We consider the spectral statistics of the Floquet operator for disordered, periodically driven spin chains in their quantum chaotic and many-body localized (MBL) phases. The spectral statistics are characterized by the traces of powers $t$ of the Floquet operator, and our approach hinges on the fact that for integer $t$ in systems with local interactions, these traces can be re-expressed in terms of products of dual transfer matrices, each representing a spatial slice of the system. We focus on properties of the dual transfer matrix products as represented by a spectrum of Lyapunov exponents, which we call spectral Lyapunov exponents. In particular, we examine the features of this spectrum that distinguish chaotic and MBL phases. The transfer matrices can be block diagonalized using time-translation symmetry, and so the spectral Lyapunov exponents are classified according to a momentum in the time direction. For large $t$ we argue that the leading Lyapunov exponents in each momentum sector tend to zero in the chaotic phase, while they remain finite in the MBL phase. These conclusions are based on results from three complementary types of calculation. We find exact results for the chaotic phase by considering a Floquet random quantum circuit with on-site Hilbert space dimension $q$ in the large-$q$ limit. In the MBL phase, we show that the spectral Lyapunov exponents remain finite by systematically analyzing models of noninteracting systems, weakly coupled systems, and local integrals of motion. Numerically, we compute the Lyapunov exponents for a Floquet random quantum circuit and for the kicked Ising model in the two phases. As an additional result, we calculate exactly the higher-point spectral form factors (hpSFFs) in the large-$q$ limit and show that the generalized Thouless time scales logarithmically in system size for all hpSFFs in the large-$q$ chaotic phase.

Spin torques are at the heart of spin manipulations in spintronic devices. Here, we examine the existence of an optical spin-orbit torque, a relativistic spin torque originating from the spin-orbit coupling of an oscillating applied field with the spins. We compare the effect of the nonrelativistic Zeeman torque with the relativistic optical spin-orbit torque for ferromagnetic systems excited by a circularly polarized laser pulse. The latter torque depends on the helicity of the light and scales with the intensity, while being inversely proportional to the frequency. Our results show that the optical spin-orbit torque can provide a torque on the spins, which is quantitatively equivalent to the Zeeman torque. Moreover, temperature-dependent calculations show that the effect of optical spin-orbit torque decreases with increasing temperature. However, the effect does not vanish in a ferromagnetic system, even above its Curie temperature.

Novel designs of Josephson weak links based on semiconducting nanowires combined with circuit QED techniques have enabled the resolution of their fine structure due to spin-orbit interactions, opening a path towards Andreev spin qubits. Nevertheless, direct manipulation of the spin within a given Andreev state is in general suppressed compared to interdoublet manipulation in the absence of Zeeman effects. In addition, noisy spin-flip mechanisms limit any coherent manipulation protocol to spin postselection. We propose a combination of a spin polarization protocol analogous to sideband cooling with stimulated Raman adiabatic passage specifically tailored for these systems. We show this approach is robust for a large range of design parameters, including the currently rather stringent coherence times.

Dynamical multiferroicity features entangled dynamic orders: fluctuating electric dipoles induce magnetization. Hence, the material with paraelectric fluctuations can develop magnetic signatures if dynamically driven. We identify the paraelectric ${\mathrm{KTaO}}_3$ (KTO) as a prime candidate for the observation of the dynamical multiferroicity. We show that when a KTO sample is exposed to a circularly polarized laser pulse, the dynamically induced ionic magnetic moments are of the order of 5% of the nuclear magneton per unit cell. We determine the phonon spectrum using ab initio methods, and we identify $T_{1u}$ as relevant phonon modes that couple to the external field and induce magnetic polarization. We also predict a corresponding electron effect for the dynamically induced magnetic moment, which is enhanced by several orders of magnitude due to the significant mass difference between electron and ionic nucleus.

A muonium hydride molecule is a bound state of muonium and hydrogen atoms. It has half the mass of a parahydrogen molecule and very similar electronic properties in its ground state. The phase diagram of an assembly of such particles is investigated by first-principles quantum simulations. In the bulk limit, the low-temperature equilibrium phase is a crystal of extraordinarily low density, lower than that of any other known atomic or molecular crystal. Despite the low density and particle mass, the melting temperature is surprisingly high (close to 9 K). No (metastable) supersolid phase is observed. We investigated the physical properties of nanoscale clusters (up to 200 particles) of muonium hydride and found the superfluid response to be greatly enhanced compared to that of parahydrogen clusters. The possible experimental realization of these systems is discussed.

