Single charge nanoscale detection in ambient conditions is a current frontier in metrology that has diverse interdisciplinary applications. Here, such single charge detection is demonstrated using two nitrogen-vacancy (NV) centers in diamond. One NV center is employed as a sensitive electrometer to detect the change in electric field created by the displacement of a single electron resulting from the optical switching of the other NV center between its neutral ($\mathrm{NV}{}^0$) and negative ($\mathrm{NV}{}^{-}$) charge states. As a consequence, our measurements also provide direct insight into the charge dynamics inside the material.

We report experimental results on x-ray diffraction of quantum-state-selected and strongly aligned ensembles of the prototypical asymmetric rotor molecule 2,5-diiodobenzonitrile using the Linac Coherent Light Source. The experiments demonstrate first steps toward a new approach to diffractive imaging of distinct structures of individual, isolated gas-phase molecules. We confirm several key ingredients of single molecule diffraction experiments: the abilities to detect and count individual scattered x-ray photons in single shot diffraction data, to deliver state-selected, e.g., structural-isomer-selected, ensembles of molecules to the x-ray interaction volume, and to strongly align the scattering molecules. Our approach, using ultrashort x-ray pulses, is suitable to study ultrafast dynamics of isolated molecules.

High-resolution x-ray imaging techniques offer a variety of possibilities for studying the nanoscale structure of biological cells. A challenging task remains the study of cells by x rays in their natural, aqueous environment. Here, we overcome this limitation by presenting scanning x-ray diffraction measurements with beam sizes in the range of a few hundred nm on living and fixed-hydrated eukaryotic cells in microfluidic devices which mimic a native environment. The direct comparison between fixed-hydrated and living cells shows distinct differences in the scattering signal, pointing to structural changes on the order of 30 to 50 nm.

The new regime of resonant nuclear photoexcitation rendered possible by x-ray free-electron laser beams interacting with solid state targets is investigated theoretically. Our results unexpectedly show that secondary processes coupling nuclei to the atomic shell in the created cold high-density plasma can dominate direct photoexcitation. As an example, we discuss the case of ${}^{93m}\mathrm{Mo}$ isomer depletion for which nuclear excitation by electron capture as a secondary process is shown to be orders of magnitude more efficient than the direct laser-nucleus interaction. General arguments revisiting the role of the x-ray free-electron laser in nuclear experiments involving solid-state targets are further deduced.

We investigate theoretically the suppression of two-body losses when the on-site loss rate is larger than all other energy scales in a lattice. This work quantitatively explains the recently observed suppression of chemical reactions between two rotational states of fermionic KRb molecules confined in one-dimensional tubes with a weak lattice along the tubes [Yan et al., Nature (London) 501, 521 (2013)]. New loss rate measurements performed for different lattice parameters but under controlled initial conditions allow us to show that the loss suppression is a consequence of the combined effects of lattice confinement and the continuous quantum Zeno effect. A key finding, relevant for generic strongly reactive systems, is that while a single-band theory can qualitatively describe the data, a quantitative analysis must include multiband effects. Accounting for these effects reduces the inferred molecule filling fraction by a factor of 5. A rate equation can describe much of the data, but to properly reproduce the loss dynamics with a fixed filling fraction for all lattice parameters we develop a mean-field model and benchmark it with numerically exact time-dependent density matrix renormalization group calculations.

We discuss the dc conductivity of holographic theories with translational invariance broken by a background lattice. We show that the presence of the lattice induces an effective mass for the graviton via a gravitational version of the Higgs mechanism. This allows us to obtain, at leading order in the lattice strength, an analytic expression for the dc conductivity in terms of the size of the lattice at the horizon. In locally critical theories this leads to a power law resistivity that is in agreement with an earlier field theory analysis of Hartnoll and Hofman.

We use the context of dryland vegetation to study a general problem of complex pattern-forming systems: multiple pattern-forming instabilities that are driven by distinct mechanisms but share the same spectral properties. We find that the co-occurrence of two Turing instabilities when the driving mechanisms counteract each other in some region of the parameter space results in the growth of a single mode rather than two interacting modes. The interplay between the two mechanisms compensates for the simpler dynamics of a single mode by inducing a wider variety of patterns, which implies higher biodiversity in dryland ecosystems.

Squeezed vacuum states constitute a particularly useful resource in quantum information as well as in quantum metrology. The frequency conversion of these states is important to provide the bridge between different wavelengths within a sequence of downstream applications and also to provide a way for squeezed-state generation at so-far inaccessible wavelengths. Here we demonstrate the external quantum up-conversion of carrier-light-free squeezed vacuum states for the first time. Our result proves that nondegenerate sum-frequency generation preserves the coherences that are present between photon pairs and higher-order photon pairs of the squeezed input state.

We study a hybrid system formed from an optomechanical resonator and a cavity mode strongly coupled to an excitonic transition inside a quantum well. We show that due to the mixing of cavity photon and exciton states, the emergent quasiparticles—polaritons—possess coupling to the mechanical mode of both a dispersive and dissipative nature. We calculate the occupancies of polariton modes and reveal bistable behavior, which deviates from conventional Kerr nonlinearity or dispersive coupling cases due to the dissipative coupling. The described system serves as a good candidate for future polaritonic devices.

We propose a class of attacks on quantum key distribution (QKD) systems where an eavesdropper actively engineers new loopholes by using damaging laser illumination to permanently change properties of system components. This can turn a perfect QKD system into a completely insecure system. A proof-of-principle experiment performed on an avalanche photodiode-based detector shows that laser damage can be used to create loopholes. After $\sim 1\mathrm{W}$ illumination, the detectors’ dark count rate reduces 2–5 times, permanently improving single-photon counting performance. After $\sim 1.5\mathrm{W}$, the detectors switch permanently into the linear photodetection mode and become completely insecure for QKD applications.

Penning ionization initiates the evolution of a dense molecular Rydberg gas to plasma. This process selects for pairs of excited molecules separated by a distance of two Rydberg orbital diameters or less. The deactivated Penning partners predissociate, depleting the leading edge of the distribution of nearest-neighbor distances. For certain density and orbital radii, this sequence of events can form a plasma in which large distances separate a disproportionate fraction of the ions. Experimental results and model calculations suggest that the reduced potential energy of this Penning lattice significantly affects the development of strong coupling in an ultracold plasma.

We report an observation of long-lived spin-singlet states in a ${{}^{13}\mathrm{C}\text{−}{}^1\mathrm{H}}^{}$ spin pair in a zero magnetic field. In ${}^{13}\mathrm{C}$-labeled formic acid, we observe spin-singlet lifetimes as long as 37 s, about a factor of 3 longer than the $T_1$ lifetime of dipole polarization in the triplet state. In contrast to common high-field experiments, the observed coherence is a singlet-triplet coherence with a lifetime $T_2$ longer than the $T_1$ lifetime of dipole polarization in the triplet manifold. Moreover, we demonstrate that heteronuclear singlet states formed between a ${}^1\mathrm{H}$ and a ${}^{13}\mathrm{C}$ nucleus can exhibit longer lifetimes than the respective triplet states even in the presence of additional spins that couple to the spin pair of interest. Although long-lived homonuclear spin-singlet states have been extensively studied, this is the first experimental observation of analogous singlet states in heteronuclear spin pairs.