- Open Access
Relativistic and recoil corrections to light-fermion vacuum polarization for bound systems of spin-0, spin-, and spin-1 particles
Phys. Rev. D 113, 056029 – Published 30 March, 2026
DOI: https://doi.org/10.1103/lll9-9wxz
Abstract
In bound systems whose constituent particles are heavier than the electron, the dominant radiative correction to energy levels is given by light-fermion (electronic) vacuum polarization. In consequence, relativistic and recoil corrections to the one-loop vacuum-polarization correction are phenomenologically relevant. Here, we generalize the treatment, previously accomplished for systems with orbiting muons, to bound systems of constituents with more general spins: spin-0, spin-, and spin-1. We discuss the application of our more general expressions to various systems of interest, including spinless systems (pionium), muonic hydrogen and deuterium, and devote special attention to the excited non- states of deuteronium, the bound system of a deuteron and its antiparticle. The obtained energy corrections are of order , where is the fine-structure constant and is the reduced mass.
Physics Subject Headings (PhySH)
Article Text
References (93)
- R. Pohl et al., The size of the proton, Nature (London) 466, 213 (2010).
- R. Pohl et al., Laser spectroscopy of muonic deuterium, Science 353, 669 (2016).
- K. Pachucki, V. Lensky, F. Hagelstein, S. S. Li Muli, S. Bacca, and R. Pohl, Comprehensive theory of the Lamb shift in light muonic atoms, Rev. Mod. Phys. 96, 015001 (2024).
- X. Kong and F. Ravndal, Relativistic corrections to the pionium lifetime, Phys. Rev. D 61, 077506 (2000).
- J. Gasser, V. E. Lyubovitskij, A. Rusetsky, and A. Gall, Decays of atom, Phys. Rev. D 64, 016008 (2001).
- U. D. Jentschura, G. Soff, and P. Indelicato, Breit Hamiltonian and quantum electrodynamic effects for spinless systems, J. Phys. B 35, 2459 (2002).
- J. Schweizer, Decay widths and energy shifts of and atoms, Phys. Lett. B 587, 33 (2004).
- J. Schweizer, Spectra and decays of and atoms, Eur. Phys. J. C 36, 483 (2004).
- J. Schweizer, Spectrum and decays of hadronic atoms, Int. J. Mod. Phys. A 20, 358 (2005).
- J. Gasser, V. E. Lyubovitskij, and A. Rusetsky, Hadronic atoms in , Phys. Rep. 456, 167 (2008).
- J. Gasser, V. E. Lyubovitskij, and A. Rusetsky, Hadronic atoms, Annu. Rev. Nucl. Part. Sci. 59, 169 (2009).
- B. Adeva et al. (DIRAC Collaboration), First measurement of the atom lifetime, Phys. Lett. B 619, 50 (2005).
- B. Adeva et al. (DIRAC Collaboration), First observation of long-lived atoms, Phys. Lett. B 751, 12 (2015).
- See the web page of the Pionic Hydrogen Collaboration at PSI, https://collaborations.fz-juelich.de/ikp/exotic-atoms/index.php.
- V. E. Lyubovitskij and A. Rusetsky, atom in ChPT: Strong energy-level shift, Phys. Lett. B 494, 9 (2000).
- P. Hauser et al. (PSI Pionic Hydrogen Collaboration), New precision measurement of the pionic deuterium -wave strong interaction parameters, Phys. Rev. C 58, R1869 (1998).
- U.-G. Meißner, U. Raha, and A. Rusetsky, The pion-nucleon scattering lengths from pionic deuterium, Eur. Phys. J. C 41, 213 (2005).
- G. Beer et al. (DEAR Collaboration), Measurement of the kaonic hydrogen X–ray spectrum, Phys. Rev. Lett. 94, 212302 (2005).
- U.-G. Meißner, U. Raha, and A. Rusetsky, Kaon–nucleon scattering lengths from kaonic deuterium experiments, Eur. Phys. J. C 47, 473 (2006).
- M. Döring and U.-G. Meißner, Kaon–nucleon scattering lengths from kaonic deuterium experiments revisited, Phys. Lett. B 704, 663 (2011).
- S. Wycech, A. M. Green, and J. A. Niskanen, On the energy levels in antiprotonic deuterium, Phys. Lett. 152B, 308 (1985).
- Y. Yan, K. Khosonthongkee, C. Kobdaj, P. Suebka, Th. Gutsche, A. Faessler, and V. E. Lyubovitskij, atoms in realistic potentials, Phys. Lett. B 659, 555 (2008).