The collective modes of a quantum liquid shape and impact its properties profoundly, including its emergent phenomena such as superfluidity. Here we present how a two-dimensional Bose gas responds to a moving lattice potential. In particular, we discuss how the induced heating rate depends on the interaction strength and the temperature. This study is motivated by the recent measurements of Sobirey et al. [arXiv:2005.07607], for which we provide a satisfying understanding. Going beyond the existing measurements, we demonstrate that this probing method allows us to identify two sound modes in quantum liquids. We show that the two sound modes undergo hybridization as a function of interaction strength, which we propose to detect experimentally. This gives insight into the two regimes of Bose gases, defined via the hierarchy of sound modes.

Chiral matter has a structure that lacks inversion, mirror, and rotoreflection symmetry; thus, a given chiral material has either a right- or left-handed structure. In chiral matter, electricity and magnetism can be coupled in an exotic manner beyond the classical electromagnetism (e.g., magneto chiral effect in chiral magnets). In this paper, we give a firm experimental proof of the linear electric-current-induced magnetization effect in bulk nonmagnetic chiral matter elemental trigonal tellurium. We measured a ${}^{125}\mathrm{Te}$ nuclear magnetic resonance (NMR) spectral shift under a pulsed electric current for trigonal tellurium single crystals. We provide general symmetry considerations to discuss the electrically (electric-field- and electric-current-) induced magnetization and clarify that the NMR shift observed in trigonal tellurium is caused by the linear current-induced magnetization effect, not by a higher-order magnetoelectric effect. We also show that the current-induced NMR shift is reversed by a chirality reversal of the tellurium crystal structure. This result is direct evidence of crystal-chirality-induced spin polarization, which is an inorganic-bulk-crystal analog of the chirality-induced spin selectivity in chiral organic molecules. The present findings also show that nonmagnetic chiral crystals may be applied to spintronics and coil-free devices to generate magnetization beyond the classical electromagnetism.

We study a planar Josephson junction under an applied DC voltage bias in the presence of an in-plane magnetic field. Upon tuning the bias voltage across the junction $V_{\mathrm{J}}$, the two ends of the junction are shown to simultaneously host both zero and $\pi$ Majorana modes. These modes can be probed using either a scanning-tunneling-microscopy measurement or through resonant Andreev tunneling from a lead coupled to the junction. While these modes are mostly bound to the junction's ends, they can hybridize with the bulk by absorbing or emitting photons. We analyze this process both numerically and analytically, demonstrating that it can become negligible under typical experimental conditions. Transport signatures of the zero and $\pi$ Majorana states are shown to be robust to moderate disorder.

Quantum vortices in superfluids have been an important research area for many decades. Naturally, research on this topic has focused on two-dimensional (2D) and 3D superfluids, in which vortex cores form points and lines, respectively. Very recently, however, there has been growing interest in the quantum simulation of systems with four spatial dimensions; this raises the question of how vortices would behave in a higher-dimensional superfluid. In this paper, we begin to establish the phenomenology of vortices in 4D superfluids under rotation, where the vortex core can form a plane. In 4D, the most generic type of rotation is a “double rotation” with two angles (or frequencies). We show, by solving the Gross-Pitaevskii equation, that the simplest case of equal-frequency double rotation can stabilize a pair of vortex planes intersecting at a point. This opens up a wide number of future research topics, including into realistic experimental models; unequal-frequency double rotations; the stability and potential reconnection dynamics of intersecting vortex surfaces; and the possibility of closed vortex surfaces.

Coupling a system to a nonthermal environment can profoundly affect the phase diagram of the closed system, giving rise to a special class of dissipation-induced phase transitions. Such transitions take the system out of its ground state and stabilize a higher-energy stationary state, rendering it the sole attractor of the dissipative dynamics. In this paper, we present a unifying methodology, which we use to characterize this ubiquitous phenomenology and its implications for the open system dynamics. Specifically, we analyze the closed system's phase diagram, including symmetry-broken phases, and explore their corresponding excitations' spectra. Opening the system, the environment can overwhelm the system's symmetry-breaking tendencies, and changes its order parameter. As a result, isolated distinct phases of similar order become connected, and new phase-costability regions appear. Interestingly, the excitations differ in the newly connected regions through a change in their symplectic norm, which is robust to the introduction of dissipation. As a result, by tuning the system from one phase to the other across the dissipation-stabilized region, the open system fluctuations exhibit an exceptional pointlike scenario, where the fluctuations become overdamped, only to reappear with an opposite sign in the dynamical response function of the system. The overdamped region is also associated with squeezing of the fluctuations. We demonstrate the pervasive nature of such dissipation-induced phenomena in two prominent examples, namely, in parametric resonators and in light-matter systems. Our work draws a crucial distinction between quantum phase transitions and their zero-temperature open system counterparts.

