Export citation

Export citation

Choose format for download:

Download Citation

    Phase diagrams and two key factors to superconductivity of Ruddlesden-Popper nickelates

    Zhenfeng Ouyang1,2, Rong-Qiang He1,2,*, and Zhong-Yi Lu1,2,3,†

    • 1School of Physics and Beijing Key Laboratory of Opto-electronic Functional Materials & Micro-nano Devices, Renmin University of China, Beijing 100872, China
    • 2Key Laboratory of Quantum State Construction and Manipulation (Ministry of Education), Renmin University of China, Beijing 100872, China
    • 3Hefei National Laboratory, Hefei 230088, China

    • *Contact author: rqhe@ruc.edu.cn
    • †Contact author: zlu@ruc.edu.cn

    Phys. Rev. B 112, 045127 – Published 17 July, 2025

    DOI: https://doi.org/10.1103/1412-nfzm

    Abstract

    The discovery of superconductivity in Ruddlesden-Popper (RP) nickelates has drawn great attention. Many works have been done to study the superconductivity as well as to find more superconducting RP nickelates. However, there is a lack of general understanding regarding the key factors that contribute to the superconductivity of RP nickelates. Here, we systematically study the series of RP nickelates under doping or high-pressure conditions by means of density functional theory plus dynamical mean-field theory. We find that enhanced quasiparticle weights and local spin fluctuation of the Ni−eg orbitals are commonly realized by hole doping or high pressure in the known superconducting RP nickelates, suggesting that they are crucial to the superconductivity. We also summarize experimentally synthesized RP nickelates into phase diagrams with local spin moment and local entanglement entropy as parameters, where phases of spin density wave/antiferromagnetism, superconductivity, and Fermi liquid are distinguished. At last, we predict a promising candidate for superconducting RP nickelates, which is constructed in a “bilayer-trilayer” stacking sequence.

    Physics Subject Headings (PhySH)

    See Also

    Magnetic correlations and pairing tendencies of the hybrid stacking nickelate superlattice La7Ni5O17 (La3Ni2O7/La4Ni3O10) under pressure

    Yang Zhang, Ling-Fang Lin, Adriana Moreo, Thomas A. Maier, and Elbio Dagotto
    Phys. Rev. B 112, 024508 (2025)

    Authorization Required

    We need you to provide your credentials before accessing this content.

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation