The coherent storage and phase modulation of x-ray single-photon wave packets in the resonant scattering of light off nuclei is theoretically investigated. We show that by switching off and on again the magnetic field in the nuclear sample, phase-sensitive storage of photons in the keV regime can be achieved. Corresponding $\pi$ phase modulation of the stored photon can be accomplished if the retrieving magnetic field is rotated by 180°. The development of such x-ray single-photon control techniques is a first step towards forwarding quantum optics and quantum information to shorter wavelengths and more compact photonic devices.

We investigate the efficiency of systems of molecular motors operating at maximum power. We consider two models of kinesin motors on a microtubule: for both the simplified and the detailed model, we find that the many-body exclusion effect enhances the efficiency at maximum power of the many-motor system, with respect to the single motor case. Remarkably, we find that this effect occurs in a limited region of the system parameters, compatible with the biologically relevant range.

We report on the results of a search for the electron electric dipole moment $d_e$ using paramagnetic ferroelectric ${\mathrm{Eu}}_{0.5}{\mathrm{Ba}}_{0.5}{\mathrm{TiO}}_3$. The electric polarization creates an effective electric field that makes it energetically favorable for the spins of the seven unpaired $4f$ electrons of the ${\mathrm{Eu}}^{2+}$ to orient along the polarization, provided that $d_e\ne 0$. This interaction gives rise to sample magnetization, correlated with its electric polarization, and is therefore equivalent to a linear magnetoelectric effect. A SQUID magnetometer is used to search for the resulting magnetization. We obtain $d_e=(-1.07\pm {3.06}_{\mathrm{stat}}\pm {1.74}_{\mathrm{syst}})\times {10}^{-25}e\mathrm{cm}$, implying an upper limit of $|d_e|<6.05\times {10}^{-25}e\mathrm{cm}$ (90% confidence).

In this Letter, we show through numerical simulations and analytical results that overlapping multiple ($N$) laser beams in plasmas can lead to strong stochastic ion heating from many ($\propto N^2$) electrostatic perturbations driven by beat waves between pairs of laser beams. For conditions typical of inertial-confinement-fusion experiment conditions, hundreds of such beat waves are driven in ${\mathrm{mm}}^3$-scale plasmas, leading to ion heating rates of several $\mathrm{keV}/\mathrm{ns}$. This mechanism saturates cross-beam energy transfer, with a reduction of linear gains by a factor $\sim 4–5$ and can strongly modify the overall hydrodynamics evolution of such laser-plasma systems.

We demonstrate both theoretically and experimentally nonparaxial Mathieu and Weber accelerating beams, generalizing the concept of previously found accelerating beams. We show that such beams bend into large angles along circular, elliptical, or parabolic trajectories but still retain nondiffracting and self-healing capabilities. The circular nonparaxial accelerating beams can be considered as a special case of the Mathieu accelerating beams, while an Airy beam is only a special case of the Weber beams at the paraxial limit. Not only do generalized nonparaxial accelerating beams open up many possibilities of beam engineering for applications, but the fundamental concept developed here can be applied to other linear wave systems in nature, ranging from electromagnetic and elastic waves to matter waves.

Nonequilibrium molecular dynamics simulations are used to show that the shear viscosity of a polymer melt can be significantly reduced when filled with small energetically neutral nanoparticles, apparently independent of the polymer’s chain length. Analogous to solvent molecules, small nanoparticles act akin to plasticizers and reduce the viscosity of a polymer melt. This effect, which persists for particles whose sizes are as large as the chain size or the entanglement mesh size, whichever is smaller, can be overcome by making the chain-nanoparticle interactions significantly attractive. Our simulations allow us to systematically organize the viscosity data of filled polymer melts, and thus provide a strong basis from which to predict the flow behavior of these commercially important class of materials.

In this Letter we show that quantum nonlocality can be superactivated. That is, one can obtain violations of Bell inequalities by tensorizing a local state with itself. In the second part of this work we study how large these violations can be. In particular, we show the existence of quantum states with very low Bell violation but such that five copies of them give very large violations. In fact, this gap can be made arbitrarily large by increasing the dimension of the states.

