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Diffuselet method for three-dimensional turbulent mixing of a cloudy air filament

Vladyslav Pushenko1, Simone Scollo2, Patrice Meunier2, Emmanuel Villermaux2,3, and Jörg Schumacher1,4

Phys. Rev. Fluids 10, 074503 – Published 16 July, 2025

DOI: https://doi.org/10.1103/1bt3-mlpm

Abstract

The mixing properties of vapor content, temperature, and particle fields are of paramount importance in cloud turbulence as they pertain to essential processes, such as cloud water droplet evaporation and entrainment. Our study examines the mixing of a single cloudy air (which implies droplet-laden) filament with its clear air environment, a characteristic process at the cloud edge, in two ways. The first consists of three-dimensional combined Euler-Lagrangian direct numerical simulations which describe the scalar supersaturation as an Eulerian field and the individual cloud water droplets as an ensemble of Lagrangian tracers. The second way builds on the recently developed diffuselet method, a kinematic Lagrangian framework that decomposes a scalar filament into a collection of small sections subject to deformation by local stirring and cross-sheet diffusion. The Schmidt number is Sc=0.7. The entrainment process causes a deformation of the supersaturated cloud filament in combination with diffusion until the system reaches a well-mixed equilibrium state, which implies for the present configuration that all droplets are evaporated. We compare the time dependence of the mean square and probability density function of the supersaturation field. For the initial period of the mixing process, they agree very well; at later stages, deviations caused by nonzero mean of the conserved scalar are observed. For the cases including cloud water droplets, we also investigate the impact of droplet number density and condensation growth response. Turbulence causes deviations from the d2 law similar to recent experiments in sprays. A simulation at a Schmidt number that is by a factor of 100 larger than in clouds improves the agreement between simulation and diffuselet method significantly. The latter result promotes the diffuselet framework as an efficient parametrization for turbulent high-Sc mixing which can reduce the resolution efforts of the viscous-convective range of scalar turbulence.

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References (51)

