Export citation

Export citation

Choose format for download:

Download Citation
  • Letter

Interplay between percolation and glassiness in the random Lorentz gas

Giulio Biroli1, Patrick Charbonneau2,3, Eric I. Corwin4, Yi Hu2,*, Harukuni Ikeda5, Grzegorz Szamel6, and Francesco Zamponi1

  • 1Laboratoire de Physique de l'Ecole Normale Supérieure, ENS, Université PSL, CNRS, Sorbonne Université, Université de Paris, F-75005 Paris, France
  • 2Department of Chemistry, Duke University, Durham, North Carolina 27708, USA
  • 3Department of Physics, Duke University, Durham, North Carolina 27708, USA
  • 4Department of Physics and Material Science Institute, University of Oregon, Eugene, Oregon 97403, USA
  • 5Graduate School of Arts and Sciences, The University of Tokyo, Tokyo 153-8902, Japan
  • 6Department of Chemistry, Colorado State University, Fort Collins, Colorado 80523, USA

  • *yi.hu@duke.edu

Phys. Rev. E 103, L030104 – Published 17 March, 2021

DOI: https://doi.org/10.1103/PhysRevE.103.L030104

Abstract

The random Lorentz gas (RLG) is a minimal model of transport in heterogeneous media that exhibits a continuous localization transition controlled by void space percolation. The RLG also provides a toy model of particle caging, which is known to be relevant for describing the discontinuous dynamical transition of glasses. In order to clarify the interplay between the seemingly incompatible percolation and caging descriptions of the RLG, we consider its exact mean-field solution in the infinite-dimensional d→∞ limit and perform numerics in d=2...20. We find that for sufficiently high d the mean-field caging transition precedes and prevents the percolation transition, which only happens on timescales diverging with d. We further show that activated processes related to rare cage escapes destroy the glass transition in finite dimensions, leading to a rich interplay between glassiness and percolation physics. This advance suggests that the RLG can be used as a toy model to develop a first-principle description of particle hopping in structural glasses.

Physics Subject Headings (PhySH)

Authorization Required

We need you to provide your credentials before accessing this content.

Supplemental Material (Subscription Required)

References (Subscription Required)

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation