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Magnetic diffuse scattering study of the dipolar-octupolar pyrochlore
Phys. Rev. B 114, 154419 – Published 21 September, 2026
DOI: https://doi.org/10.1103/zz5z-gzzt
Abstract
We report diffuse scattering measurements on the dipolar-octupolar pyrochlore to elucidate its magnetic correlations within the correlated paramagnetic regime above its ordering temperature . The magnetic transition at , observed in recent specific heat measurements, has been interpreted within the nearest-neighbor XYZ model as a transition into an all-in-all-out (AIAO) magnetic order. However, the observed diffuse scattering above argues against an AIAO magnetic order by exhibiting no short-range order at the AIAO wave vectors, inconsistent with the nearest-neighbor model. Instead, the observed diffuse scattering strongly resembles that observed in classical dipolar spin ice, , and suggests the presence of short-range correlated structures such as chains or clusters in the low-energy manifold of , favored by further neighbor interactions. We discuss how chainlike states qualitatively account for the observed H-T phase diagram under a [1,1,0] field.