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  • Letter
  • Open Access

Fluctuation corrections to Lifshitz tails in disordered systems

Enrique Rozas Garcia1,* and Johannes Hofmann1,2,†

  • 1Department of Physics, Gothenburg University, 41296 Gothenburg, Sweden
  • 2Nordita, Stockholm University and KTH Royal Institute of Technology, 10691 Stockholm, Sweden

  • *enrique.rozas.garcia@physics.gu.se
  • †johannes.hofmann@physics.gu.se

Phys. Rev. E 109, L032103 – Published 7 March, 2024

DOI: https://doi.org/10.1103/PhysRevE.109.L032103

Abstract

Quenched disorder in semiconductors induces localized electronic states at the band edge, which manifest as an exponential tail in the density of states. For large impurity densities, this tail takes a universal Lifshitz form that is characterized by short-ranged potential fluctuations. We provide both analytical expressions and numerical values for the Lifshitz tail of a parabolic conduction band including its exact fluctuation prefactor. Our analysis is based on a replica field integral approach, where the leading exponential scaling of the tail is determined by an instanton profile and fluctuations around the instanton determine the subleading preexponential factor. This factor contains the determinant of a fluctuation operator, and we avoid a full computation of its spectrum by using a Gel'fand-Yaglom formalism, which provides a concise general derivation of fluctuation corrections in disorder problems. We provide a revised result for the disorder band tail in two dimensions.

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References (55)

