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High sensitivity characterization of an ultrahigh purity NaI(Tl) crystal scintillator with the SABRE proof-of-principle detector

F. Calaprice1, S. Copello2, I. Dafinei3, D. D’Angelo4,5, G. D’Imperio3, G. Di Carlo6, M. Diemoz3, A. Di Giacinto6, A. Di Ludovico1 et al.

A. Ianni6, M. Iannone3, F. Marchegiani6, A. Mariani7,*, S. Milana3, S. Nisi6, F. Nuti8, D. Orlandi6, V. Pettinacci3, L. Pietrofaccia1, S. Rahatlou3,9, M. Souza1, B. Suerfu10,†, C. Tomei3, C. Vignoli6, M. Wada11, and A. Zani4

  • 1Physics Department, Princeton University, Princeton, New Jersey 08544, USA
  • 2Dipartimento di Fisica, Università degli Studi di Genova and INFN Genova, Genova I-16146, Italy
  • 3INFN—Sezione di Roma, Roma I-00185, Italy
  • 4INFN—Sezione di Milano, Milano I-20133, Italy
  • 5Dipartimento di Fisica, Università degli Studi di Milano, Milano I-20133, Italy
  • 6INFN—Laboratori Nazionali del Gran Sasso, Assergi (L’Aquila) I-67100, Italy
  • 7Gran Sasso Science Institute, L’Aquila I-67100, Italy
  • 8School of Physics, The University of Melbourne, Melbourne, Victoria 3010, Australia
  • 9Dipartimento di Fisica, Sapienza Università di Roma, Roma I-00185, Italy
  • 10University of California Berkeley, Department of Physics, Berkeley, California 94720, USA
  • 11AstroCeNT, Nicolaus Copernicus Astronomical Center of the Polish Academy of Sciences, Warsaw, Poland

  • *ambra.mariani@gssi.it
  • †suerfu@alumni.princeton.edu

Phys. Rev. D 104, L021302 – Published 9 July, 2021

DOI: https://doi.org/10.1103/PhysRevD.104.L021302

Abstract

We present new results on the radiopurity of a 3.4-kg NaI(Tl) crystal scintillator operated in the SABRE proof-of-principle detector setup. The amount of potassium contamination, determined by the direct counting of radioactive K40, is found to be 2.2±1.5  ppb, lowest ever achieved for NaI(Tl) crystals. With the active veto, the average background rate in the crystal in the 1–6 keV energy region of interest (ROI) is 1.20±0.05  counts/day/kg/keV, which is a breakthrough since the DAMA/LIBRA experiment. Our background model indicates that the rate is dominated by Pb210 and that about half of this contamination is located in the polytetrafluoroethylene reflector. We discuss ongoing developments of the crystal manufacture aimed at the further reduction of the background, including data from purification by zone refining. A projected background rate lower than ∼0.2  counts/day/kg/keV in the ROI is within reach. These results represent a benchmark for the development of next-generation NaI(Tl) detector arrays for the direct detection of dark matter particles.

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