- R. Lazauskas and J. Carbonell, Antiproton-deuteron hydrogenic states in optical models, Phys. Lett. B 820, 136573 (2021).
- P.-Y. Duerinck, R. Lazauskas, and J. Carbonell, Corrigendum to “Antiproton-deuteron hydrogenic states in optical models” [Phys. Lett. B 820, 136573 (2021)]; 841, 137936 (2023).
- P.-Y. Duerinck, R. Lazauskas, and J. Dohet-Eraly, Antiproton-deuteron hydrogenic states from a coupled-channel approach, Phys. Rev. C 108, 054003 (2023).
- G. Baptista et al., Towards precision spectroscopy of antiprotonic atoms for probing strong-field QED, Proc. Sci. EXA-LEAP2024 (2025) 085 [arXiv:2501.08893].
- C. B. Dover and J. M. Richard, Elastic, charge exchange, and inelastic cross sections in the optical model, Phys. Rev. C 21, 1466 (1980).
- C. J. Batty, Antiprotonic-hydrogen atoms, Rep. Prog. Phys. 52, 1165 (1989).
- J. Carbonell, J.-M. Richard, and S. Wycech, On the relation between protonium level shifts and nucleon–antinucleon scattering amplitudes, Z. Phys. A 343, 325 (1992).
- E. Klempt, F. Bradamante, A. Martin, and J.-M. Richard, Antinucleon–nucleon interaction at low energy: Scattering and protonium, Phys. Rep. 368, 119 (2002).
- G. S. Adkins and U. D. Jentschura, Bound deuteron–antideuteron system (deuteronium): Leading radiative and internal–structure corrections to bound-state energies, Phys. Rev. Res. 7, 043300 (2025).
- A. J. Krasznahorkay, M. Csatlós, L. Csige, Z. Gácsi, J. Gulyás, M. Hunyadi, I. Kuti, B. M. Nyakó, L. Stuhl, J. Timár, T. G. Tornyi, Zs. Vajta, T. J. Ketel, and A. Krasznahorkay, Observation of anomalous internal pair creation in : A possible indication of a light, neutral boson, Phys. Rev. Lett. 116, 042501 (2016).
- A. J. Krasznahorkay, M. Csatlós, L. Csige, J. Gulyás, M. Hunyadi, T. J. Ketel, A. Krasznahorkay, I. Kuti, Á. Nagy, B. M. Nyakó, N. Sas, J. Timár, and I. Vajda, New experimental results for the 17 MeV particle created in , Eur. Phys. J. Web Conf. 137, 08010 (2017).
- A. J. Krasznahorkay, M. Csatlós, L. Csige, J. Gulyás, T. J. Ketel, A. Krasznahorkay, I. Kuti, A. Nagy, B. M. Nyako, N. Sas, and J. Timar, On the creation of the 17 MeV X boson in the 17.6 MeV M1 transition of , Eur. Phys. J. Web Conf. 142, 01019 (2017).
- A. J. Krasznahorkay, M. Csatlós, L. Csige, J. Gulyás, M. Koszta, B. Szihalmi, J. Timár, D. S. Firak, Á. Nagy, N. J. Sas, and A. Krasznahorkay, New evidence supporting the existence of the hypothetic X17 particle, arXiv:1910.10459.
- D. S. M. Alves et al., Shedding light on X17: Community report, Eur. Phys. J. C 83, 230 (2023).
- A. J. Krasznahorkay, A. Krasznahorkay, M. Csatlós, J. Timár, M. Begala, A. Krakó, I. Rajta, I. Vajda and N. J. Sas, An update of the hypothetical X17 particle, Universe 10, 409 (2024).
- U. D. Jentschura, G. Soff, V. G. Ivanov, and S. G. Karshenboim, Bound system, Phys. Rev. A 56, 4483 (1997).
- S. G. Karshenboim, U. D. Jentschura, V. G. Ivanov, and G. Soff, Next-to-leading and higher order corrections to the decay rate of dimuonium, Phys. Lett. B 424, 397 (1998).
- I. F. Ginzburg, U. D. Jentschura, S. G. Karshenboim, F. Krauss, V. G. Serbo, and G. Soff, Production of bound systems in relativistic heavy ion collisions, Phys. Rev. C 58, 3565 (1998).
- V. W. Hughes and B. Maglic, True muonium, Bull. Am. Phys. Soc. 16, 65 (1971).
- S. J. Brodsky and R. F. Lebed, Production of the Smallest QED Atom: True Muonium (), Phys. Rev. Lett. 102, 213401 (2009).
