- Open Access
Dynamics in vibrofluidized beds: A diffusing wave spectroscopy study
Phys. Rev. E 112, 025405 – Published 4 August, 2025
DOI: https://doi.org/10.1103/f3m6-b42t
Abstract
We demonstrate the densification of a granular model system of polystyrene spheres over time by shaking with varying excitation amplitudes or effective temperatures. This densification is quantified by the mean-square displacement (MSD), which is measured by diffuse wave spectroscopy (DWS) of a sinusoidally excited vibrating fluidized granular bed. The DWS method also extracts the inherent heterogeneous dynamics of the system in the bulk and at the wall. Through an empirical model-based extraction, we obtain the ballistic and diffusive time constants, as well as caging sizes, which were found to depend on temperature and density. The results obtained from this study reveal a subdiffusive power-law behavior in the MSD, indicating an arrest of motion and potentially a glassy system, especially in cases where the excitation is low to moderate compared to gravity. The extracted MSD caging sizes are two orders smaller than the Lindeman length found in colloidal systems.
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References (64)
- H. M. Jaeger, S. R. Nagel, and R. P. Behringer, Granular solids, liquids, and gases, Rev. Mod. Phys. 68, 1259 (1996).
- B. Andreotti, Y. Forterre, and O. Pouliquen, Granular Media: Between Fluid and Solid (Cambridge University Press, Cambridge, 2013).
- J. Duran, Sands, Powders, and Grains: An Introduction to the Physics of Granular Materials (Springer Science & Business Media, New York, 2012).
- A. D. Rosato and C. Windows-Yule, Segregation in Vibrated Granular Systems (Academic Press, New York, 2020).
- A. J. Liu and S. R. Nagel, Jamming is not just cool any more, Nature (London) 396, 21 (1998).
- L. Berthier and G. Biroli, Glasses and aging, a statistical mechanics perspective on (Springer, Berlin, 2009).
- A.-L. Barabási, R. Albert, and P. Schiffer, The physics of sand castles: Maximum angle of stability in wet and dry granular media, Physica A 266, 366 (1999).
- I. Tomasetta, D. Barletta, and M. Poletto, Correlation of powder flow properties to interparticle interactions at ambient and high temperatures, Particuology 12, 90 (2014).
- E. Ehrichs, H. Jaeger, G. S. Karczmar, J. B. Knight, V. Y. Kuperman, and S. R. Nagel, Granular convection observed by magnetic resonance imaging, Science 267, 1632 (1995).
- R. D. Wildman, J. M. Huntley, and D. J. Parker, Granular temperature profiles in three-dimensional vibrofluidized granular beds, Phys. Rev. E 63, 061311 (2001).
- B. J. Berne and R. Pecora, Dynamic Light Scattering: With Applications to Chemistry, Biology, and Physics (Courier Corporation, Toronto, 2000).
- E. M. Furst and T. M. Squires, Microrheology (Oxford University Press, Oxford, 2017).
- N. Menon and D. J. Durian, Diffusing-wave spectroscopy of dynamics in a three-dimensional granular flow, Science 275, 1920 (1997).
- N. Menon and D. J. Durian, Particle motions in a gas-fluidized bed of sand, Phys. Rev. Lett. 79, 3407 (1997).
- M. J. Biggs, D. Glass, L. Xie, V. Zivkovic, A. Buts, and M. Curt Kounders, Granular temperature in a gas fluidized bed, Granul. Matter 10, 63 (2008).
- C. Hanotin, P. Marchal, L. J. Michot, C. Baravian, and S. K. de Richter, Dynamics of vibrated granular suspensions probed by mechanical spectroscopy and diffusing wave spectroscopy measurements, Soft Matter 9, 9352 (2013).
- C. Hanotin, S. Kiesgen de Richter, L. Michot, and P. Marchal, Viscoelasticity of vibrated granular suspensions, J. Rheol. 59, 253 (2015).
- K. Kim, J. J. Park, J. K. Moon, H. K. Kim, and H. K. Pak, Solid-liquid transition in a highly dense 3D vibro-fluidized granular system, J. Korean Phys. Soc. 40, 983 (2002).
