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    Magnetic correlations and pairing tendencies of the hybrid stacking nickelate superlattice La7Ni5O17 (La3Ni2O7/La4Ni3O10) under pressure

    Yang Zhang1, Ling-Fang Lin1,*, Adriana Moreo1,2, Thomas A. Maier3,†, and Elbio Dagotto1,2,‡

    • *Contact author: lflin@utk.edu
    • †Contact author: maierta@ornl.gov
    • ‡Contact author: edagotto@utk.edu

    Phys. Rev. B 112, 024508 – Published 17 July, 2025

    DOI: https://doi.org/10.1103/t4zz-zbw1

    Abstract

    Motivated by the recent rapid progress in high-Tc nickelate superconductors, we comprehensively study the physical properties of the alternating bilayer trilayer stacking nickelate La7Ni5O17. The high-symmetry phase of this material, without the tilting of oxygen octahedra, is not stable at ambient conditions but becomes stable under high pressure, where a small hole pocket γ0, composed of the d3z2−r2 states in the trilayer sublattice, appears. This pocket was identified in our previous work for trilayer La4Ni3O10 as important to develop superconductivity. Moreover, using random-phase approximation calculations, we find a leading s± pairing state for the high-symmetry phase under pressure with similar pairing strength as that obtained previously for the bilayer La3Ni2O7 compound, suggesting a similar or higher superconducting transition temperature Tc, at the random-phase approximation level. In addition, we find that the dominant magnetic fluctuations in the system driving this pairing state have antiferromagnetic structure both in-plane and between the planes of the top and bottom trilayer and bilayer sublattices, while the middle trilayer is magnetically decoupled.

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    See Also

    Phase diagrams and two key factors to superconductivity of Ruddlesden-Popper nickelates

    Zhenfeng Ouyang, Rong-Qiang He, and Zhong-Yi Lu
    Phys. Rev. B 112, 045127 (2025)

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