Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Particle detection using magnetic avalanches in single-molecule magnet crystals

Bailey Kohn1,*, Hao Chen1,2,†, Rupak Mahapatra1,‡, Glenn Agnolet1, Ivan Borzenets1, Philip C. Bunting3, Jeffrey R. Long4,5, Minjie Lu1, Tom Melia6 et al.

Michael Nippe7, Lok Raj Pant1, Surjeet Rajendran8, Anna Schmautz7, and Amis Sharma1

  • *Contact author: b.pickard17@tamu.edu
  • †Contact author: chenhao_fd@fudan.edu.cn
  • ‡Contact author: mahapatra@physics.tamu.edu

Phys. Rev. D 114, 012014 – Published 17 July, 2026

DOI: https://doi.org/10.1103/r1x8-qc2f

Abstract

The detection of a single quantum of energy with high efficiency and a low false positive rate is of considerable scientific interest, from serving as single quantum sensors of optical and infrared photons to enabling the direct detection of low-mass dark matter. We confirm our initial experimental demonstration of magnetic avalanches induced by scattering of quanta in single-molecule magnet (SMM) crystals made of Mn12 acetate, establishing the use of SMMs as particle detectors for the first time. Although the current setup has an energy threshold in the MeV regime, our results motivate the exploration of a wide variety of SMMs whose properties could allow for detection of sub-eV energy depositions.

View figure in article

Physics Subject Headings (PhySH)

Article Text

References (46)

