- Open Access
Direct dark matter searches with metal halide perovskites
Phys. Rev. D 112, 092005 – Published 10 November, 2025
DOI: https://doi.org/10.1103/qzlg-3dp3
Abstract
Polar materials with optical phonons in the meV range are excellent candidates for both dark matter direct detection via dark photon-mediated scattering and light dark matter absorption. In this study, we propose, for the first time, the metal halide perovskites , , and for these purposes. Our findings reveal that is the best material, significantly improving exclusion limits compared to other polar materials. For scattering, can probe dark matter masses down to the keV range. For absorption, it enhances sensitivity to detect dark photon masses below . The only material that has so far been investigated and that could provide competitive bounds is CsI, which, however, demonstrates lower stability as device platform compared to . Moreover, CsI is isotropic while the anisotropic structure of enables daily modulation analysis, showing that a significant percentage of daily modulation exceeding 1% is achievable for dark matter masses below 40 keV.
Physics Subject Headings (PhySH)
Article Text
References (71)
- E. Aprile (The XENON Collaboration), Phys. Rev. Lett. 123, 251801 (2019).
- L. J. Hall, K. Jedamzik, J. March-Russell, and S. M. West, J. High Energy Phys. 03 (2010) 080.
- N. Bernal, M. Heikinheimo, T. Tenkanen, K. Tuominen, and V. Vaskonen, Int. J. Mod. Phys. A 32, 1730023 (2017).
- D. Hooper and K. M. Zurek, Phys. Rev. D 77, 087302 (2008).
- J. L. Feng and J. Kumar, Phys. Rev. Lett. 101, 231301 (2008).
- T. Cohen, D. J. Phalen, A. Pierce, and K. M. Zurek, Phys. Rev. D 82, 056001 (2010).
- K. Schutz and K. M. Zurek, Phys. Rev. Lett. 117, 121302 (2016).
- S. Knapen, T. Lin, and K. M. Zurek, Phys. Rev. D 95, 056019 (2017).
- A. Caputo, A. Esposito, and A. D. Polosa, Phys. Rev. D 100, 116007 (2019).
- G. Baym, D. H. Beck, J. P. Filippini, C. J. Pethick, and J. Shelton, Phys. Rev. D 102, 035014 (2020).
- A. Caputo, A. Esposito, F. Piccinini, A. D. Polosa, and G. Rossi, Phys. Rev. D 103, 055017 (2021).
- S. Griffin, S. Knapen, T. Lin, and K. M. Zurek, Phys. Rev. D 98, 115034 (2018).
- S. M. Griffin, K. Inzani, T. Trickle, Z. Zhang, and K. M. Zurek, Phys. Rev. D 101, 055004 (2020).
- B. Campbell-Deem, P. Cox, S. Knapen, T. Lin, and T. Melia, Phys. Rev. D 102, 019904 (2020).
- S. M. Griffin, Y. Hochberg, K. Inzani, N. Kurinsky, T. Lin, and T. C. Yu, Phys. Rev. D 103, 075002 (2021).
- T. Trickle, Z. Zhang, and K. M. Zurek, arXiv:2009.13534.
- Y. Kahn, G. Krnjaic, and B. Mandava, Phys. Rev. Lett. 127, 081804 (2021).
- S. Knapen, J. Kozaczuk, and T. Lin, Phys. Rev. Lett. 127, 081805 (2021).
- F. Acanfora, A. Esposito, and A. D. Polosa, Eur. Phys. J. C 79, 549 (2019).
- T. Trickle, Z. Zhang, K. M. Zurek, K. Inzani, and S. M. Griffin, J. High Energy Phys. 03 (2020) 036.
- F. Paolucci and F. Giazotto, Instruments 5, 14 (2021).
- F. Paolucci, V. Buccheri, G. Germanese, N. Ligato, R. Paoletti, G. Signorelli, M. Bitossi, P. Spagnolo, P. Falferi, M. Rajteri, C. Gatti, and F. Giazotto, J. Appl. Phys. 128, 194502 (2020).
- R. M. Geilhufe, F. Kahlhoefer, and M. W. Winkler, Phys. Rev. D 101, 055005 (2020).
- A. Coskuner, A. Mitridate, A. Olivares, and K. M. Zurek, Phys. Rev. D 103, 016006 (2021).
- A. Coskuner, T. Trickle, Z. Zhang, and K. M. Zurek, Phys. Rev. D 105, 015010 (2022).
- L. M. Herz, ACS Energy Lett. 2, 1539 (2017).
- K. Freese, J. Frieman, and A. Gould, Phys. Rev. D 37, 3388 (1988).
- A. K. Drukier, K. Freese, and D. N. Spergel, Phys. Rev. D 33, 3495 (1986).
- P. Toloueinia, H. Khassaf, A. Shirazi Amin, Z. M. Tobin, S. P. Alpay, and S. L. Suib, ACS Appl. Energy Mater. 3, 8240 (2020).
- R. Montecucco, E. Quadrivi, R. Po, and G. Grancini, Adv. Energy Mater. 11, 2100672 (2021).
- N. Taufertshöfer, M. Garcia-Sciveres, and S. M. Griffin, Phys. Rev. D 110, 103552 (2024).
- J. Lewin and P. Smith, Astropart. Phys. 6, 87 (1996).
- R. Catena and P. Ullio, J. Cosmol. Astropart. Phys. 08 (2010) 004.
- P. Salucci, F. Nesti, G. Gentile, and C. F. Martins, Astron. Astrophys. 523, A83 (2010).
- S. Knapen, T. Lin, and K. M. Zurek, Phys. Rev. D 96, 115021 (2017).
- T. Trickle, Z. Zhang, and K. M. Zurek, Phys. Rev. D 105, 015001 (2022).
- S. Knapen, J. Kozaczuk, and T. Lin, Phys. Rev. D 105, 015014 (2022).
- F. Gervais and B. Piriou, J. Phys. C 7, 2374 (1974).
- S. Zollner, P. P. Paradis, F. Abadizaman, and N. S. Samarasingha, J. Vac. Sci. Technol. B 37, 012904 (2019).
- H. Fröhlich, Adv. Phys. 3, 325 (1954).
- K. A. Müller and H. Burkard, Phys. Rev. B 19, 3593 (1979).
- M. Sendner, P. K. Nayak, D. A. Egger, S. Beck, C. Müller, B. Epding, W. Kowalsky, L. Kronik, H. J. Snaith, A. Pucci, and R. Lovrinčić, Mater. Horiz. 3, 613 (2016).
- I. Maeng, S. Chen, S. Lee, S. Wang, Y.-K. Kwon, and M.-C. Jung, Mater. Today Phys. 30, 100960 (2023).
- J. R. Knab, A. J. L. Adam, E. Shaner, H. J. A. J. Starmans, and P. C. M. Planken, Opt. Express 21, 1101 (2013).
- I. A. Kaplunov, G. I. Kropotov, V. E. Rogalin, and A. A. Shakhmin, Opt. Spectrosc. 129, 775 (2021).
- A. Fung, S. Heeba, Q. Liu, V. Muralidharan, K. Schutz, and A. C. Vincent, Phys. Rev. D 109, 083011 (2024).
- W. DeRocco, P. W. Graham, and S. Rajendran, Phys. Rev. D 102, 075015 (2020).
- S. Davidson, S. Hannestad, and G. Raffelt, J. High Energy Phys. 05 (2000) 003.
- P. Giannozzi et al., J. Phys. Condens. Matter 21, 395502 (2009).
- P. Giannozzi et al., J. Phys. Condens. Matter 29, 465901 (2017).
- A. Marronnier, G. Roma, S. Boyer-Richard, L. Pedesseau, J.-M. Jancu, Y. Bonnassieux, C. Katan, C. C. Stoumpos, M. G. Kanatzidis, and J. Even, ACS Nano 12, 3477 (2018).
- D. B. Straus, S. Guo, and R. J. Cava, J. Am. Chem. Soc. 141, 11435 (2019).
- A. Glazer, Acta Crystallogr. Sect. A 31, 756 (1975).
- H. J. Monkhorst and J. D. Pack, Phys. Rev. B 13, 5188 (1976).
- A. Togo, L. Chaput, T. Tadano, and I. Tanaka, J. Phys. Condens. Matter 35, 353001 (2023).
- A. Togo, J. Phys. Soc. Jpn. 92, 012001 (2023).
- R. M. Pick, M. H. Cohen, and R. M. Martin, Phys. Rev. B 1, 910 (1970).
- P. Giannozzi, S. de Gironcoli, P. Pavone, and S. Baroni, Phys. Rev. B 43, 7231 (1991).
- X. Gonze, J.-C. Charlier, D. Allan, and M. Teter, Phys. Rev. B 50, 13035 (1994).
- S. Knapen, T. Lin, M. Pyle, and K. M. Zurek, Phys. Lett. B 785, 386 (2018).
- H. An, M. Pospelov, J. Pradler, and A. Ritz, Phys. Lett. B 747, 331 (2015).
- Y. Hochberg, T. Lin, and K. M. Zurek, Phys. Rev. D 94, 015019 (2016).
- D. Trots and S. Myagkota, J. Phys. Chem. Solids 69, 2520 (2008).
- B.-B. Zhang, B. Xiao, S. Dong, and Y. Xu, J. Cryst. Growth 498, 1 (2018).
- P. Yang, J. Liao, B. Shen, P. Shao, H. Ni, and Z. Yin, J. Cryst. Growth 236, 589 (2002).
- S. Doyle, P. Mauskopf, J. Naylon, A. Porch, and C. Duncombe, J. Low Temp. Phys. 151, 530 (2008).
- E. S. Battistelli, F. Bellini, C. Bucci, M. Calvo, L. Cardani, N. Casali, M. Castellano, I. Colantoni, A. Coppolecchia, C. Cosmelli et al., Eur. Phys. J. C 75, 353 (2015).
- I. Colantoni, C. Bellenghi, M. Calvo, R. Camattari, L. Cardani, N. Casali, A. Cruciani, S. Di Domizio, J. Goupy, V. Guidi et al., J. Low Temp. Phys. 199, 593 (2020).
- A. Cruciani, L. Bandiera, M. Calvo, N. Casali, I. Colantoni, G. Del Castello, M. del Gallo Roccagiovine, D. Delicato, M. Giammei, V. Guidi, J. Goupy, V. Pettinacci, G. Pettinari, M. Romagnoni, M. Tamisari, A. Mazzolari, A. Monfardini, and M. Vignati, Appl. Phys. Lett. 121, 213504 (2022).
- L. R. Sletten, B. A. Moores, J. J. Viennot, and K. W. Lehnert, Phys. Rev. X 9, 021056 (2019).
- C. Kittel and P. McEuen, Introduction to Solid State Physics (John Wiley & Sons, New York, 2018).