Elucidating the origin of long-range ferromagnetic order in by low-energy magnon excitation studies
Phys. Rev. B 112, 214414 – Published 8 December, 2025
DOI: https://doi.org/10.1103/zf74-j18j
Abstract
We report a detailed high-field/high-frequency ferromagnetic resonance (HF-FMR) study of low-energy magnon excitations in the van der Waals ferromagnet . At , the field dependence of the magnon branches is well described by a semiclassical domain-based model, from which we extract key microscopic parameters including the anisotropy gap , the anisotropy field , and the effective -factor . Furthermore the uniaxial anisotropy constant is determined to be . Anisotropic short-range magnetic order persists above up to approximately , as evidenced by a finite anisotropy gap and anisotropic shifts in the ferromagnetic resonance (FMR) resonance fields. Both results clearly show the presence of anisotropic local magnetic fields well above . Our findings underscore the crucial role of magnetocrystalline anisotropy in driving long-range magnetic order in .