Characterizing nonlocal magnetic fluctuations in materials with strong electronic Coulomb interactions remains one of the major outstanding challenges of modern condensed matter theory. In this Letter, we address the spatial symmetry and orbital structure of magnetic fluctuations in perovskite materials. To this aim, we develop a consistent multiorbital diagrammatic extension of dynamical mean-field theory, which we apply to an anisotropic three-orbital model of cubic $t_{2g}$ symmetry. We find that the form of spatial spin fluctuations is governed by the local Hund’s coupling. For small values of the coupling, magnetic fluctuations are anisotropic in orbital space, which reflects the symmetry of the considered $t_{2g}$ model. Large Hund’s coupling enhances collective spin excitations, which mixes orbital and spatial degrees of freedom, and magnetic fluctuations become orbitally isotropic. Remarkably, this effect can be seen only in two-particle quantities; single-particle observables remain anisotropic for any value of the Hund’s coupling. Importantly, we find that the orbital isotropy can be induced both at half filling and for the case of four electrons per lattice site, where the magnetic instability is associated with different, antiferromagnetic and ferromagnetic, modes, respectively.

We report the observation of the unidirectional spin Hall magnetoresistance (USMR), which depends on the current or magnetization direction, in heavy-metal–ferromagnetic-insulator bilayer, $\mathrm{Pt}\text{−}{\mathrm{Y}}_3{\mathrm{Fe}}_5{\mathrm{O}}_{12}$ (YIG). This USMR is apparently not caused by the mechanisms established in metallic bilayer, in which the ferromagnetic layer is required to be electrically conductive. From the magnetic field, current, temperature, and YIG thickness dependent measurements, the USMR is attributed to the asymmetric magnon creation and annihilation induced by the spin-orbit torque. This asymmetry and the resultant USMR are further revealed by the micromagnetic simulations combined with the spin-orbit torque and the spin drift-diffusion model. Our finding exhibits a nonlinear manipulation of magnons with the charge current.

The short timescale spin dynamics in antiferromagnets is an attractive feature from the standpoint of ultrafast spintronics. Yet generating highly polarized spin current at room temperature remains a fundamental challenge for antiferromagnets. We propose a spin circular photogalvanic effect (spin CPGE), in which circularly polarized light can produce a highly spin-polarized current at room temperature, through an “injection-current-like” mechanism in parity-time ($PT$)-symmetric antiferromagnetic (AFM) insulators. We demonstrate this effect by first-principles simulations of bilayer ${\mathrm{CrI}}_3$ and room-temperature-AFM hematite. The spin CPGE is significant, and the magnitude of spin photocurrent is comparable with the widely observed charge photocurrent in ferroelectric materials. Interestingly, this spin photocurrent is not sensitive to spin-orbit interactions, which were regarded as fundamental mechanisms for generating spin current. Given the fast response of light-matter interactions, large energy scale, and insensitivity to spin-orbit interactions, our work gives hope to realizing fast-dynamic and temperature-robust pure spin current in a wide range of $PT$-symmetric AFM materials, including topological axion insulators and weak-relativistic magnetic insulators.

We examine the stochastic dynamics of two enzymes that are mechanically coupled to each other, e.g., through an elastic substrate or a fluid medium. The enzymes undergo conformational changes during their catalytic cycle, which itself is driven by stochastic steps along a biased chemical free energy landscape. We find conditions under which the enzymes can synchronize their catalytic steps, and discover that the coupling can lead to a significant enhancement in their overall catalytic rate. Both effects can be understood as arising from a global bifurcation in the underlying dynamical system at sufficiently strong coupling. Our findings suggest that, despite their molecular scale, enzymes can be cooperative and improve their performance in metabolic clusters.

We show that combining randomized measurement protocols with importance sampling allows for characterizing entanglement in significantly larger quantum systems and in a more efficient way than in previous work. A drastic reduction of statistical errors is obtained using classical techniques of machine learning and tensor networks using partial information on the quantum state. In current experimental settings of engineered many-body quantum systems this significantly increases the (sub-)system sizes for which entanglement can be measured. In particular, we show an exponential reduction of the required number of measurements to estimate the purity of product states and GHZ states.