We report the discovery of the formation of an electron Cooper pair approximately 40 eV above the double-ionization threshold in benzene, naphthalene, anthracene, and coronene after absorption of a single photon. We have measured the ratios of doubly to singly charged parent ions of the above mentioned molecules as well as pyrrole and furan by using monochromatized synchrotron radiation up to 100 eV above the corresponding thresholds. We also recorded photoelectron spectra of benzene and naphthalene at selected energies. The electron-pair formation is based on the specific structure of the molecules and does not exist for pyrrole and furan.

We report on the direct observation of coherent backscattering (CBS) of ultracold atoms in a quasi-two-dimensional configuration. Launching atoms with a well-defined momentum in a laser speckle disordered potential, we follow the progressive build up of the momentum scattering pattern, consisting of a ring associated with multiple elastic scattering, and the CBS peak in the backward direction. Monitoring the depletion of the initial momentum component and the formation of the angular ring profile allows us to determine microscopic transport quantities. We also study the time evolution of the CBS peak and find it in fair agreement with predictions, at long times as well as at short times. The observation of CBS can be considered a direct signature of coherence in quantum transport of particles in disordered media. It is responsible for the so called weak localization phenomenon, which is the precursor of Anderson localization.

In a three-dimensional Fermi liquid, quasiparticles near the Fermi surface may possess a Berry curvature. We show that if the Berry curvature has a nonvanishing flux through the Fermi surface, the particle number associated with this Fermi surface has a triangle anomaly in external electromagnetic fields. We show how Landau’s Fermi liquid theory should be modified to take into account the Berry curvature. We show that the “chiral magnetic effect” also emerges from the Berry curvature flux.

We investigate the effect of an ambient fluid on the dynamics of collapse and spread of a granular column simulated by means of the contact dynamics method interfaced with computational fluid dynamics. The runout distance is found to increase as a power law with the aspect ratio of the column, and, surprisingly, for a given aspect ratio and packing fraction, it may be similar in the grain-inertial and fluid-inertial regimes but with considerably longer duration in the latter case. We show that the effect of fluid in viscous and fluid-inertial regimes is to both reduce the kinetic energy during collapse and enhance the flow by lubrication during spread. Hence, the runout distance in a fluid may be below or equal to that in the absence of fluid due to compensation between those effects.

We have discovered a new type of interaction between micro- or nanoscale particles that results from the entanglement of strands attached to their surfaces. Self-complementary DNA single strands on a particle can hybridize to form loops. A similar proximal particle can have its loops catenate with those of the first. Unlike conventional thermodynamic interparticle interactions, the catenation interaction is strongly history and protocol dependent, allowing for nonequilibrium particle assembly. The interactions can be controlled by an interesting combination of forces, temperature, light sensitive cross-linking and enzymatic unwinding of the topological links. This novel topological interaction may lead to new materials and phenomena such as particles strung on necklaces, confined motions on designed contours and surfaces, and colloidal Olympic gels.

We demonstrate rotational and vibrational cooling of cesium dimers by optical pumping techniques. We use two laser sources exciting all the populated rovibrational states, except a target state that thus behaves like a dark state where molecules pile up thanks to absorption-spontaneous emission cycles. We are able to accumulate photoassociated cold ${\mathrm{Cs}}_2$ molecules in their absolute ground state ($v=0$, $J=0$) with up to 40% efficiency. Given its simplicity, the method could be extended to other molecules and molecular beams. It also opens up general perspectives in laser cooling the external degrees of freedom of molecules.

The influence of quantum effects on the processes of initiation of combustion and detonation of hydrogen and acetylene near the low-temperature limits at elevated pressures is analyzed. A theoretical consideration which allows quantification of the quantum corrections to the rate constants of endothermic reactions associated with an increase in the high-energy tail of the equilibrium momentum distribution function at high pressures is presented. This quantum effect is caused by a manifestation of the principle of uncertainty for the energy of the colliding particles at a high frequency of collisions. It is shown that significant deviations of experimentally observed ignition and detonation delay time from the predictions of kinetic calculations are quite well described by the proposed quantum corrections. This general mechanism should be considered in the safety problem with emergency emissions of hydrogen at nuclear power stations, as well as problems of the safe production and storage of hydrogen and acetylene, which have a fundamental importance for industry and power engineering.