Spins of relativistic fermions are related to their orbital degrees of freedom. In order to quantify the effect of hybridization between relativistic and nonrelativistic degrees of freedom on spin-orbit coupling, we focus on the spin-orbital (SO) crossed susceptibility arising from spin-orbit coupling. The SO crossed susceptibility is defined as the response function of their spin polarization to the “orbital” magnetic field, namely, the effect of magnetic field on the orbital motion of particles as the vector potential. Once relativistic and nonrelativistic fermions are hybridized, their SO crossed susceptibility gets modified at the Fermi energy around the band hybridization point, leading to spin polarization of nonrelativistic fermions as well. These effects are enhanced under a dynamical magnetic field that violates thermal equilibrium, arising from the interband process permitted by the band hybridization. Its experimental realization is discussed for Dirac electrons in solids with slight breaking of crystalline symmetry or doping, and also for quark matter including dilute heavy quarks strongly hybridized with light quarks, arising in a relativistic heavy-ion collision process.

Magnetization switching using in-plane charge current recently has been widely investigated in heavy metal/ferromagnet bilayers with the switching mechanism usually attributed to the action of the spin-orbit coupling. Here we study in-plane current induced magnetization switching in model epitaxial bilayers that consist of Au(001) and Fe(001) grown on MgO(001). We use the planar Hall effect combined with magnetooptical Kerr effect (MOKE) microscopy to investigate magnetic properties of the bilayers and current-induced switching. We show that a current density beyond $1.4\times {10}^7$ A/cm can be employed for reproducible electrical switching of the magnetization between multiple stable states that correspond to different arrangements of magnetic domains with magnetization direction along one of the in-plane easy magnetization axes of the Fe(001) film. Lower current densities result in stable intermediate transversal resistances which are interpreted based on MOKE-microscopy investigations as resulting from the current-induced magnetic domain structure that is formed in the area of the Hall cross. We find that the physical mechanism of the current-induced magnetization switching of the Au/Fe/MgO(001) system at room temperature can be fully explained by the Oersted field, which is generated by the charge current flowing mostly through the Au layer.

A Schrödinger-cat state is a coherent superposition of macroscopically distinguishable quantum states, in quantum optics usually realized as superposition of coherent states. Protocols to prepare photonic cats have been presented for atomic systems. Here we investigate in what manner and how well the preparation protocols can be transferred to a solid-state platform, namely, a semiconductor quantum-dot–cavity system. In quantum-dot–cavity systems there are many disruptive influences like cavity losses, the radiative decay of the quantum dot, and the coupling to longitudinal acoustic phonons. We show that for one of the protocols these influences kill the quantum coherence between the states forming the cat, while for a second protocol a parameter regime can be identified where the essential characteristics of Schrödinger-cat states survive the environmental influences under conditions that can be realized with current equipment.

While the symmetry-based diagnosis of topological insulators and semimetals has enabled large-scale discovery of topological materials candidates, the extension of these approaches to the diagnosis of topological superconductors remains a major open question. One important new ingredient in the analysis of topological superconductivity is the presence of ${\mathbb{Z}}_2$-valued Pfaffian invariants associated with certain high-symmetry momenta. Such topological invariants lie beyond the conventional scope of symmetry representation theory for band structures, and as such they are nontrivial to incorporate into the systematic calculations of the symmetry indicators of band topology. Here, we overcome this challenge and report the full computation of the ${\mathbb{Z}}_2$-enriched symmetry indicators for superconductors in all symmetry settings. Our results indicate that incorporating the ${\mathbb{Z}}_2$ band labels enhance the diagnostic power of the scheme in roughly $60\%$ of the symmetry settings. Our framework can also be readily integrated with first-principles calculations to elucidate on the possible properties of unconventional superconductivity in a given compound. As a demonstration, we analyze explicitly the interplay between pairing symmetry and topological superconductivity in the recently discovered superconductors CaPtAs and ${\mathrm{CaSb}}_2$.

We report magneto-optical spectroscopy of gated monolayer ${\mathrm{MoS}}_2$ in high magnetic fields up to $28\mathrm{T}$ and obtain new insights on the many-body interaction of neutral and charged excitons with the resident charges of distinct spin and valley texture. For neutral excitons at low electron doping, we observe a nonlinear valley Zeeman shift due to dipolar spin-interactions that depends sensitively on the local carrier concentration. As the Fermi energy increases to dominate over the other relevant energy scales in the system, the magneto-optical response depends on the occupation of the fully spin-polarized Landau levels (LL) in both $K/K^{\prime }$ valleys. This manifests itself in a many-body state. Our experiments demonstrate that the exciton in monolayer semiconductors is only a single particle boson close to charge neutrality. We find that away from charge neutrality it smoothly transitions into polaronic states with a distinct spin-valley flavor that is defined by the LL quantized spin and valley texture.