  1. S. Komiyama, O. Astafiev, V. Antonov, T. Kutsuwa, and H. Hiral, A single-photon detector in the far-infrared range, Nature (London) 403, 405 (2000).
  2. A. E. Lita, A. J. Miller, and S. W. Nam, Counting near-infrared single-photons with 95% efficiency, Opt. Express 16, 3032 (2008).
  3. M. D. Eisaman, J. Fan, A. Migdall, and S. V. Polyakov, Invited review article: Single-photon sources and detectors, Rev. Sci. Instrum. 82, 071101 (2011).
  4. T. D. Ladd, F. Jelezko, R. Laflamme, Y. Nakamura, C. Monroe, and J. L. O’Brien, Quantum computers, Nature (London) 464, 45 (2010).
  5. E. Knill, R. Laflamme, and G. J. Milburn, A scheme for efficient quantum computation with linear optics, Nature (London) 409, 46 (2001).
  6. Z. Hong, R. Ren, N. Kurinsky, E. Figueroa-Feliciano, L. Wills, S. Ganjam, R. Mahapatra, N. Mirabolfathi, B. Nebolsky, H. Pinckney, and M. Platt, Single electron-hole pair sensitive silicon detector with surface event discrimination, Nucl. Instrum. Methods Phys. Res., Sect. A 963, 163757 (2020).
  7. X. Rong, M. Wang, J. Geng, X. Qin, M. Guo, M. Jiao, Y. Xie, P. Wang, p. Huang, F. Shi, Y.-F. Cai, C. Zou, and J. Du, Searching for an exotic spin-dependent interaction with a single electron-spin quantum sensor, Nat. Commun. 9, 739 (2018).
  8. P. C. Bunting, G. Gratta, T. Melia, and S. Rajendran, Magnetic bubble chambers and sub-GeV dark matter direct detection, Phys. Rev. D 95, 095001 (2017).
  9. M. J. Dolan, F. Kahlhoefer, and C. McCabe, Directly detecting sub-GeV dark matter with electrons from nuclear scattering, Phys. Rev. Lett. 121, 101801 (2018).
  10. M. Battaglieri et al., US cosmic visions: New ideas in dark matter 2017: Community report, in U.S. Cosmic Visions: New Ideas in Dark Matter College Park, MD, USA, 2017(2017), arXiv:1707.04591.
  11. P. W. Graham, J. Mardon, and S. Rajendran, Vector dark matter from inflationary fluctuations, Phys. Rev. D 93, 103520 (2016).
  12. T. K. Bui et al. (TESSERACT Collaboration), First limits on light dark matter interactions in a low threshold two-channel Athermal Phonon Detector from the tesseract collaboration, Phys. Rev. Lett. 135, 161002 (2025).
  13. A. H. Abdelhameed et al. (CRESST Collaboration), First results from the cresst-III low-mass dark matter program, Phys. Rev. D 100, 102002 (2019).
  14. G. Angloher et al. (CRESST Collaboration), Results on sub-GeV dark matter from a 10 eV threshold cresst-III silicon detector, Phys. Rev. D 107, 122003 (2023).
  15. E. Armengaud et al. (EDELWEISS Collaboration), Searching for low-mass dark matter particles with a massive Ge bolometer operated above ground, Phys. Rev. D 99, 082003 (2019).
  16. I. Alkhatib et al. (SuperCDMS Collaboration), Light dark matter search with a high-resolution athermal phonon detector operated above ground, Phys. Rev. Lett. 127, 061801 (2021).
  17. I. Arnquist et al. (DAMIC-M Collaboration), First constraints from damic-m on sub-GeV dark-matter particles interacting with electrons, Phys. Rev. Lett. 130, 171003 (2023).
  18. O. Abramoff, L. Barak, I. M. Bloch, L. Chaplinsky, M. Crisler, Dawa, A. Drlica-Wagner, R. Essig, J. Estrada, E. Etzion, G. Fernandez, D. Gift, M. Sofo-Haro, J. Taenzer, J. Tiffenberg, T. Volansky, and T.-T. Yu (SENSEI Collaboration), Sensei: Direct-detection constraints on sub-GeV dark matter from a shallow underground run using a prototype skipper CCD, Phys. Rev. Lett. 122, 161801 (2019).
  19. H. Neog, R. Mahapatra, N. Mirabolfathi, M. Platt, A. Jastram, G. Agnolet, H. Chen, B. Mohanty, and A. Kubik, Phonon-mediated high-voltage detector with background rejection for low-mass dark matter and reactor coherent neutrino scattering experiments, Nucl. Instrum. Methods Phys. Res., Sect. A 1033, 166707 (2022).
  20. G. Chesi, L. Malinverno, A. Allevi, R. Santoro, M. Caccia, A. Martemiyanov, and M. Bondani, Optimizing Silicon photomultipliers for quantum optics, Sci. Rep. 9, 1 (2019).
  21. O. Knopfmacher, M. L. Hammock, A. L. Appleton, G. Schwartz, J. Mei, T. Lei, J. Pei, and Z. Bao, Highly stable organic polymer field-effect transistor sensor for selective detection in the marine environment, Nat. Commun. 5, 2954 (2014).
