Effect of transient shell formation on shock-induced atomization of an evaporating nanofluid droplet
Phys. Rev. Fluids 11, 103603 – Published 14 October, 2026
DOI: https://doi.org/10.1103/9jns-3l1z
Abstract
Understanding the breakup of evaporating nanofluid droplets under extreme aerodynamic loads is essential for applications in drug delivery, material deposition, defense, and propulsion. This study investigates the shock-induced atomization dynamics of an acoustically levitated TM-10 nanofluid droplet subjected to a coaxially propagating blast wave and subsequent compressible vortex ring, generated using a compact wire-explosion shock source. The blast wave imposes a sharp velocity discontinuity, followed by a decaying flow field and a vortex-dominated interaction that drives droplet disintegration. Laser-induced heating promotes evaporation, increasing nanoparticle concentration, viscosity, and agglomeration within the droplet. Progressive evaporation leads to interfacial nanoparticle accumulation, initiating a sol-gel transition when the local volume fraction exceeds the gelation threshold, and ultimately forming a solid outer shell as the maximum packing limit is approached. Shock interactions are systematically examined across three evaporation stages: (1) steady liquid phase, (2) gel-shell phase, and (3) solid-shell phase. Each regime exhibits distinct atomization responses due to the evolving interfacial morphology. In the gel-shell regime, deformation is resisted by the viscous shell, producing a bag-on-sheet mode, followed by puncture, jetting, and eventual shell delamination. In the solid-shell regime, interactions intensify, resulting in brittle fragmentation and catastrophic fracture. The findings reveal how evaporation-driven interfacial transitions fundamentally alter breakup mechanisms under transient shock loading. By linking nanoparticle transport, shell formation, and flow-droplet interaction across multiple timescales, this work establishes physical insights into the atomization of complex, multicomponent, multiphase, and transiently evolving droplets under extreme aerodynamic conditions.