaritons in organic semiconductors and may lead to increased polariton-polariton Coulombic interactions that lower the threshold for nonlinear phenomena such as polariton condensation and lasing.

The fast evaporative cooling of micrometer-sized water droplets in a vacuum offers the appealing possibility to investigate supercooled water—below the melting point but still a liquid—at temperatures far beyond the state of the art. However, it is challenging to obtain a reliable value of the droplet temperature under such extreme experimental conditions. Here, the observation of morphology-dependent resonances in the Raman scattering from a train of perfectly uniform water droplets allows us to measure the variation in droplet size resulting from evaporative mass losses with an absolute precision of better than 0.2%. This finding proves crucial to an unambiguous determination of the droplet temperature. In particular, we find that a fraction of water droplets with an initial diameter of $6379\pm 12\mathrm{nm}$ remain liquid down to $230.6\pm 0.6\mathrm{K}$. Our results question temperature estimates reported recently for larger supercooled water droplets and provide valuable information on the hydrogen-bond network in liquid water in the hard-to-access deeply supercooled regime.

Gravitational waves (GWs) cause the apparent position of distant stars to oscillate with a characteristic pattern on the sky. Astrometric measurements (e.g., those made by Gaia) provide a new way to search for GWs. The main difficulty facing such a search is the large size of the data set; Gaia observes more than one billion stars. In this Letter the problem of searching for GWs from individually resolvable supermassive black hole binaries using astrometry is addressed for the first time; it is demonstrated how the data set can be compressed by a factor of more than $10^6$, with a loss of sensitivity of less than 1%. This technique was successfully used to recover artificially injected GW signals from mock Gaia data and to assess the GW sensitivity of Gaia. Throughout the Letter the complementarity of Gaia and pulsar timing searches for GWs is highlighted.

Theoretical predictions have suggested that molecular motion at interfaces—which influences processes including heterogeneous catalysis, (bio)chemical sensing, lubrication and adhesion, and nanomaterial self-assembly—may be dominated by hypothetical “hops” through the adjacent liquid phase, where a diffusing molecule readsorbs after a given hop according to a probabilistic “sticking coefficient.” Here, we use three-dimensional (3D) single-molecule tracking to explicitly visualize this process for human serum albumin at solid-liquid interfaces that exert varying electrostatic interactions on the biomacromolecule. Following desorption from the interface, a molecule experiences multiple unproductive surface encounters before readsorption. An average of approximately seven surface collisions is required for the repulsive surfaces, decreasing to approximately two and a half for surfaces that are more attractive. The hops themselves are also influenced by long-range interactions, with increased electrostatic repulsion causing hops of longer duration and distance. These findings explicitly demonstrate that interfacial diffusion is dominated by biased 3D Brownian motion involving bulk-surface coupling and that it can be controlled by influencing short- and long-range adsorbate-surface interactions.

The Laguerre-Gaussian (LG) modes constitute a complete basis set for representing the transverse structure of a paraxial photon field in free space. Earlier workers have shown how to construct a device for sorting a photon according to its azimuthal LG mode index, which describes the orbital angular momentum (OAM) carried by the field. In this paper we propose and demonstrate a mode sorter based on the fractional Fourier transform to efficiently decompose the optical field according to its radial profile. We experimentally characterize the performance of our implementation by separating individual radial modes as well as superposition states. The reported scheme can, in principle, achieve unit efficiency and thus can be suitable for applications that involve quantum states of light. This approach can be readily combined with existing OAM mode sorters to provide a complete characterization of the transverse profile of the optical field.

We report on the realization of a matter-wave interferometer based on single-photon interaction on the ultranarrow optical clock transition of strontium atoms. We experimentally demonstrate its operation as a gravimeter and as a gravity gradiometer. No reduction of interferometric contrast was observed for a total interferometer time up to $\sim 10\mathrm{ms}$, limited by geometric constraints of the apparatus. Single-photon interferometers represent a new class of high-precision sensors that could be used for the detection of gravitational waves in so far unexplored frequency ranges and to enlighten the boundary between quantum mechanics and general relativity.

Quantum confinement permits the existence of multiple terahertz magnon modes in atomically engineered ultrathin magnetic films and multilayers. By means of spin-polarized high-resolution electron energy-loss spectroscopy, we report on the direct experimental detection of all exchange-dominated terahertz confined magnon modes in a 3 ML Co film. We demonstrate that, by tuning the structural and magnetic properties of the Co film, through its epitaxial growth on different surfaces, e.g., Ir(001), Cu(001), and Pt(111), one can achieve entirely different in-plane magnon dispersions, characterized by positive and negative group velocities. Our first-principles calculations show that spin-dependent many-body correlation effects in Co films play an important role in the determination of the energies of confined magnon modes. Our results suggest a pathway towards the engineering of the group velocity of confined ultrafast magnons.

The low-energy quasiparticles of Weyl semimetals are a condensed-matter realization of the Weyl fermions introduced in relativistic field theory. Chiral anomaly, the nonconservation of the chiral charge under parallel electric and magnetic fields, is arguably the most important phenomenon of Weyl semimetals and has been explained as an imbalance between the occupancies of the gapless, zeroth Landau levels with opposite chiralities. This widely accepted picture has served as the basis for subsequent studies. Here we report the breakdown of the chiral anomaly in Weyl semimetals in a strong magnetic field based on ab initio calculations. A sizable energy gap that depends sensitively on the direction of the magnetic field may open up due to the mixing of the zeroth Landau levels associated with the opposite-chirality Weyl points that are away from each other in the Brillouin zone. Our study provides a theoretical framework for understanding a wide range of phenomena closely related to the chiral anomaly in topological semimetals, such as magnetotransport, thermoelectric responses, and plasmons, to name a few.

The propagation of light beams is well described using the paraxial approximation, where field components along the propagation direction are usually neglected. For strongly inhomogeneous or shaped light fields, however, this approximation may fail, leading to intriguing variations of the light-matter interaction. This is the case of twisted light having opposite orbital and spin angular momenta. We compare experimental data for the excitation of a quadrupole transition in a single trapped ${}^{40}{\mathrm{Ca}}^{+}$ ion from Schmiegelow et al. [Nat. Commun. 7, 12998 (2016)] with a complete model where longitudinal components of the electric field are taken into account. Our model matches the experimental data and excludes by 11 standard deviations the approximation of a complete transverse field. This demonstrates the relevance of all field components for the interaction of twisted light with matter.

We provide a new perspective on fracton topological phases, a class of three-dimensional topologically ordered phases with unconventional fractionalized excitations that are either completely immobile or only mobile along particular lines or planes. We demonstrate that a wide range of these fracton phases can be constructed by strongly coupling mutually intersecting spin chains and explain via a concrete example how such a coupled-spin-chain construction illuminates the generic properties of a fracton phase. In particular, we describe a systematic translation from each coupled-spin-chain construction into a parton construction where the partons correspond to the excitations that are mobile along lines. Remarkably, our construction of fracton phases is inherently based on spin models involving only two-spin interactions and thus brings us closer to their experimental realization.

Gravity gradients represent a major obstacle in high-precision measurements by atom interferometry. Controlling their effects to the required stability and accuracy imposes very stringent requirements on the relative positioning of freely falling atomic clouds, as in the case of precise tests of Einstein’s equivalence principle. We demonstrate a new method to exactly compensate the effects introduced by gravity gradients in a Raman-pulse atom interferometer. By shifting the frequency of the Raman lasers during the central $\pi$ pulse, it is possible to cancel the initial position- and velocity-dependent phase shift produced by gravity gradients. We apply this technique to simultaneous interferometers positioned along the vertical direction and demonstrate a new method for measuring local gravity gradients that does not require precise knowledge of the relative position between the atomic clouds. Based on this method, we also propose an improved scheme to determine the Newtonian gravitational constant $G$ towards the 10 ppm relative uncertainty.

The modern semiclassical theory of a Bloch electron in a magnetic field encompasses the orbital magnetization and geometric phase. Beyond this semiclassical theory lies the quantum description of field-induced tunneling between semiclassical orbits, known as magnetic breakdown. Here, we synthesize the modern semiclassical notions with quantum tunneling—into a single Bohr-Sommerfeld quantization rule that is predictive of magnetic energy levels. This rule is applicable to a host of topological solids with unremovable geometric phase, that also unavoidably undergo breakdown. A notion of topological invariants is formulated that nonperturbatively encode tunneling, and is measurable in the de Haas–van Alphen effect. Case studies are discussed for topological metals near a metal-insulator transition and overtilted Weyl fermions.

The detection of an electromagnetic counterpart (GRB 170817A) to the gravitational-wave signal (GW170817) from the merger of two neutron stars opens a completely new arena for testing theories of gravity. We show that this measurement allows us to place stringent constraints on general scalar-tensor and vector-tensor theories, while allowing us to place an independent bound on the graviton mass in bimetric theories of gravity. These constraints severely reduce the viable range of cosmological models that have been proposed as alternatives to general relativistic cosmology.

The observation of GW170817 and its electromagnetic counterpart implies that gravitational waves travel at the speed of light, with deviations smaller than a $\mathrm{few}\times {10}^{-15}$. We discuss the consequences of this experimental result for models of dark energy and modified gravity characterized by a single scalar degree of freedom. To avoid tuning, the speed of gravitational waves must be unaffected not only for our particular cosmological solution but also for nearby solutions obtained by slightly changing the matter abundance. For this to happen, the coefficients of various operators must satisfy precise relations that we discuss both in the language of the effective field theory of dark energy and in the covariant one, for Horndeski, beyond Horndeski, and degenerate higher-order theories. The simplification is dramatic: of the three functions describing quartic and quintic beyond Horndeski theories, only one remains and reduces to a standard conformal coupling to the Ricci scalar for Horndeski theories. We show that the deduced relations among operators do not introduce further tuning of the models, since they are stable under quantum corrections.

The LIGO and VIRGO Collaborations have recently announced the detection of gravitational waves from a neutron star–neutron star merger (GW170817) and the simultaneous measurement of an optical counterpart (the $\gamma$-ray burst GRB 170817A). The close arrival time of the gravitational and electromagnetic waves limits the difference in speed of photons and gravitons to be less than about 1 part in $10^{15}$. This has three important implications for cosmological scalar-tensor gravity theories that are often touted as dark energy candidates and alternatives to the $\mathrm{\Lambda }$ cold dark matter model. First, for the most general scalar-tensor theories—beyond Horndeski models—three of the five parameters appearing in the effective theory of dark energy can now be severely constrained on astrophysical scales; we present the results of combining the new gravity wave results with galaxy cluster observations. Second, the combination with the lack of strong equivalence principle violations exhibited by the supermassive black hole in M87 constrains the quartic galileon model to be cosmologically irrelevant. Finally, we derive a new bound on the disformal coupling to photons that implies that such couplings are irrelevant for the cosmic evolution of the field.