Quantum critical behavior of many-body phase transitions is one of the most fascinating yet challenging questions in quantum physics. Here, we improved the band-mapping method to investigate the quantum phase transition from superfluid to Mott insulators, and we observed the critical behaviors of quantum phase transitions in both the dynamical steady-state-relaxation region and the phase-oscillation region. Based on various observables, two different values for the same quantum critical parameter are observed. This result is beyond a universal-scaling-law description of quantum phase transitions known as the Kibble-Zurek mechanism, and suggests that multiple quantum critical mechanisms are competing in many-body quantum phase transition experiments in inhomogeneous systems.

Theoretical treatments of periodically driven quantum thermal machines (PD-QTMs) are largely focused on the limit-cycle stage of operation characterized by a periodic state of the system. Yet, this regime is not immediately accessible for experimental verification. Here, we present a general thermodynamic framework that handles the performance of PD-QTMs both before and during the limit-cycle stage of operation. It is achieved by observing that periodicity may break down at the ensemble average level, even in the limit-cycle phase. With this observation, and using conventional thermodynamic expressions for work and heat, we find that a complete description of the first law of thermodynamics for PD-QTMs requires a new contribution, which vanishes only in the limit-cycle phase under rather weak system-bath couplings. Significantly, this contribution is substantial at strong couplings even at limit cycle, thus largely affecting the behavior of the thermodynamic efficiency. We demonstrate our framework by simulating a quantum Otto engine building upon a driven resonant level model. Our results provide new insights towards a complete description of PD-QTMs, from turn-on to the limit-cycle stage and, particularly, shed light on the development of quantum thermodynamics at strong coupling.

This Letter reports results from the first long-baseline search for sterile antineutrinos mixing in an accelerator-based antineutrino-dominated beam. The rate of neutral-current interactions in the two NOvA detectors, at distances of 1 and 810 km from the beam source, is analyzed using an exposure of $12.51\times {10}^{20}$ protons-on-target from the NuMI beam at Fermilab running in antineutrino mode. A total of 121 of neutral-current candidates are observed at the far detector, compared to a prediction of $122\pm 11(\mathrm{stat}.)\pm 15(\mathrm{syst}.)$ assuming mixing only between three active flavors. No evidence for ${\overline{\nu }}_{\mu }\to {\overline{\nu }}_s$ oscillation is observed. Interpreting this result within a $3+1$ model, constraints are placed on the mixing angles ${\theta }_{24}<25°$ and ${\theta }_{34}<32°$ at the 90% C.L. for $0.05{\mathrm{eV}}^2\le \mathrm{\Delta }{m}_{41}^2\le 0.5{\mathrm{eV}}^2$, the range of mass splittings that produces no significant oscillations at the near detector. These are the first $3+1$ confidence limits set using long-baseline accelerator antineutrinos.

We study the fragmentation of ${\mathrm{He}}_2$ dimers into ${\mathrm{He}}^{+}$ ions by relativistic highly charged projectiles. We demonstrate that the interaction between an ultrafast projectile with an extremely extended object—the helium dimer—possesses interesting features that are absent in collisions with “normal” molecules. We also show that such projectiles, due to their enormous interaction range, can accurately probe the ground state of the dimer and even be used for a determination of its binding energy.

We show that some tripartite quantum correlations are inexplicable by any causal theory involving bipartite nonclassical common causes and unlimited shared randomness. This constitutes a device-independent proof that nature’s nonlocality is fundamentally at least tripartite in every conceivable physical theory—no matter how exotic. To formalize this claim, we are compelled to substitute Svetlichny’s historical definition of genuine tripartite nonlocality with a novel theory-agnostic definition tied to the framework of local operations and shared randomness. A companion article by Coiteux-Roy et al. generalizes these concepts to any $N\ge 3$ number of parties, providing experimentally amenable device-independent inequality constraints along with quantum correlations violating them, thereby certifying that nature’s nonlocality must be boundlessly multipartite.

The Bose polaron has attracted theoretical and experimental interest because the mobile impurity is surrounded by a bath that undergoes a superfluid-to-normal phase transition. Although many theoretical works have studied this system in its ground state, only a few analyze its behavior at finite temperature. We have studied the effect of temperature on a Bose polaron system performing ab initio path integral Monte Carlo simulations. This method is able to approach the critical temperature without losing accuracy, in contrast with perturbative approximations. We have calculated the polaron energy for the repulsive and attractive branches and we have observed an asymmetric behavior between the two branches. When the potential is repulsive, the polaron energy decreases when the temperature increases, and contrariwise for the attractive branch. Our results for the effective mass and the dynamical structure factor of the polaron show unambiguously that its quasiparticle nature disappears close to the critical temperature, in agreement with recent experimental findings. Finally, we have also estimated the fraction of bosons in the condensate as well as the superfluid fraction, and we have concluded that the impurity hinders the condensation of the rest of bosons.

