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    Elucidating the origin of long-range ferromagnetic order in Fe3GeTe2 by low-energy magnon excitation studies

    B. G. Beier1, E. S. Beier1, J. Arneth1, E. Brücher2, R. K. Kremer2, and R. Klingeler1,*

    • *Contact author: klingeler@kip.uni-heidelberg.de

    Phys. Rev. B 112, 214414 – Published 8 December, 2025

    DOI: https://doi.org/10.1103/zf74-j18j

    Abstract

    We report a detailed high-field/high-frequency ferromagnetic resonance (HF-FMR) study of low-energy magnon excitations in the van der Waals ferromagnet Fe2.92(1)Ge1.02(3)Te2. At 2K, the field dependence of the magnon branches is well described by a semiclassical domain-based model, from which we extract key microscopic parameters including the anisotropy gap Δ=170(4)GHz, the anisotropy field BA=5.85(8)T, and the effective g-factor gab=gc=2.07(4). Furthermore the uniaxial anisotropy constant is determined to be K=10.50(23)×106erg/cm3. Anisotropic short-range magnetic order persists above TC up to approximately 270K, as evidenced by a finite anisotropy gap and anisotropic shifts in the ferromagnetic resonance (FMR) resonance fields. Both results clearly show the presence of anisotropic local magnetic fields well above TC. Our findings underscore the crucial role of magnetocrystalline anisotropy in driving long-range magnetic order in Fe3GeTe2.

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