Using a superconducting circuit, the Josephson mixer, we demonstrate the first experimental realization of spatially separated two-mode squeezed states of microwave light. Driven by a pump tone, a first Josephson mixer generates, out of quantum vacuum, a pair of entangled fields at different frequencies on separate transmission lines. A second mixer, driven by a $\pi$-phase shifted copy of the first pump tone, recombines and disentangles the two fields. The resulting output noise level is measured to be lower than for the vacuum state at the input of the second mixer, an unambiguous proof of entanglement. Moreover, the output noise level provides a direct, quantitative measure of entanglement, leading here to the demonstration of $6\mathrm{Mebit}·{\mathrm{s}}^{-1}$ (mega entangled bits per second) generated by the first mixer.

Phase transitions are not usually seen in the time domain. Here, we report on the finding of critical times at which a physical observable, in the thermodynamic limit, becomes nonanalytic as a function of time. We find that the coherence of a probe spin coupled to a many-body system vanishes at times in one-to-one correspondence to the Lee-Yang zeros of the partition function of the many-body system. In the thermodynamic limit, the Lee-Yang zeros form a continuum cut in the complex plane of fugacity and the probe spin coherence presents sudden death and birth at the critical times corresponding to the Yang-Lee singularities. These results provide new experimental possibilities in many-body physics.

The emission of plasmonic light from a single ${\mathrm{C}}_{60}$ molecule on Cu(111) is probed in a scanning tunneling microscope from the weak-coupling, tunneling range to strong coupling of the molecule to the electrodes at contact. At positive sample voltage the photon yield decreases owing to shot-noise suppression in an increasingly transparent quantum contact. At reversed bias an unexpected nonlinear increase occurs. First-principles transport calculations reveal that ultrafast charge fluctuations on the molecule give rise to additional noise at optical frequencies beyond the shot noise of the current that is injected to the tip.

We studied the low-energy states of spin-$1/2$ quantum dots defined in $\mathrm{InAs}/\mathrm{InP}$ nanowires and coupled to aluminum superconducting leads. By varying the superconducting gap $\Delta$ with a magnetic field $B$ we investigated the transition from strong coupling $\Delta \ll T_K$ to weak-coupling $\Delta \gg T_K$, where $T_K$ is the Kondo temperature. Below the critical field, we observe a persisting zero-bias Kondo resonance that vanishes only for low $B$ or higher temperatures, leaving the room to more robust subgap structures at bias voltages between $\Delta$ and $2\Delta$. For strong and approximately symmetric tunnel couplings, a Josephson supercurrent is observed in addition to the Kondo peak. We ascribe the coexistence of a Kondo resonance and a superconducting gap to a significant density of intragap quasiparticle states, and the finite-bias subgap structures to tunneling through Shiba states. Our results, supported by numerical calculations, own relevance also in relation to tunnel-spectroscopy experiments aiming at the observation of Majorana fermions in hybrid nanostructures.

We report numerical simulations of membrane tubulation driven by large colloidal particles. Using Monte Carlo simulations we study how the process depends on particle size and binding strength, and present accurate free energy calculations to sort out how tube formation compares with the competing budding process. We find that tube formation is a result of the collective behavior of the particles adhering on the surface, and it occurs for binding strengths that are smaller than those required for budding. We also find that long linear aggregates of particles forming on the membrane surface act as nucleation seeds for tubulation by lowering the free energy barrier associated to the process.

How nanoparticles interact with biomembranes is central for understanding their bioactivity. In this Letter, we report novel tubular membrane structures induced by adsorbed spherical nanoparticles, which we obtain from energy minimization. The membrane tubules enclose linear aggregates of particles and protrude into the vesicles. The high stability of the particle-filled tubules implies strongly attractive, membrane-mediated interactions between the particles. The tubular structures may provide a new route to encapsulate nanoparticles reversibly in vesicles.