- K. Kim, J. K. Moon, J. J. Park, H. K. Kim, and H. K. Pak, Jamming transition in a highly dense granular system under vertical vibration, Phys. Rev. E 72, 011302 (2005).
- V. Zivkovic, M. J. Biggs, and D. Glass, Scaling of granular temperature in a vibrated granular bed, Phys. Rev. E 83, 031308 (2011).
- T. Blochowicz, Jamming in granularen medien, Grundpraktikumsanleitung TU Darmstadt, University of Darmstadt (2015).
- C. Mayo, M. Kunzner, M. Sperl, and J. P. Gabriel, Observing the glass and jamming transitions of dense granular material in microgravity, arXiv:2504.04161.
- S. Garland, G. Gauthier, J. Martin, and J. Morris, Normal stress measurements in sheared non-Brownian suspensions, J. Rheo. 57, 71 (2013).
- A. Schella, S. Herminghaus, and M. Schröter, Influence of humidity on tribo-electric charging and segregation in shaken granular media, Soft Matter 13, 394 (2017).
- J. Schindelin, I. Arganda-Carreras, E. Frise, V. Kaynig, M. Longair, T. Pietzsch, S. Preibisch, C. Rueden, S. Saalfeld, B. Schmid et al., Fiji: An open-source platform for biological-image analysis, Nat. Methods 9, 676 (2012).
- P. Evesque, E. Szmatula, and J.-P. Denis, Surface fluidization of a sand pile, Europhys. Lett. 12, 623 (1990).
- S. Douady, S. Fauve, and C. Laroche, Subharmonic instabilities and defects in a granular layer under vertical vibrations, Europhys. Lett. 8, 621 (1989).
- P. Eshuis, K. Van Der Weele, D. Van Der Meer, R. Bos, and D. Lohse, Phase diagram of vertically shaken granular matter, Phys. Fluids 19, 123301 (2007).
- C. Laroche, S. Douady, and S. Fauve, Convective flow of granular masses under vertical vibrations, J. Physique 50, 699 (1989).
- M. Schröter, A local view on the role of friction and shape, in EPJ Web of Conferences (EDP Sciences, 2017), Vol. 140, p. 01008.
- W. Brown, Dynamic Light Scattering (Clarendon Press, 1993), Chap. 16.
- D. Weitz, J. Zhu, D. Durian, H. Gang, and D. Pine, Diffusing-wave spectroscopy: The technique and some applications, Phys. Scr. 1993, 610 (1993).
- S. Utermann, Friction and diffusive light transport in a granular medium, Ph.D. thesis, Georg-August-Universität Göttingen, 2012, http://hdl.handle.net/11858/00-1735-0000-0006-B54C-1.
- G. Mie, Beiträge zur Optik trüber Medien, speziell kolloidaler Metallösungen, Ann. Phys. 330, 377 (1908).
- B. J. Sumlin, W. R. Heinson, and R. K. Chakrabarty, Retrieving the aerosol complex refractive index using pymiescatt: A Mie computational package with visualization capabilities, J. Quant. Spectrosc. Radiat. Transfer 205, 127 (2018).
- H. Hertz, Über die Berührung fester elastischer Körper, J. Reine Angew. Math. 92, 156 (1881).
- N. V. Brilliantov, F. Spahn, J.-M. Hertzsch, and T. Pöschel, Model for collisions in granular gases, Phys. Rev. E 53, 5382 (1996).
- K. L. Johnson, One hundred years of Hertz contact, Proc. Inst. Mech. Eng. 196, 363 (1982).
- J.-F. Camenen, Y. Descantes, and P. Richard, Effect of confinement on dense packings of rigid frictionless spheres and polyhedra, Phys. Rev. E 86, 061317 (2012).
- J. B. Knight, C. G. Fandrich, C. N. Lau, H. M. Jaeger, and S. R. Nagel, Density relaxation in a vibrated granular material, Phys. Rev. E 51, 3957 (1995).
- E. R. Nowak, J. B. Knight, E. Ben-Naim, H. M. Jaeger, and S. R. Nagel, Density fluctuations in vibrated granular materials, Phys. Rev. E 57, 1971 (1998).