Rapid solidification experiments on thin film aluminum samples reveal the presence of lattice orientation gradients within crystallizing grains. To study this phenomenon, a single-component phase-field crystal (PFC) model that captures the properties of solid, liquid, and vapor phases is proposed to model pure aluminium quantitatively. A coarse-grained amplitude representation of this model is used to simulate solidification in samples approaching micrometer scales. The simulations reproduce the experimentally observed orientation gradients within crystallizing grains when grown at experimentally relevant rapid quenches. We propose a causal connection between defect formation and orientation gradients.

At the interface between a ferromagnetic insulator and a superconductor there is a coupling between the spins of the two materials. We show that when a supercurrent carried by triplet Cooper pairs flows through the superconductor, the coupling induces a magnon spin current in the adjacent ferromagnetic insulator. The effect is dominated by Cooper pairs polarized in the same direction as the ferromagnetic insulator, so that charge and spin supercurrents produce similar results. Our findings demonstrate a way of converting Cooper pair supercurrents to magnon spin currents.

Generating high-fidelity, tunable entanglement between qubits is crucial for realizing gate-based quantum computation. In superconducting circuits, tunable interactions are often implemented using flux-tunable qubits or coupling elements, adding control complexity and noise sources. Here, we realize a tunable $ZZ$ interaction between two transmon qubits with fixed frequencies and fixed coupling, induced by driving both transmons off resonantly. We show tunable coupling over 1 order of magnitude larger than the static coupling, and change the sign of the interaction, enabling cancellation of the idle coupling. Further, this interaction is amenable to large quantum processors: the drive frequency can be flexibly chosen to avoid spurious transitions, and because both transmons are driven, it is resilient to microwave cross talk. We apply this interaction to implement a controlled phase (CZ) gate with a gate fidelity of 99.43(1)% as measured by cycle benchmarking, and we find the fidelity is limited by incoherent errors.

The prompt production of the charm baryon ${\mathrm{\Lambda }}_c^{+}$ and the ${\mathrm{\Lambda }}_c^{+}/D^0$ production ratios were measured at midrapidity with the ALICE detector in $pp$ and $p$-Pb collisions at $\sqrt{s_{\mathrm{NN}}}=5.02\mathrm{TeV}$. These new measurements show a clear decrease of the ${\mathrm{\Lambda }}_c^{+}/D^0$ ratio with increasing transverse momentum ($p_T$) in both collision systems in the range $2<p_T<12\mathrm{GeV}/c$, exhibiting similarities with the light-flavor baryon-to-meson ratios $p/\pi$ and $\mathrm{\Lambda }/K_S^0$. At low $p_T$, predictions that include additional color-reconnection mechanisms beyond the leading-color approximation, assume the existence of additional higher-mass charm-baryon states, or include hadronization via coalescence can describe the data, while predictions driven by charm-quark fragmentation processes measured in $e^{+}{e}^{-}$ and $e^{-}p$ collisions significantly underestimate the data. The results presented in this Letter provide significant evidence that the established assumption of universality (colliding-system independence) of parton-to-hadron fragmentation is not sufficient to describe charm-baryon production in hadronic collisions at LHC energies.

A crucial subroutine for various quantum computing and communication algorithms is to efficiently extract different classical properties of quantum states. In a notable recent theoretical work by Huang, Kueng, and Preskill [Nat. Phys. 16, 1050 (2020)], a thrifty scheme showed how to project the quantum state into classical shadows and simultaneously predict $M$ different functions of a state with only $\mathcal{O}({\log }_{2}M)$ measurements, independent of the system size and saturating the information-theoretical limit. Here, we experimentally explore the feasibility of the scheme in the realistic scenario with a finite number of measurements and noisy operations. We prepare a four-qubit GHZ state and show how to estimate expectation values of multiple observables and Hamiltonians. We compare the measurement strategies with uniform, biased, and derandomized classical shadows to conventional ones that sequentially measure each state function exploiting either importance sampling or observable grouping. We next demonstrate the estimation of nonlinear functions using classical shadows and analyze the entanglement of the prepared quantum state. Our experiment verifies the efficacy of exploiting (derandomized) classical shadows and sheds light on efficient quantum computing with noisy intermediate-scale quantum hardware.