- G. Källén and A. Sabry, Fourth order vacuum polarization, Kong. Dan. Vid. Sel. Mat. Fys. Med. 29, 1 (1955).
- J. Schwinger, Particles, Sources and Fields (Volume III) (Addison-Wesley, Reading, MA, 1989).
- J. Blomqvist, Vacuum polarization in exotic atoms, Nucl. Phys. B48, 95 (1972).
- K.-N. Huang, Calculation of the vacuum-polarization potential, Phys. Rev. A 14, 1311 (1976).
- E. Borie and G. A. Rinker, The energy levels of muonic atoms, Rev. Mod. Phys. 54, 67 (1982).
- S. Laporta and U. D. Jentschura, Dimensional regularization and two–loop vacuum polarization operator: Master integrals, analytic results and energy shifts, Phys. Rev. D 109, 096020 (2024).
- T. Kinoshita and W. B. Lindquist, Parametric formula for the sixth-order vacuum polarization contribution in quantum electrodynamics, Phys. Rev. D 27, 853 (1983).
- D. J. Broadhurst, A. L. Kataev, and O. V. Tarasov, Analytical on-shell QED results: 3-loop vacuum polarization, 4-loop -function and the muon anomaly, Phys. Lett. B 298, 445 (1993).
- P. A. Baikov and D. J. Broadhurst, Three–loop QED vacuum polarization and the four–loop muon anomalous magnetic moment, arXiv:hep-ph/9504398.
- T. Kinoshita and M. Nio, Sixth-order vacuum-polarization contribution to the Lamb shift of muonic hydrogen, Phys. Rev. Lett. 82, 3240 (1999); 103, 079901(E) (2009).
- T. Kinoshita and M. Nio, Accuracy of calculations involving vacuum-polarization diagrams: Muonic hydrogen Lamb shift and muon , Phys. Rev. D 60, 053008 (1999).
- V. G. Ivanov, E. Yu. Korzinin, and S. G. Karshenboim, Second-order corrections to the wave function at the origin in muonic hydrogen and pionium, Phys. Rev. D 80, 027702 (2009).
- A. I. Onishchenko, Three-loop photon spectral density in QED, arXiv:2212.03502v1.
- G. S. Adkins and U. D. Jentschura, Irreducible three–loop vacuum–polarization correction in muonic bound systems, Phys. Rev. D 111, 056016 (2025).
- F. Forner, C. Nega, and L. Tancredi, On the photon self-energy to three loops in QED, J. High Energy Phys. 03 (2025) 148.
- U. D. Jentschura and G. S. Adkins, Quantum Electrodynamics: Atoms, Lasers and Gravity (World Scientific, Singapore, 2022).
- K. Pachucki, Theory of the Lamb shift in muonic hydrogen, Phys. Rev. A 53, 2092 (1996).
- U. D. Jentschura, Relativistic reduced–mass and recoil corrections to vacuum polarization in muonic hydrogen, muonic deuterium and muonic helium ions, Phys. Rev. A 84, 012505 (2011).
- E. Borie, Lamb shift in light muonic atoms - revisited, arXiv:1103.1772v7.
- E. Borie, Lamb shift in light muonic atoms–Revisited, Ann. Phys. (N.Y.) 327, 733 (2012).
- A. Veitia and K. Pachucki, Nuclear recoil effects in antiprotonic and muonic atoms, Phys. Rev. A 69, 042501 (2004).
- S. G. Karshenboim, V. G. Ivanov, and E. Yu. Korzinin, Relativistic recoil corrections to the electron-vacuum-polarization contribution in light muonic atoms, Phys. Rev. A 85, 032509 (2012).
- E. Yu. Korzinin, V. G. Ivanov, and S. G. Karshenboim, contributions to the Lamb shift and the fine structure in light muonic atoms, Phys. Rev. D 88, 125019 (2013).
- S. G. Karshenboim, E. Yu. Korzinin, V. A. Shelyuto, and V. G. Ivanov, Theory of the Lamb shift in muonic tritium and the muonic ion, Phys. Rev. A 96, 022505 (2017).
- G. S. Adkins and U. D. Jentschura, Relativistic and reduced–mass corrections to vacuum polarization in muonic systems: Three–photon exchange, gauge invariance, and numerical values, Phys. Rev. A 110, 032816 (2024).
- E. A. Uehling, Polarization effects in the positron theory, Phys. Rev. 48, 55 (1935).
