- Open Access
Experimental search for electric dipole moments of light radioactive nuclei
Phys. Rev. D 112, 076031 – Published 23 October, 2025
DOI: https://doi.org/10.1103/hl5s-dqqw
Abstract
We discuss a search for the electric dipole moment (EDM) of a light beta-radioactive ion using a compact ion trap by adapting the “frozen-spin” method. The measurement will be done on ions stripped of their valence electrons, thereby bypassing the significant Schiff screening that hinders the application of successful contemporary EDM searches using heavy neutral atoms and molecules to light nuclei. We identified as the most promising candidate for a proof-of-concept EDM search and we estimate that the current indirect proton EDM limit of a few set by measurements can be surpassed with a week of measurement time at existing facilities.
Physics Subject Headings (PhySH)
Article Text
References (57)
- T. E. Chupp, P. Fierlinger, M. J. Ramsey-Musolf, and J. T. Singh, Electric dipole moments of atoms, molecules, nuclei, and particles, Rev. Mod. Phys. 91, 015001 (2019).
- G. Lüders, On the equivalence of invariance under time reversal and under particle-antiparticle conjugation for relativistic field theories, Dan. Mat. Fys. Medd. 28, 1 (1954), https://cds.cern.ch/record/1071765.
- A. Tureanu, and Lorentz invariance: Their relation and violation, J. Phys. Conf. Ser. 474, 012031 (2013).
- M. Kobayashi and T. Maskawa, violation in the renormalizable theory of weak interaction, Prog. Theor. Phys. 49, 652 (1973).
- A. Hocker, H. Lacker, S. Laplace, and F. L. Diberder, CKM matrix: Status and new developments, AIP Conf. Proc. 618, 27 (2002).
- M. Pospelov and A. Ritz, CKM benchmarks for electron electric dipole moment experiments, Phys. Rev. D 89, 056006 (2014).
- J. H. Smith, E. M. Purcell, and N. F. Ramsey, Experimental limit to the electric dipole moment of the neutron, Phys. Rev. 108, 120 (1957).
- J. Alexander et al., The storage ring proton EDM experiment, arXiv:2205.00830.
- F. Rathmann, A. Saleev, and N. N. Nikolaev, Search for electric dipole moments of light ions in storage rings, Phys. Part. Nucl. 45, 229 (2014).
- CERN Yellow Reports: Monographs, CERN yellow reports: Monographs, Vol. 3 (2021): Storage ring to search for electric dipole moments of charged particles: Feasibility study (2021).
- F. Rathmann, N. N. Nikolaev, and J. Slim, Spin dynamics investigations for the electric dipole moment experiment, Phys. Rev. Accel. Beams 23, 024601 (2020).
- S. Karanth et al., First search for axionlike particles in a storage ring using a polarized deuteron beam, Phys. Rev. X 13, 031004 (2023).
- B. Graner, Y. Chen, E. G. Lindahl, and B. R. Heckel, Reduced limit on the permanent electric dipole moment of Hg-199, Phys. Rev. Lett. 116, 161601 (2016).
- L. I. Schiff, Measurability of nuclear electric dipole moments, Phys. Rev. 132, 2194 (1963).
- A. Adelmann et al., A compact frozen-spin trap for the search for the electric dipole moment of the muon, Eur. Phys. J. C 85, 622 (2025).
- V. F. Dmitriev and R. A. Sen’kov, Schiff moment of the mercury nucleus and the proton dipole moment, Phys. Rev. Lett. 91, 212303 (2003).
- W. Gins et al., A new beamline for laser spin-polarization at ISOLDE, Nucl. Instrum. Methods Phys. Res., Sect. A 925, 24 (2019).
- T. Chupp and M. Ramsey-Musolf, Electric dipole moments: A global analysis, Phys. Rev. C 91, 035502 (2015).
- I. B. Khriplovich, Feasibility of search for nuclear electric dipole moments at ion storage rings, Phys. Lett. B 444, 98 (1998).
- Y. K. Semertzidis, A sensitive search for a muon electric dipole moment, in AIP Conference Proceedings (AIP, New York, 2001).
- F. J. M. Farley, K. Jungmann, J. P. Miller, W. M. Morse, Y. F. Orlov, B. L. Roberts, Y. K. Semertzidis, A. Silenko, and E. J. Stephenson, A new method of measuring electric dipole moments in storage rings, Phys. Rev. Lett. 93, 052001 (2004).
- P. Schmidt-Wellenburg, C. Calzolaio, A. Doinaki, C. Dutsov, M. Giovannozzi, T. Hume, and F. Trillaud, Preparations for a search of the muon EDM at PSI, EPJ Web Conf. 289, 01008 (2023).
- M. Sakurai et al., muEDM: Towards a search for the muon electric dipole moment at PSI using the frozen-spin technique, J. Phys. Soc. Jpn. 37, 020604 (2022).
- A. Adelmann et al., Search for a muon EDM using the frozen-spin technique, arXiv:2102.08838.
- P. Schmidt-Wellenburg, C. Calzolaio, R. Chakraborty, A. Doinaki, C. Dutsov, T. Hume, L. Morvaj, A. Papa, and M. Sakurai, Search for a muon EDM at the paul scherrer institute, Proc. Sci., Muon4Future2023 (2023) 018.
- I. B. Khriplovich, Electric dipole moments and ion storage rings, in Trapped Particles and Fundamental Physics, edited by S. N. Atutov, R. Calabrese, and L. Moi (Springer, Dordrecht, 2002), pp. 259–278.
- U. C. Bergmann et al., Light exotic isotopes: Recent beam developments and physics applications at ISOLDE, Nucl. Phys. A701, 363 (2002).
- L. H. Thomas, The motion of the spinning electron, Nature (London) 117, 514 (1926).
- L. H. Thomas, I. The kinematics of an electron with an axis, London, Edinburgh, Dublin Philos. Mag. J. Sci. 3, 1 (1927).
- V. Bargmann, L. Michel, and V. L. Telegdi, Precession of the polarization of particles moving in a homogeneous electromagnetic field, Phys. Rev. Lett. 2, 435 (1959).
- V. Anastassopoulos et al., A storage ring experiment to detect a proton electric dipole moment, Rev. Sci. Instrum. 87, 115116 (2016).
- From ENSDF database as of july 1, 2024. version available at http://www.nndc.bnl.gov/ensarchivals/ (2024), accessed on: July 1, 2024.
- T. J. Mertzimekis, K. Stamou, and A. Psaltis, An online database of nuclear electromagnetic moments, Nucl. Instrum. Methods Phys. Res., Sect. A 807, 56 (2016).
- T. J. Mertzimekis, Development of a dedicated online database for nuclear moments data, Technical Report No. INDC(NDS)-0704 (International Atomic Energy Agency (IAEA), 2016).
- The ISOLDE yield database, version 0.2, https://cern.ch/isolde-yields (2021), [Online; accessed 20.08.2024].
- J. Ballof, J. Ramos, A. Molander, K. Johnston, S. Rothe, T. Stora, and C. Düllmann, The upgraded isolde yield database—A new tool to predict beam intensities, Nucl. Instrum. Methods Phys. Res., Sect. B 463, 211 (2020).
- C. D. P. Levy, R. Baartman, J. A. Behr, A. Hatakeyama, Y. Hirayama, R. F. Kiefl, G. D. Morris, R. Nussbaumer, R. Poutissou, and G. W. Wight, A highly polarized ion beam at ISAC, in Polarized Sources and Targets (World Scientific, Singapore, 2002).
- T. Hume, R. Chakraborty, A. Doinaki, C. Dutsov, M. Giovannozzi, K. Michielsen, L. Morvaj, A. Papa, P. Schmidt-Wellenburg, and D. Stäger, Implementation of the frozen-spin technique for the search for a muon electric dipole moment, J. Instrum. 19, P01021 (2024).
- R. Catherall et al., The isolde facility, J. Phys. G 44, 094002 (2017).
- S. Lechner et al., Simulations of a cryogenic, buffer-gas filled paul trap for low-emittance ion bunches, Nucl. Instrum. Methods Phys. Res., Sect. A 1065, 169471 (2024).
- G. Guidoboni et al., How to reach a thousand-second in-plane polarization lifetime with deuterons in a storage ring, Phys. Rev. Lett. 117, 054801 (2016).
- S. Afach et al., Observation of gravitationally induced vertical striation of polarized ultracold neutrons by spin-echo spectroscopy, Phys. Rev. Lett. 115, 162502 (2015).
- G. Cavoto et al., Anomalous spin precession systematic effects in the search for a muon EDM using the frozen-spin technique, Eur. Phys. J. C 84, 262 (2024).
- T. Albahri et al., Magnetic-field measurement and analysis for the muon experiment at fermilab, Phys. Rev. A 103, 042208 (2021).
- D. P. Aguillard et al. (Muon Collaboration), Measurement of the positive muon anomalous magnetic moment to 127 ppb, Phys. Rev. Lett. 135, 101802 (2025).
- C. Abel et al., Measurement of the permanent electric dipole moment of the neutron, Phys. Rev. Lett. 124, 081803 (2020).
- M. V. Berry, Quantal phase factors accompanying adiabatic changes, Proc. R. Soc. A 392, 45 (1984).
- V. V. Flambaum, M. Pospelov, A. Ritz, and Y. V. Stadnik, Sensitivity of EDM experiments in paramagnetic atoms and molecules to hadronic violation, Phys. Rev. D 102, 035001 (2020).
- B. Graner, Y. Chen, E. G. Lindahl, and B. R. Heckel, Reduced limit on the permanent electric dipole moment of Hg199, Phys. Rev. Lett. 116, 161601 (2016); 119, 119901(E) (2017).
- A. van Hees, A. Wolters, and P. Glaudemans, Static moments and phenomenological interactions, Nucl. Phys. A476, 61 (1988).
- N. Yamanaka, Review of the electric dipole moment of light nuclei, Int. J. Mod. Phys. E 26, 1730002 (2017).
- N. Yamanaka, T. Yamada, and Y. Funaki, Nuclear electric dipole moment in the cluster model with a triton: and , Phys. Rev. C 100, 055501 (2019).
- J. Engel, Nuclear schiff moments and violation, Annu. Rev. Nucl. Part. Sci. 75, 129 (2025).
- O. Lebedev, K. A. Olive, M. Pospelov, and A. Ritz, Probing violation with the deuteron electric dipole moment, Phys. Rev. D 70, 016003 (2004).
- W. Dekens, J. de Vries, J. Bsaisou, W. Bernreuther, C. Hanhart, U.-G. Meißner, A. Nogga, and A. Wirzba, Unraveling models of violation through electric dipole moments of light nuclei, J. High Energy Phys. 07 (2014) 069.
- J. de Vries, E. Epelbaum, L. Girlanda, A. Gnech, E. Mereghetti, and M. Viviani, Parity- and time-reversal-violating nuclear forces, Front. Phys. 8, 18 (2020).
- http://www-nds.iaea.org/publications/indc/indc-nds-0704/.