Power broadening—the broadening of the spectral line profile of a two-state quantum transition as the amplitude of the driving field increases—is a well-known and thoroughly examined phenomenon in spectroscopy. It typically occurs in continuous-wave driving when the intensity of the radiation field increases beyond the saturation intensity of the transition. In pulsed-field excitation, linear power broadening occurs for a pulse of rectangular temporal shape. Pulses with smooth shapes are known to exhibit much less power broadening, e.g., logarithmic for a Gaussian pulse shape. It has been predicted, but never experimentally verified, that pulse shapes which vanish in time as $\sim |t{|}^{-\lambda }$ should exhibit the opposite effect—power narrowing—in which the postpulse transition line width decreases as the amplitude of the driving pulse increases. In this Letter, power narrowing is demonstrated for a class of powers-of-Lorentzian pulse shapes on the IBM Quantum processor ibmq_manila. Reduction of the line width by a factor of over 10 is observed when increasing the pulse area from $\pi$ to $7\pi$, in a complete reversal of the power broadening paradigm. Moreover, thorough study is conducted on the truncation of the pulse wings which introduces a (small) power-broadened term which prevents power narrowing from reaching extreme values. In the absence of other power broadening mechanisms, Lorentzian pulses truncated at sufficiently small values can achieve as narrow line profiles as desired.

When hypothetical neutrino secret interactions ($\nu \mathrm{SI}$) are large, they form a fluid in a supernova (SN) core, flow out with sonic speed, and stream away as a fireball. For the first time, we tackle the complete dynamical problem and solve all steps, systematically using relativistic hydrodynamics. The impact on SN physics and the neutrino signal is remarkably small. For complete thermalization within the fireball, the observable spectrum changes in a way that is independent of the coupling strength. One potentially large effect beyond our study is quick deleptonization if $\nu \mathrm{SI}$ violate lepton number. By present evidence, however, SN physics leaves open a large region in parameter space, where laboratory searches and future high-energy neutrino telescopes will probe $\nu \mathrm{SI}$.

We have studied the mutual neutralization reaction of vibronically cold ${\mathrm{NO}}^{+}$ with ${\mathrm{O}}^{-}$ at a collision energy of $\approx 0.1\mathrm{eV}$ and under single-collision conditions. The reaction is completely dominated by production of three ground-state atomic fragments. We employ product-momentum analysis in the framework of a simple model, which assumes the anion acts only as an electron donor and the product neutral molecule acts as a free rotor, to conclude that the process occurs in a two-step mechanism via an intermediate Rydberg state of NO which subsequently fragments.

We introduce a general method to engineer arbitrary Hamiltonians in the Floquet phase space of a periodically driven oscillator, based on the noncommutative Fourier transformation technique. We establish the relationship between an arbitrary target Floquet Hamiltonian in phase space and the periodic driving potential in real space. We obtain analytical expressions for the driving potentials in real space that can generate novel Hamiltonians in phase space, e.g., rotational lattices and sharp-boundary wells. Our protocol can be realized in a range of experimental platforms for nonclassical state generation and bosonic quantum computation.

We experimentally demonstrate optoacoustic cooling via stimulated Brillouin-Mandelstam scattering in a 50 cm long tapered photonic crystal fiber. For a 7.38 GHz acoustic mode, a cooling rate of 219 K from room temperature has been achieved. As anti-Stokes and Stokes Brillouin processes naturally break the symmetry of phonon cooling and heating, resolved sideband schemes are not necessary. The experiments pave the way to explore the classical to quantum transition for macroscopic objects and could enable new quantum technologies in terms of storage and repeater schemes.

The hexatic phase is an intermediate stage in the melting process of a 2D crystal due to topological defects. Recently, this exotic phase was experimentally identified in the vortex lattice of 2D weakly disordered superconducting MoGe by scanning tunneling microscopic measurements. Here, we study this vortex state by the Nernst effect, which is an effective and sensitive tool to detect vortex motion, especially in the superconducting fluctuation regime. We find a surprising Nernst sign reversal at the melting transition of the hexatic phase. We propose that they are a consequence of vortex dislocations in the hexatic state which diffuse preferably from the cold to hot.