- G. S. Adkins and U. D. Jentschura, Bound deuteron–antideuteron system: energy corrections (to be published).
- G. S. Adkins and U. D. Jentschura, Short–range hard–sphere potential and Coulomb interaction: Deser–Trueman formula for Rydberg states of exotic atomic systems, Atoms 13, 081 (2025).
- J. Zatorski and K. Pachucki, Electrodynamics of finite-size particles with arbitrary spin, Phys. Rev. A 82, 052520 (2010).
- J. Zatorski, V. Patkóš, and K. Pachucki, Quantum electrodynamics of two-body systems with arbitrary masses up to order, Phys. Rev. A 106, 042804 (2022).
- P. J. Mohr, D. B. Newell, B. N. Taylor, and E. Tiesinga, CODATA recommended values of the fundamental physical constants: 2022, Rev. Mod. Phys. 97, 025002 (2025).
- K. Pachucki and S. G. Karshenboim, Nuclear-spin-dependent recoil correction to the Lamb shift, J. Phys. B 28, L221 (1995).
- U. D. Jentschura, Proton radius, Darwin-Foldy term and radiative corrections, Eur. Phys. J. D 61, 7 (2011).
- X. Gao, N. Karthik, S. Mukherjee, P. Petreczky, S. Syritsyn, and Y. Zhao, Pion form factor and charge radius from lattice QCD at the physical point, Phys. Rev. D 104, 114515 (2021).
- Z.-F. Cui, D. Binosi, C. D. Roberts, and S. M. Schmidt, Pion charge radius from elastic scattering data, Phys. Lett. B 822, 136631 (2021).
- S. Navas et al. (Particle Data Group), Review of particle physics, Phys. Rev. D 110, 030001 (2024).
- E. Borie, Lamb shift in light muonic atoms - revisited, arXiv:1103.1772v5.
- V. Patkóš and K. Pachucki, Antiprotonic atoms with nonperturbative inclusion of vacuum polarization and finite nuclear mass, Phys. Rev. A 112, 052808 (2025).
- A. P. Martynenko, 2S Hyperfine splitting of muonic hydrogen, Phys. Rev. A 71, 022506 (2005).
- J. M. B. Kellogg, I. I. Rabi, N. F. Ramsey, Jr., and J. R. Zacharias, An electrical quadrupole moment of the deuteron, Phys. Rev. 55, 318 (1939).
- J. M. B. Kellogg, I. I. Rabi, N. F. Ramsey, Jr., and J. R. Zacharias, An Electrical Quadrupole Moment of the Deuteron: The Radiofrequency Spectra of HD and Molecules in a Magnetic Field, Phys. Rev. 57, 677 (1940).
- M. Puchalski, J. Komasa, and K. Pachucki, Hyperfine structure of the first rotational level in , and molecules and the deuteron quadrupole moment, Phys. Rev. Lett. 125, 253001 (2020).
- A. A. Krutov and A. P. Martynenko, Lamb shift in the muonic deuterium atom, Phys. Rev. A 84, 052514 (2011).
- K. Pachucki, Nuclear structure corrections in muonic deuterium, Phys. Rev. Lett. 106, 193007 (2011).
- M. Kalinowski, K. Pachucki, and V. A. Yerokhin, Nuclear-structure corrections to the hyperfine splitting in muonic deuterium, Phys. Rev. A 98, 062513 (2018).
- R. N. Faustov, A. P. Martynenko, G. A. Martynenko, and V. V. Sorokin, Hyperfine structure of states in muonic deuterium, Phys. Rev. A 90, 012520 (2014).
- R. N. Faustov, A. P. Martynenko, G. A. Martynenko, and V. V. Sorokin, Hyperfine structure of states in muonic deuterium, Phys. Rev. A 92, 052512 (2015).
- C. Ji, X. Zhang, and L. Platter, Nuclear structure effects on hyperfine splittings in ordinary and muonic deuterium, Phys. Rev. Lett. 133, 042502 (2024).
- J. J. Krauth, M. Diepold, B. Franke, A. Antognini, F. Kottmann, and R. Pohl, Theory of the levels in muonic deuterium, Ann. Phys. (N.Y.) 366, 168 (2016).
- R. J. Hill, G. Lee, G. Paz, and M. P. Solon, NRQED Lagrangian at order , Phys. Rev. D 87, 053017 (2013).
- G. S. Adkins, Three-dimensional Fourier transforms, integrals of spherical Bessel functions, and novel delta function identities, Bull. Allahabad Math. Soc. 31, 215 (2016).