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Magnetic diffuse scattering study of the dipolar-octupolar pyrochlore Ce2Sn2O7

B. Yuan1, M. Powell2, X. Liu1, J. Ni1, E. M. Smith1, R. Schäfer3, R. Moessner4, F. Ye5, J. Dudemaine6,7 et al.

A. D. Bianchi6,7,8, J. W. Kolis2, and B. D. Gaulin1,9,10

Phys. Rev. B 114, 154419 – Published 21 September, 2026

DOI: https://doi.org/10.1103/zz5z-gzzt

Abstract

We report diffuse scattering measurements on the dipolar-octupolar pyrochlore Ce2Sn2O7 to elucidate its magnetic correlations within the correlated paramagnetic regime above its ordering temperature TN∼40mK. The magnetic transition at TN, observed in recent specific heat measurements, has been interpreted within the nearest-neighbor XYZ model as a transition into an all-in-all-out (AIAO) magnetic order. However, the observed diffuse scattering above TN argues against an AIAO magnetic order by exhibiting no short-range order at the AIAO wave vectors, inconsistent with the nearest-neighbor model. Instead, the observed diffuse scattering strongly resembles that observed in classical dipolar spin ice, Dy2Ti2O7, and suggests the presence of short-range correlated structures such as chains or clusters in the low-energy manifold of Ce2Sn2O7, favored by further neighbor interactions. We discuss how chainlike states qualitatively account for the observed H-T phase diagram under a [1,1,0] field.

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