  1. R. A. Shaw, Particle-turbulence interactions in atmospheric clouds, Annu. Rev. Fluid Mech. 35, 183 (2003).
  2. E. Bodenschatz, S. P. Malinowski, R. A. Shaw, and F. Stratmann, Can we understand clouds without turbulence? Science 327, 970 (2010).
  3. B. Stevens and S. Bony, Water in the atmosphere, Phys. Today 66(6), 29 (2013).
  4. R. Vogel, A. L. Albright, J. Vial, G. George, B. Stevens, and S. Bony, Strong cloud–circulation coupling explains weak trade cumulus feedback, Nature (London) 612, 696 (2022).
  5. R. R. Rogers and M. K. Yau, A Short Course in Cloud Physics (Butterworth-Heinemann, Oxford, UK, 1989).
  6. M. B. Baker, R. E. Breidenthal, T. W. Choularton, and J. Latham, The effects of turbulent mixing in clouds, J. Atmos. Sci. 41, 299 (1984).
  7. M. Andrejczuk, W. W. Grabowski, S. P. Malinowski, and P. K. Smolarkiewicz, Numerical simulation of cloud–clear air interfacial mixing: Effects on cloud microphysics, J. Atmos. Sci. 63, 3204 (2006).
  8. A. Celani, A. Mazzino, and M. Tizzi, The equivalent size of cloud condensation nuclei, New J. Phys. 10, 075021 (2008).
  9. G. Sardina, F. Picano, L. Brandt, and R. Caballero, Continuous growth of droplet size variance due to condensation in turbulent clouds, Phys. Rev. Lett. 115, 184501 (2015).
  10. B. Kumar, P. Götzfried, N. Suresh, J. Schumacher, and R. A. Shaw, Scale dependence of cloud microphysical response to turbulent entrainment and mixing, J. Adv. Model. Earth Syst. 10, 2777 (2018).
  11. J. Fries, G. Sardina, G. Svensson, and B. Mehlig, Key parameters for droplet evaporation and mixing at the cloud edge, Q. J. R. Meteorol. Soc. 147, 2160 (2021).
  12. B. Kumar, R. Ranjan, M. K. Yau, S. Bera, and S. A. Rao, Impact of high and low vorticity turbulence on cloud environment mixing and cloud microphysics processes, Atmos. Chem. Phys. 21, 12317 (2021).
  13. W. W. Grabowski, L. Thomas, and B. Kumar, Impact of cloud-base turbulence on CCN activation: single-size CCN, J. Atmos. Sci. 79, 551 (2022).
  14. J. Fries, G. Sardina, G. Svensson, A. Pumir, and B. Mehlig, Lagrangian supersaturation fluctuations at the cloud edge, Phys. Rev. Lett. 131, 254201 (2023).
  15. L. Magaritz-Ronen, M. Pinsky, and A. Khain, Drizzle formation in stratocumulus clouds: Effects of turbulent mixing, Atmos. Chem. Phys. 16, 1849 (2016).
  16. P. E. Dimotakis, Turbulent mixing, Annu. Rev. Fluid Mech. 37, 329 (2005).
  17. K. R. Sreenivasan and J. Schumacher, Lagrangian views on turbulent mixing of passive scalars, Phil. Trans. R. Soc. A 368, 1561 (2010).
  18. K. R. Sreenivasan, Turbulent mixing: A perspective, Proc. Natl. Acad. Sci. USA 116, 18175 (2019).
  19. E. Villermaux, Mixing versus stirring, Annu. Rev. Fluid Mech. 51, 245 (2019).
  20. G. K. Batchelor, Small-scale variation of convected quantities like temperature in turbulent fluid Part 1. General discussion and the case of small conductivity, J. Fluid Mech. 5, 113 (1959).
  21. R. H. Kraichnan, Small-scale structure of a scalar field convected by turbulence, Phys. Fluids 11, 945 (1968).
  22. E. Villermaux and J. Duplat, Mixing as an aggregation process, Phys. Rev. Lett. 91, 184501 (2003).
  23. P. Meunier and E. Villermaux, How vortices mix, J. Fluid Mech. 476, 213 (2003).
  24. P. Meunier and E. Villermaux, The diffusive strip method for scalar mixing in two dimensions, J. Fluid Mech. 662, 134 (2010).
  25. P. Meunier and E. Villermaux, The diffuselet concept for scalar mixing, J. Fluid Mech. 951, A33 (2022).
  26. B. Kumar, F. Janetzko, J. Schumacher, and R. A. Shaw, Extreme responses of a coupled scalar–particle system during turbulent mixing, New J. Phys. 14, 115020 (2012).
  27. B. Kumar, J. Schumacher, and R. A. Shaw, Cloud microphysical effects of turbulent mixing and entrainment, Theor. Comput. Fluid Dyn. 27, 361 (2013).
  28. B. Kumar, J. Schumacher, and R. A. Shaw, Lagrangian mixing dynamics at the cloudy–clear air interface, J. Atmos. Sci. 71, 2564 (2014).
  29. P. Götzfried, B. Kumar, R. A. Shaw, and J. Schumacher, Droplet dynamics and fine-scale structure in a shearless turbulent mixing layer with phase changes, J. Fluid Mech. 814, 452 (2017).
  30. A. Celani, G. Falkovich, A. Mazzino, and A. Seminara, Droplet condensation in turbulent flows, Europhys. Lett. 70, 775 (2005).
  31. V. Pushenko and J. Schumacher, Connecting finite-time Lyapunov exponents with supersaturation and droplet dynamics in a turbulent bulk flow, Phys. Rev. E 109, 045101 (2024).
  32. J. Schumacher, Sub-Kolmogorov-scale fluctuations in fluid turbulence, Europhys. Lett. 80, 54001 (2007).
  33. A. de Rivas and E. Villermaux, Dense spray evaporation as a mixing process, Phys. Rev. Fluids 1, 014201 (2016).
  34. A. N. Kolmogorov, The local structure of turbulence in incompressible viscous fluid for very large Reynolds numbers, Dokl. Akad. Nauk SSSR 30, 299 (1941).
  35. A. M. Obukhov, Structure of the temperature field in a turbulent flow, Izv. Akad. Nauk SSSR, Ser. Geogr. and Geofiz. 13, 281 (1949).
  36. S. Corrsin, On the spectrum of isotropic temperature fluctuations in an isotropic turbulence, J. Appl. Phys. 22, 469 (1951).
  37. J. M. Ottino, Mixing, chaotic advection, and turbulence, Annu. Rev. Fluid Mech. 22, 207 (1990).
  38. D. Pekurovsky, P3DFFT: A framework for parallel computations of Fourier transforms in three dimensions, SIAM J. Sci. Comput. 34, C192 (2012).
  39. P. K. Yeung and S. B. Pope, An algorithm for tracking fluid particles in numerical simulations of homogeneous turbulence, J. Comput. Phys. 79, 373 (1988).
  40. W. E. Ranz, Applications of a stretch model to mixing, diffusion, and reaction in laminar and turbulent flows, AIChE J. 25, 41 (1979).
  41. W. T. Ashurst, A. R. Kerstein, R. M. Kerr, and C. H. Gibson, Alignment of vorticity and scalar gradient with strain rate in simulated Navier–Stokes turbulence, Phys. Fluids 30, 2343 (1987).
  42. S. S. Girimaji and S. B. Pope, Material-element deformation in isotropic turbulence, J. Fluid Mech. 220, 427 (1990).
  43. G. Zinchenko, V. Pushenko, and J. Schumacher, Local precursors to anomalous dissipation in Navier-Stokes turbulence: Burgers vortex-type models and simulation analysis, Phys. Rev. Fluids 9, 114608 (2024).
  44. G. C. Burton and W. J. A. Dahm, Multifractal subgrid-scale modeling for large-eddy simulation. II. Backscatter limiting and a posteriori evaluation, Phys. Fluids 17, 075112 (2005).
  45. G. C. Burton, The nonlinear large-eddy simulation method applied to Sc≈1 and Sc≫1 passive-scalar mixing, Phys. Fluids 20, 035103 (2008).
  46. P. Götzfried, M. S. Emran, E. Villermaux, and J. Schumacher, Comparison of Lagrangian and Eulerian frames of passive scalar turbulent mixing, Phys. Rev. Fluids 4, 044607 (2019).
  47. R. C. Srivastava, Growth of cloud drops by condensation: A criticism of currently accepted theory and a new approach, J. Atmos. Sci. 46, 869 (1989).
  48. E. Villermaux, A. Moutte, M. Amielh, and P. Meunier, Fine structure of the vapor field in evaporating dense sprays, Phys. Rev. Fluids 2, 074501 (2017).
  49. https://www.gauss-centre.eu.
  50. https://www.lrz.de.
  51. 10.5281/zenodo.15853362.

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