  22. S. Sorgenfrei, C. Y. Chiu, R. L. Gonzalez, Y. J. Yu, P. Kim, C. Nuckolls, and K. L. Shepard, Label-free single-molecule detection of DNA-hybridization kinetics with a carbon nanotube field-effect transistor, Nat. Nanotechnol. 6, 126 (2011).
  23. C. Amole et al. (PICO Collaboration), Dark matter search results from the complete exposure of the PICO-60 C3F8 bubble chamber, Phys. Rev. D 100, 022001 (2019).
  24. R. Sessoli, D. Gatteschi, A. Caneschi, and M. A. Novak, Magnetic bistability in a metal-ion cluster, Nature (London) 365, 141 (1993).
  25. T. Lis, Preparation, structure, and magnetic properties of a dodecanuclear mixed-valence manganese carboxylate, Acta Crystallogr. Sect. B 36, 2042 (1980).
  26. L. Bogani and W. Wernsdorfer, Molecular quantum spintronics using single-molecule magnets, Nat. Mater. 7, 179 (2008).
  27. M. Leuenberger and D. Loss, Quantum computing in molecular magnets, Nature (London) 410, 789 (2001).
  28. A.-L. Barra, P. Debrunner, D. Gatteschi, C. E. Schulz, and R. Sessoli, Superparamagnetic-like behavior in an octanuclear iron cluster, Europhys. Lett. 35, 133 (1996).
  29. C. Paulsen and J.-G. Park, Evidence for quantum tunneling of the magnetization in MN12A C, in Quantum Tunneling of Magnetization—QTM ’94, edited by L. Gunther and B. Barbara (Springer Netherlands, Dordrecht, 1995), pp. 189–207.
  30. Y. Suzuki, M. P. Sarachik, E. M. Chudnovsky, S. McHugh, R. Gonzalez-Rubio, N. Avraham, Y. Myasoedov, E. Zeldov, H. Shtrikman, N. E. Chakov, and G. Christou, Propagation of avalanches in Mn12-acetate: Magnetic deflagration, Phys. Rev. Lett. 95, 147201 (2005).
  31. T. Leviant, A. Keren, E. Zeldov, and Y. Myasoedov, Quantum ignition of deflagration in the Fe8 molecular magnet, Phys. Rev. B 90, 134405 (2014).
  32. D. A. Garanin and E. M. Chudnovsky, Theory of magnetic deflagration in crystals of molecular magnets, Phys. Rev. B 76, 054410 (2007).
  33. S. Velez, J. M. Hernandez, A. Fernandez, F. Macià, C. Magen, P. A. Algarabel, J. Tejada, and E. M. Chudnovsky, Magnetic deflagration in Gd5Ge4, Phys. Rev. B 81, 064437 (2010).
  34. A. Hernández-Mínguez, J. M. Hernandez, F. Macià, A. García-Santiago, J. Tejada, and P. V. Santos, Quantum magnetic deflagration in Mn12 acetate, Phys. Rev. Lett. 95, 217205 (2005).
  35. F. Macià, A. Hernández-Mínguez, G. Abril, J. M. Hernandez, A. García-Santiago, J. Tejada, F. Parisi, and P. V. Santos, Observation of phonon-induced magnetic deflagration in manganites, Phys. Rev. B 76, 174424 (2007).
  36. S. McHugh, R. Jaafar, M. P. Sarachik, Y. Myasoedov, A. Finkler, H. Shtrikman, E. Zeldov, R. Bagai, and G. Christou, Effect of quantum tunneling on the ignition and propagation of magnetic avalanches in Mn12 acetate, Phys. Rev. B 76, 172410 (2007).
  37. P. Subedi, S. Vélez, F. Macià, S. Li, M. P. Sarachik, J. Tejada, S. Mukherjee, G. Christou, and A. D. Kent, Onset of a propagating self-sustained spin reversal front in a magnetic system, Phys. Rev. Lett. 110, 207203 (2013).
  38. H. An, M. Pospelov, J. Pradler, and A. Ritz, Direct detection constraints on dark photon dark matter, Phys. Lett. B 747, 331 (2015).
  39. H. Chen, R. Mahapatra, G. Agnolet, M. Nippe, M. Lu, P. C. Bunting, T. Melia, S. Rajendran, G. Gratta, and J. Long, Quantum detection using magnetic avalanches in single-molecule magnets, arXiv:2002.09409.
  40. H. Chen, Magnetic bubble chamber prototype development, Ph.D. thesis, Texas A&M University, 2019.
  41. J. M. North, Synthesis and characterization of single-molecule magnets: Mn12-acetate, Fe8Br8, and analogs, Ph.D. thesis, The Florida State University, 2004.
  42. A. Zabala-Lekuona, J. M. Seco, and E. Colacio, Single-molecule magnets: From MN12-AC to dysprosium metallocenes, a travel in time, Coord. Chem. Rev. 441, 213984 (2021).
  43. J. R. Friedman and M. P. Sarachik, Single-molecule nanomagnets, Annu. Rev. Condens. Matter Phys. 1, 109 (2010).
  44. G. Jungman, M. Kamionkowski, and K. Griest, Supersymmetric dark matter, Phys. Rep. 267, 195 (1996).
  45. M. Manoli, R. Inglis, M. J. Manos, V. Nastopoulos, W. Wernsdorfer, E. K. Brechin, and A. J. Tasiopoulos, A [mn32] double-decker wheel, Angew. Chem., Int. Ed. 50, 4441 (2011).
  46. I. Borzents, B. Kohn, R. Mahapatra, L. R. Pant, and A. Sharma, Particle induced magnetic avalanche data in mn12-ac taken in spring 2025 (2026).

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation