Coherence time is an essential parameter for quantum sensing, quantum information, and quantum computation. In this work, we demonstrate electron spin coherence times as long as 0.1 s for an ensemble of rubidium atoms trapped in a solid parahydrogen matrix. We explore the underlying physics limiting the coherence time. The properties of these matrix isolated atoms are very promising for future applications, including quantum sensing of nuclear spins. If combined with efficient single-atom readout, this would enable NMR and magnetic resonance imaging of single molecules cotrapped with alkali-metal atom quantum sensors within a parahydrogen matrix.

Absolute rotation rate sensing with extreme sensitivity requires a combination of several large scale gyroscopes in order to obtain the full vector of rotation. We report on the construction and operation of a four-component, tetrahedral laser gyroscope array as large as a five story building and situated in a near surface, underground laboratory. It is demonstrated that reconstruction of the full Earth rotation vector can be achieved with sub-arcsecond resolution over more than six weeks.

We demonstrate Bragg diffraction of the antibiotic ciprofloxacin and the dye molecule phthalocyanine at a thick optical grating. The observed patterns show a single dominant diffraction order with the expected dependence on the incidence angle as well as oscillating population transfer between the undiffracted and diffracted beams. We achieve an equal-amplitude splitting of $14\hslash k$ (photon momenta) and maximum momentum transfer of $18\hslash k$. This paves the way for efficient, large-momentum beam splitters and mirrors for hot and complex molecules.

Optical spectroscopy constitutes the historical path to accumulate basic knowledge on the atom and its structure. Former work based on fluorescence and resonance ionization spectroscopy enabled identifying optical spectral lines up to element 102, nobelium. The new challenges faced in this research field are the refractory nature of the heavier elements and the decreasing production yields. A new concept of ion-mobility-assisted laser spectroscopy is proposed to overcome the sensitivity limits of atomic structure investigations persisting in the region of the superheavy elements. The concept offers capabilities of both broadband-level searches and high-resolution hyperfine spectroscopy of synthetic elements beyond nobelium.

With growing interest in quantum technologies, possibilities of synchronizing quantum systems have garnered significant recent attention. In experiments with dilute ensemble of laser cooled spin-1 ${}^{87}\mathrm{Rb}$ atoms, we observe phase difference of spin coherences to synchronize with phases of external classical fields. An initial limit-cycle state of a spin-1 atom localizes in phase space due to dark-state polaritons generated by classical two-photon tone fields. In particular, when the two couplings fields are out of phase, the limit-cycle state synchronizes only with two artificially engineered, anisotropic decay rates. Furthermore, we observe a blockade of synchronization due to quantum interference and emergence of Arnold-tongue-like features. Such anisotropic decay induced synchronization of spin-1 systems with no classical analog can provide insights in open quantum systems and find applications in synchronized quantum networks.

We demonstrate the formation of a single NaCs molecule in an optical tweezer by magnetoassociation through an $s$-wave Feshbach resonance at 864.11(5) G. Starting from single atoms cooled to their motional ground states, we achieve conversion efficiencies of 47(1)%, and measure a molecular lifetime of 4.7(7) ms. By construction, the single molecules are predominantly [77(5)%] in the center-of-mass motional ground state of the tweezer. Furthermore, we produce a single $p$-wave molecule near 807 G by first preparing one of the atoms with one quantum of motional excitation. Our creation of a single weakly bound molecule in a designated internal state in the motional ground state of an optical tweezer is a crucial step towards coherent control of single molecules in optical tweezer arrays.

We investigate the number entropy $S_N$—which characterizes particle-number fluctuations between subsystems—following a quench in one-dimensional interacting many-body systems with potential disorder. We find evidence that in the regime which is expected to show many-body localization and where the entanglement entropy grows as $S\sim \ln t$ as function of time $t$, the number entropy grows as $S_N\sim \ln \ln t$, indicating continuing subdiffusive particle transport at a very slow rate. We demonstrate that this growth is consistent with a relation between entanglement and number entropy recently established for noninteracting systems.

We experimentally investigate the effects of the linear photon momentum on the momentum distributions of photoions and photoelectrons generated in one-photon ionization in an energy range of $300\mathrm{eV}\le E_{\gamma }\le 40\mathrm{keV}$. Our results show that for each ionization event the photon momentum is imparted onto the photoion, which is essentially the system’s center of mass. Nevertheless, the mean value of the ion momentum distribution along the light propagation direction is backward-directed by $-3/5$ times the photon momentum. These results experimentally confirm a 90-year-old prediction.