Low-energy transport in quantum Hall states is carried through edge modes and is dictated by bulk topological invariants and possibly microscopic Boltzmann kinetics at the edge. Here, we show how the presence or breaking of symmetries of the edge Hamiltonian underlie transport properties, specifically dc conductance and noise. We demonstrate this through the analysis of hole-conjugate states of the quantum Hall effect, specifically the $\nu =2/3$ case in a quantum point-contact geometry. We identify two symmetries, a continuous SU(3) symmetry and a discrete $Z_3$ symmetry, whose presence or absence (different symmetry scenarios) dictate qualitatively different types of behavior of conductance and shot noise. While recent measurements are consistent with one of these symmetry scenarios, others can be realized in future experiments.

Recent years have seen a revived interest in the diagrammatic Monte Carlo (DiagMC) methods for interacting fermions on a lattice. A promising recent development allows one to now circumvent the analytical continuation of dynamic observables in DiagMC calculations within the Matsubara formalism. This is made possible by symbolic algebra algorithms, which can be used to analytically solve the internal Matsubara frequency summations of Feynman diagrams. In this paper, we take a different approach and show that it yields improved results. We present a closed-form analytical solution of imaginary-time integrals that appear in the time-domain formulation of Feynman diagrams. We implement and test a DiagMC algorithm based on this analytical solution and show that it has numerous significant advantages. Most importantly, the algorithm is general enough for any kind of single-time correlation function series, involving any single-particle vertex insertions. Therefore, it readily allows for the use of action-shifted schemes, aimed at improving the convergence properties of the series. By performing a frequency-resolved action-shift tuning, we are able to further improve the method and converge the self-energy in a nontrivial regime, with only 3–4 perturbation orders. Finally, we identify time integrals of the same general form in many commonly used Monte Carlo algorithms and therefore expect a broader usage of our analytical solution.

Although stoquastic Hamiltonians are known to be simulable via sign-problem-free quantum Monte Carlo (QMC) techniques, the nonstoquasticity of a Hamiltonian does not necessarily imply the existence of a QMC sign problem. We give a sufficient and necessary condition for the QMC-simulability of Hamiltonians in a given basis: We prove that a QMC simulation will be sign-problem-free if and only if all the overall total phases along the chordless cycles of the weighted graph whose adjacency matrix is the Hamiltonian are zero (modulo $2\pi$). We use our findings to provide a construction for nonstoquastic, yet sign-problem-free and hence QMC-simulable, quantum many-body models. We also demonstrate why the simulation of truly sign-problematic models using the QMC weights of the stoquasticized Hamiltonian is generally suboptimal. We offer a superior alternative.

The concept of Fermi liquid lays a solid cornerstone to the understanding of electronic correlations in quantum matter. This ordered many-body state rigorously organizes electrons at zero temperature in progressively higher momentum states, up to the Fermi surface. As such, it displays rigidity against perturbations. Such rigidity generates Fermi-surface resonances which manifest as longitudinal and transverse collective modes. Although these Fermi-liquid collective modes have been analyzed and observed in electrically neutral liquid helium, they remain unexplored in charged solid-state systems up to date. In this paper I analyze the transverse shear response of charged three-dimensional Fermi liquids as a function of temperature, excitation frequency and momentum, for interactions expressed in terms of the first symmetric Landau parameter. I consider the effect of momentum-conserving quasiparticle collisions and momentum-relaxing scattering in relaxation-time approximation on the coupling between photons and Fermi-surface collective modes, thus deriving the Fermi-liquid optical conductivity and dielectric function. In the high-frequency, long-wavelength excitation regime the electrodynamic response entails two coherent and frequency-degenerate polaritons, and its spatial nonlocality is encoded by a frequency- and interaction-dependent generalized shear modulus; in the opposite high-momentum low-frequency regime anomalous skin effect takes place. I identify observable signatures of propagating shear collective modes in optical spectroscopy experiments, with applications to the surface impedance and the optical transmission of thin films.

Despite many efforts to rationalize the strongly correlated electronic ground states in doped Mott insulators, the nature of the doping-induced insulator-to-metal transition is still a subject under intensive investigation. Here, we probe the nanoscale electronic structure of the Mott insulator ${\mathrm{Sr}}_2{\mathrm{IrO}}_{4-\delta }$ with low-temperature scanning tunneling microscopy and find an enhanced local density of states (LDOS) inside the Mott gap at the location of individual defects which we interpret as defects at apical oxygen sites. A chiral behavior in the topography for those defects has been observed. We also visualize the local enhanced conductance arising from the overlapping of defect states which induces finite LDOS inside of the Mott gap. By combining these findings with the typical spatial extension of isolated defects of about 2 nm, our results indicate that the insulator-to-metal transition in ${\mathrm{Sr}}_2{\mathrm{IrO}}_{4-\delta }$ could be percolative in nature.