  1. P. Van Mieghem, Rev. Mod. Phys. 64, 755 (1992).
  2. E. P. George, D. Raabe, and R. O. Ritchie, Nat. Rev. Mater. 4, 515 (2019).
  3. M. Mézard, G. Parisi, and M. A. Virasoro, Spin Glass Theory and Beyond: An Introduction to the Replica Method and Its Applications (World Scientific, Singapore, 1987), Vol. 9.
  4. N. E. Cusack and D. L. Stein, The Physics of Structurally Disordered Matter: An Introduction (American Institute of Physics, Woodbury, NY, 1988).
  5. D. S. Wiersma, Nat. Photon. 7, 188 (2013).
  6. S. Yu, C.-W. Qiu, Y. Chong, S. Torquato, and N. Park, Nat. Rev. Mater. 6, 226 (2021).
  7. G. Roati, C. D'Errico, L. Fallani, M. Fattori, C. Fort, M. Zaccanti, G. Modugno, M. Modugno, and M. Inguscio, Nature (London) 453, 895 (2008).
  8. J. Billy, V. Josse, Z. Zuo, A. Bernard, B. Hambrecht, P. Lugan, D. Clément, L. Sanchez-Palencia, P. Bouyer, and A. Aspect, Nature (London) 453, 891 (2008).
  9. M. Shur and M. Hack, J. Appl. Phys. 55, 3831 (1984).
  10. M. A. Khayer and R. K. Lake, J. Appl. Phys. 110, 074508 (2011).
  11. J. Jean, T. S. Mahony, D. Bozyigit, M. Sponseller, J. Holovský, M. G. Bawendi, and V. Bulović, ACS Energy Lett. 2, 2616 (2017).
  12. J. Wong, S. T. Omelchenko, and H. A. Atwater, ACS Energy Lett. 6, 52 (2021).
  13. N. F. Mott, Philos. Mag. 19, 835 (1969).
  14. E. Economou, M. H. Cohen, K. F. Freed, and E. Kirkpatrick, Amorphous and Liquid Semiconductors (Springer, Berlin, 1974), pp. 101–158.
  15. D. J. Thouless, Phys. Rep. 13, 93 (1974).
  16. N. Mott, Int. Rev. Phys. Chem. 4, 1 (1985).
  17. I. Lifshitz, Sov. Phys. JETP 17, 1159 (1963).
  18. I. Lifshitz, Adv. Phys. 13, 483 (1964).
  19. B. I. Halperin, Phys. Rev. 139, A104 (1965).
  20. B. I. Halperin and M. Lax, Phys. Rev. 148, 722 (1966).
  21. B. Halperin and M. Lax, Phys. Rev. 153, 802 (1967).
  22. J. Zittartz and J. S. Langer, Phys. Rev. 148, 741 (1966).
  23. J. Meibohm and M. Esposito, New J. Phys. 25, 023034 (2023).
  24. J. Meibohm, K. Gustavsson, and B. Mehlig, Phys. Rev. Fluids 8, 024305 (2023).
  25. S. John and M. Stephen, J. Phys. C: Solid State Phys. 17, L559 (1984).
  26. I. Affleck, J. Phys. C: Solid State Phys. 16, 5839 (1983).
  27. S. Yaida, Phys. Rev. B 93, 075120 (2016).
  28. P. Stollmann, Caught by Disorder: Bound States in Random Media (Springer, Berlin, 2001), Vol. 20.
  29. O. Khorunzhiy, W. Kirsch, and P. Müller, Ann. Appl. Probab. 16, 295 (2006).
  30. M. Gebert and C. Rojas-Molina, Ann. Henri Poincaré 23, 4149 (2022).
  31. E. Brézin and G. Parisi, J. Phys. C: Solid State Phys. 13, L307 (1980).
  32. E. Brézin and G. Parisi, J. Stat. Phys. 19, 269 (1978).
  33. E. Brézin, J. C. Le Guillou, and J. Zinn-Justin, Phys. Rev. D 15, 1544 (1977).
  34. M. Mariño, Instantons and Large N: An Introduction to Non-Perturbative Methods in Quantum Field Theory (Cambridge University Press, Cambridge, UK, 2015).
  35. I. M. Gel'fand and A. M. Yaglom, J. Math. Phys. 1, 48 (1960).
  36. S. Levit and U. Smilansky, Proc. Am. Math. Soc. 65, 299 (1977).
  37. S. F. Edwards and R. C. Jones, J. Phys. A: Math. Gen. 9, 1595 (1976).
  38. G. Livan, M. Novaes, and P. Vivo, Introduction to Random Matrices: Theory and Practice, Springer Briefs in Mathematical Physics (Springer, Berlin, 2018), Vol. 63.
  39. C. G. Callan Jr. and S. Coleman, Phys. Rev. D 16, 1762 (1977).
  40. J. L. Cardy, J. Phys. C: Solid State Phys. 11, L321 (1978).
  41. J. Zinn-Justin, Quantum Field Theory and Critical Phenomena, 4th ed., International Series of Monographs on Physics (Clarendon Press, Oxford, UK, 2002), Vol. 113.
  42. S. F. Edwards and P. W. Anderson, J. Phys. F: Met. Phys. 5, 965 (1975).
  43. C. M. Bender, S. Orszag, and S. A. Orszag, Advanced Mathematical Methods for Scientists and Engineers I: Asymptotic Methods and Perturbation Theory (Springer, Berlin, 1999).
  44. A. Altland and B. D. Simons, Condensed Matter Field Theory, 2nd ed. (Cambridge University Press, Cambridge, UK, 2010).
  45. D. J. Thouless and M. E. Elzain, J. Phys. C: Solid State Phys. 11, 3425 (1978).
  46. S. Coleman, V. Glaser, and A. Martin, Commun. Math. Phys. 58, 211 (1978).
  47. See Supplemental Material at http://link.aps.org/supplemental/10.1103/PhysRevE.109.L032103 for details, which includes Ref. [55].
  48. S. Coleman, Aspects of Symmetry: Selected Erice Lectures (Cambridge University Press, Cambridge, UK, 1985).
  49. R. Rajaraman, Solitons and Instantons: An Introduction to Solitons and Instantons in Quantum Field Theory (North-Holland, Amsterdam, 1982).
  50. G. V. Dunne and K. Kirsten, J. Phys. A: Math. Gen. 39, 11915 (2006).
  51. K. Kirsten and A. J. McKane, J. Phys. A: Math. Gen. 37, 4649 (2004).
  52. G. V. Dunne, J. Phys. A: Math. Theor. 41, 304006 (2008).
  53. K. Kirsten and P. Loya, Am. J. Phys. 76, 60 (2008).
  54. G. V. Dunne and H. Min, Phys. Rev. D 72, 125004 (2005).
  55. M. J. Ablowitz and Z. H. Musslimani, Opt. Lett. 30, 2140 (2005).

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