We present a framework for controlling the observables of a general correlated electron system driven by an incident laser field. The approach provides a prescription for the driving required to generate an arbitrary predetermined evolution for the expectation value of a chosen observable, together with a constraint on the maximum size of this expectation. To demonstrate this, we determine the laser fields required to exactly control the current in a Fermi-Hubbard system under a range of model parameters, fully controlling the nonlinear high-harmonic generation and optically observed electron dynamics in the system. This is achieved for both the uncorrelated metalliclike state and deep in the strongly correlated Mott insulating regime, flipping the optical responses of the two systems so as to mimic the other, creating “driven imposters.” We also present a general framework for the control of other dynamical variables, opening a new route for the design of driven materials with customized properties.

Optomechanical systems in the well-resolved-sideband regime are ideal for studying a myriad of quantum phenomena with mechanical systems, including backaction-evading measurements, mechanical squeezing, and nonclassical states generation. For these experiments, the mechanical oscillator should be prepared in its ground state, i.e., exhibit negligible residual excess motion compared to its zero-point motion. This can be achieved using the radiation pressure of laser light in the cavity by selectively driving the lower motional sideband, leading to sideband cooling. To date, the preparation of sideband-resolved optical systems to their zero-point energy has eluded laser cooling because of strong optical absorption heating. The alternative method of passive cooling suffers from the same problem, as the requisite milliKelvin environment is incompatible with the strong optical driving needed by many quantum protocols. Here, we employ a highly sideband-resolved silicon optomechanical crystal in a ${}^3\mathrm{He}$ buffer-gas environment at $\sim 2\mathrm{K}$ to demonstrate laser sideband cooling to a mean thermal phonon occupancy of ${0.09}_{-0.01}^{+0.02}$ quantum (self-calibrated using motional sideband asymmetry), which is $-7.4\mathrm{dB}$ of the oscillator’s zero-point energy and corresponds to 92% ground state probability. Achieving such low occupancy by laser cooling opens the door to a wide range of quantum-optomechanical experiments in the optical domain.

We report an observation of a 148-fold suppression of resonant absorption of 14.4 keV photons from $\exp (-5.2)$ to $\exp (-0.2)$ with preservation of their spectral and temporal characteristics in an ensemble of the resonant two-level ${}^{57}\mathrm{Fe}$ nuclei at room temperature. The transparency was induced via collective acoustic oscillations of nuclei. The proposed technique allows extending the concept of induced optical transparency to a hard x-ray or $\gamma$-ray range and paves the way for acoustically controllable interface between x-ray or $\gamma$-ray photons and nuclear ensembles, advancing the field of x-ray or $\gamma$-ray quantum optics.

We demonstrate a new mechanical transduction platform for individual spin qubits. In our approach, single micromagnets are trapped using a type-II superconductor in proximity of spin qubits, enabling direct magnetic coupling between the two systems. Controlling the distance between the magnet and the superconductor during cooldown, we demonstrate three-dimensional trapping with quality factors around $1\times {10}^6$ and kHz trapping frequencies. We further exploit the large magnetic moment to mass ratio of this mechanical oscillator to couple its motion to the spin degrees of freedom of an individual nitrogen vacancy center in diamond. Our approach provides a new path towards interfacing individual spin qubits with mechanical motion for testing quantum mechanics with mesoscopic objects, realization of quantum networks, and ultrasensitive metrology.

We show that the lifetime of ultracold ground-state ${}^{87}\mathrm{Rb}{}^{133}\mathrm{Cs}$ molecules in an optical trap is limited by fast optical excitation of long-lived two-body collision complexes. We partially suppress this loss mechanism by applying square-wave modulation to the trap intensity, such that the molecules spend 75% of each modulation cycle in the dark. By varying the modulation frequency, we show that the lifetime of the collision complex is $0.53\pm 0.06\mathrm{ms}$ in the dark. We find that the rate of optical excitation of the collision complex is $3_{-2}^{+4}\times {10}^3{\mathrm{W}}^{-1}{\mathrm{cm}}^2{\mathrm{s}}^{-1}$ for $\lambda =1550\mathrm{nm}$, leading to a lifetime of $<100\mathrm{ns}$ for typical trap intensities. These results explain the two-body loss observed in experiments on nonreactive bialkali molecules.

We demonstrate a 1D magneto-optical trap of the polar free radical calcium monohydroxide (CaOH). A quasiclosed cycling transition is established to scatter $\sim {10}^3$ photons per molecule, predominantly limited by interaction time. This enables radiative laser cooling of CaOH while compressing the molecular beam, leading to a significant increase in on axis beam brightness and reduction in temperature from 8.4 to 1.4 mK.

