Field-induced up-up-down state and frustrated magnetism in a non-Kramers triangular antiferromagnet
Phys. Rev. Materials 10, 114403 – Published 4 November, 2026
DOI: https://doi.org/10.1103/z7n3-7s89
Abstract
A previously unreported triangular lattice (TL) antiferromagnet, , was synthesized as single crystals, and its crystal structure, magnetic susceptibilities, and specific heat were reported. Its crystal structure is isomorphic to that of the transverse-field Ising antiferromagnet , with ions located in the TLs, separated by a nonmagnetic bilayer composed mainly of and ions. The magnetic susceptibilities indicate the dominating antiferromagnetic interactions. The magnetization curves () exhibit strong easy--axis anisotropy, with a clear one-third magnetic plateau emerging, consistent with a field-induced up-up-down spin configuration. Instead of forming a conventional long-range magnetic order, the system exhibits two broad humps at 0.11 K and 2.81 K in zero-field specific heat measurements, revealing dominant strong spin fluctuations and pointing to potential relevance to Berezinskii-Kosterlitz-Thouless physics. The above results reveal its future interest in exploring exotic quantum spin states in .