- G. R. Farrell, K. M. Martini, and N. Menon, Loose packings of frictional spheres, Soft Matter 6, 2925 (2010).
- T. Itakura, H. Masuda, C. Ohtsuka, and S. Matsusaka, The contact potential difference of powder and the tribo-charge, J. Electrost. 38, 213 (1996).
- L.-S. Lu and S.-S. Hsiau, Mixing in vibrated granular beds with the effect of electrostatic force, Powder Technol. 160, 170 (2005).
- G. L. Hunter and E. R. Weeks, The physics of the colloidal glass transition, Rep. Prog. Phys. 75, 066501 (2012).
- W. van Megen and H. Schöpe, The cage effect in systems of hard spheres, J. Phys. Chem. 146, 104503 (2017).
- Z. Xing, A. Caciagli, T. Cao, I. Stoev, M. Zupkauskas, T. O'Neill, T. Wenzel, R. Lamboll, D. Liu, and E. Eiser, Microrheology of DNA hydrogels, Proc. Natl. Acad. Sci. USA 115, 8137 (2018).
- F. Cardinaux, L. Cipelletti, F. Scheffold, and P. Schurtenberger, Microrheology of giant-micelle solutions, Europhys. Lett. 57, 738 (2002).
- M. Gruber, G. Abade, A. Puertas, and M. Fuchs, Active icrorheology in a colloidal glass, Phys. Rev. E 94, 042602 (2016).
- F. Pabst, J. P. Gabriel, T. Boehmer, P. Weigl, A. Helbling, T. Richter, P. Zourchang, T. Walther, and T. Blochowicz, Generic structural relaxation in supercooled liquids, J. Phys. Chem. Lett. 12, 3685 (2021).
- T. Böhmer, F. Pabst, J. P. Gabriel, R. Zeißler, and T. Blochowicz, On the spectral shape of the structural relaxation in supercooled liquids, J. Chem. Phys. 162 (2025).
- J. H. van Zanten, S. Amin, and A. A. Abdala, Brownian motion of colloidal spheres in aqueous PEO solutions, Macromolecules 37, 3874 (2004).
- F. P. Bowden and D. Tabor, Friction: An Introduction to Tribology (R. E. Krieger Publishing Company, 1982).
- G.-J. Gao, J. Blawzdziewicz, C. S. O'Hern, and M. Shattuck, Experimental demonstration of nonuniform frequency distributions of granular packings, Phys. Rev. E 80, 061304 (2009).
- V. Tournat, V. Zaitsev, V. Gusev, V. Nazarov, P. Béquin, and B. Castagnede, Probing weak forces in granular media through nonlinear dynamic dilatancy: Clapping contacts and polarization anisotropy, Phys. Rev. Lett. 92, 085502 (2004).
- S. van den Wildenberg, M. van Hecke, and X. Jia, Evolution of granular packings by nonlinear acoustic waves, Europhys. Lett. 101, 14004 (2013).
- A. Mathey, M. L. Fur, P. Chasle, A. Amon, and J. Crassous, A device for studying elementary plasticity fluctuations in granular media, arXiv:2403.09396.
- C. Scalliet, A. Gnoli, A. Puglisi, and A. Vulpiani, Cages and anomalous diffusion in vibrated dense granular media, Phys. Rev. Lett. 114, 198001 (2015).
- P. V. Rysselberghe, Remarks concerning the Clausius-Mossotti law, J. Phys. Chem. 36, 1152 (2002).
- S. K. Nayar, I. Katsushi, and T. Kanade, Surface Reflection: Physical and Geometrical Perspectives (Carnegie Mellon University, 1989).
- D. Geldart, Types of gas fluidization, Powder Technol. 7, 285 (1973).
- M. Sperl, Nearly logarithmic decay in the colloidal hard-sphere system, Phys. Rev. E 71, 060401(R) (2005).
- M. Sperl, W. T. Kranz, and A. Zippelius, Single-particle dynamics in dense granular fluids under driving, Europhys. Lett. 98, 28001 (2012).
- F. A. Lindemann, Über die Berechnung molekularer Eigenfrequenzen, Phys. Z 11, 609 (1910).