Rydberg atoms are remarkable tools for quantum simulation and computation. They are the focus of an intense experimental activity, mainly based on low-angular-momentum Rydberg states. Unfortunately, atomic motion and levels lifetime limit the experimental timescale to about $100\mu \mathrm{s}$. Here, we demonstrate two-dimensional laser trapping of long-lived circular Rydberg states for up to 10 ms. Our method is very general and opens many opportunities for quantum technologies with Rydberg atoms. The 10 ms trapping time corresponds to thousands of interaction cycles in a circular-state-based quantum simulator. It is also promising for quantum metrology and quantum information with Rydberg atoms, by bringing atom-field interaction times into unprecedented regimes.

First ever measurements of the ratios of free cyclotron frequencies of heavy, highly charged ions with $Z>50$ with relative uncertainties close to ${10}^{-11}$ are presented. Such accurate measurements have become realistic due to the construction of the novel cryogenic multi-Penning-trap mass spectrometer PENTATRAP. Based on the measured frequency ratios, the mass differences of five pairs of stable xenon isotopes, ranging from ${}^{126}\mathrm{Xe}$ to ${}^{134}\mathrm{Xe}$, have been determined. Moreover, the first direct measurement of an electron binding energy in a heavy highly charged ion, namely of the 37th atomic electron in xenon, with an uncertainty of a few eV is demonstrated. The obtained value agrees with the calculated one using two independent, different implementations of the multiconfiguration Dirac-Hartree-Fock method. PENTATRAP opens the door to future measurements of electron binding energies in highly charged heavy ions for more stringent tests of bound-state quantum electrodynamics in strong electromagnetic fields and for an investigation of the manifestation of light dark matter in isotopic chains of certain chemical elements.

We report on new measurements of $m$-fold photodetachment ($m=2-5$) of carbon anions via $K$-shell excitation and ionization. The experiments were carried out employing the photon-ion merged-beams technique at a synchrotron light source. While previous measurements were restricted to double detachment ($m=2$) and to just the lowest-energy $K$-shell resonance at about 282 eV, our absolute experimental $m$-fold detachment cross sections at photon energies of up to 1000 eV exhibit a wealth of new thresholds and resonances. We tentatively identify these features with the aid of detailed atomic-structure calculations. In particular, we find unambiguous evidence for fivefold detachment via double $K$-hole production.

We study the phonon dynamics in lattices of optomechanical resonators where the mutually coupled photonic modes are coherently driven and the mechanical resonators are uncoupled and connected to independent thermal baths. We present a general procedure to obtain the effective Lindblad dynamics of the phononic modes for an arbitrary lattice geometry, where the light modes play the role of an effective reservoir that mediates the phonon nonequilibrium dynamics. We show how to stabilize stationary states exhibiting directional heat currents over arbitrary distance, despite the absence of thermal gradient and of direct coupling between the mechanical resonators.

The introduction of optical tweezers for trapping atoms has opened remarkable opportunities for manipulating few-body systems. Here, we present the first bottom-up assembly of atom triads. We directly observe atom loss through inelastic collisions at the single event level, overcoming the substantial challenge in many-atom experiments of distinguishing one-, two-, and three-particle processes. We measure a strong suppression of three-body loss, which is not fully explained by the presently availably theory for three-body processes. The suppression of losses could indicate the presence of local anticorrelations due to the interplay of attractive short range interactions and low dimensional confinement. Our methodology opens a promising pathway in experimental few-body dynamics.

Self-organized synchronization is a ubiquitous collective phenomenon, in which each unit adjusts their rhythms to achieve synchrony through mutual interactions. The optomechanical systems, due to their inherently engineerable nonlinearities, provide an ideal platform to study self-organized synchronization. Here, we demonstrate the self-organized synchronization of phonon lasers in a two-membrane-in-the-middle optomechanical system. The probe of each individual membrane enables us to monitor the real-time transient dynamics of synchronization, which reveals that the system enters into the synchronization regime via a torus birth bifurcation line. The phase-locking phenomenon and the transition between in-phase and antiphase regimes are directly observed. Moreover, such a system greatly facilitates the controllable synchronous states, and consequently a phononic memory is realized by tuning the system parameters. This result is an important step towards the future studies of many-body collective behaviors in multiresonator optomechanics with long distances, and might find potential applications in quantum information processing and complex networks.