Design and validation of a fission-product source for radioactive beams
J. Song, G. Savard, J. Greene, and J. A. Nolen
Phys. Rev. C 109, 024605 (2024) - Published 12 February, 2024
A neutron-generator-based source of fission products (nuCARIBU) is being developed to replace the existing source at Argonne National Laboratory. Neutrons generated by reaction are thermalized in a compact polyethylene [( moderator and impinge on a thin foil to produce fission products. Experiments have been conducted to verify the nuCARIBU concept and simulation results using a 4 MeV, proton beam from the ATLAS accelerator irradiating a LiF neutron production target and two different simplified versions of the nuCARIBU ( moderator with thicknesses of 3.81 cm and 1.91 cm separating it from the enriched fission foil. The emitted -ray peaks of 1383.93 keV (), 358.0 keV (), 565.992 keV (), and 258.411 keV () obtained from fission products are used to determine the neutron-induced fission rates in the fission foil. The measured fission rates are in good agreement with those simulated using the PHITS Monte Carlo code with user-defined neutron production cross sections based on well-known cross section data. These experimental results, consistent with the simulations, show that the current source (CARIBU) can be replaced by the neutron induced fission source (nuCARIBU).