Twisted light carries a nonzero orbital angular momentum, that can be transferred from light to electrons and particles ranging from nanometers to micrometers. Up to now, the interplay between twisted light with dipolar systems has scarcely been explored, though the latter bear abundant forms of topologies such as skyrmions and embrace strong light-matter coupling. Here, using first-principles-based simulations, we show that twisted light can excite and drive dynamical polar skyrmions and transfer its nonzero winding number to ferroelectric ultrathin films. The skyrmion is successively created and annihilated alternately at the two interfaces, and experiences a periodic transition from a markedly “Bloch” to “Néel” character, accompanied with the emergence of a “Bloch point” topological defect with vanishing polarization. The dynamical evolution of skyrmions is connected to a constant jump of topological number between “0” and “1” over time. These intriguing phenomena are found to have an electrostatic origin. Our study thus demonstrates that, and explains why this unique light-matter interaction can be very powerful in creating and manipulating topological solitons in functional materials.

We explore optical parametric oscillation (OPO) in nanophotonic resonators, enabling arbitrary, nonlinear phase matching and nearly lossless control of energy conversion. Such pristine OPO laser converters are determined by nonlinear light-matter interactions, making them both technologically flexible and broadly reconfigurable. We utilize a nanostructured inner-wall modulation in the resonator to achieve universal phase matching for OPO-laser conversion, but coherent backscattering also induces a counterpropagating pump laser. This depletes the intraresonator optical power in either direction, increasing the OPO threshold power and limiting laser-conversion efficiency, the ratio of optical power in target signal and idler frequencies to the pump. We develop an analytical model of this system that emphasizes an understanding of optimal laser-conversion and threshold behaviors, and we use the model to guide experiments with nanostructured-resonator OPO laser-conversion circuits, fully integrated on chip and unlimited by group-velocity dispersion. Our Letter demonstrates the fundamental connection between OPO laser-conversion efficiency and the resonator coupling rate, subject to the relative phase and power of counterpropagating pump fields. We achieve $(40\pm 4)\mathrm{mW}$ of on-chip power, corresponding to $(41\pm 4)\%$ conversion efficiency, and discover a path toward near-unity OPO laser-conversion efficiency.

We show here that soap films—typically expected to host symmetric molecular arrangements—can be constructed with differing opposite surfaces, breaking their symmetry, and making them reminiscent of functional biological motifs found in nature. Using fluorescent molecular probes as dopants on different sides of the film, resonance energy transfer could be employed to confirm the lack of symmetry, which was found to persist on timescales of several minutes. Further, a theoretical analysis of the main transport phenomena involved yielded good agreement with the experimental observations.

We investigate order parameter fluctuations in the Hubbard model within a time-dependent Gutzwiller approach. While in the weak coupling limit we find that the amplitude fluctuations are short-lived due to a degeneracy with the energy of the edge of the quasiparticle continua (and in agreement with $\text{Hartree-Fock}+\mathrm{RPA}$ theory), these are shifted below the edge upon increasing the interaction. Our calculations therefore predict undamped amplitude (Higgs) oscillations of the order parameter in strongly coupled superconductors, cold atomic fermion condensates, and strongly interacting charge- and spin-density wave systems. We propose an experimental realization for the detection of the spin-type Higgs mode in undoped cuprates and related materials where, due to the Dzyaloshinsky-Moriya interaction, it can couple to an out-of-plane ferromagnetic excitation that is visible via the Faraday effect.

Coupling of orbital degree of freedom with a spin exchange, i.e., Kugel-Khomskii-type interaction (KK), governs a host of material properties, including colossal magnetoresistance, enhanced magnetoelectric response, and photoinduced high-temperature magnetism. In general, KK-type interactions lead to deviation in experimental observables of coupled Hamiltonian near or below the magnetic transition. Using diffraction and spectroscopy experiments, here we report anomalous changes in lattice parameters, electronic states, spin dynamics, and phonons at four times the Néel transition temperature ($T_{\mathrm{N}}$) in ${\mathrm{CrVO}}_4$. The temperature is significantly higher than other $d$-orbital compounds such as manganites and vanadates, where effects are limited to near or below $T_{\mathrm{N}}$. The experimental observations are rationalized using first-principles and Green’s function-based phonon and spin simulations that show unprecedentedly strong KK-type interactions via a superexchange process and an orbital-selective spin-phonon coupling coefficient at least double the magnitude previously reported for strongly coupled spin-phonon systems. Our results present an opportunity to explore the effect of KK-type interactions and spin-phonon coupling well above $T_{\mathrm{N}}$ and possibly bring various properties closer to application, for example, strong room-temperature magnetoelectric coupling.