Voltage-driven breakdown of electronic order
Phys. Rev. B 114, 245101 – Published 1 October, 2026
DOI: https://doi.org/10.1103/nqcs-jd2g
Abstract
The voltage-driven breakdown of a Mott insulating state is a phenomenon where both interactions and nonequilibrium effects play crucial roles. This interesting effect has generated significant theoretical and experimental interest, and may also prove technologically relevant. Recent experiments have observed a sharp nonequilibrium insulator-to-metal transition accompanied by hysteresis, negative differential conductance, and lattice deformations, but the underlying breakdown mechanism is highly debated. Here, we describe a minimal lead-driven scenario in which the breakdown can arise from voltage-induced chemical pressure and explore its ramifications for a paradigmatic model of interacting spinless fermions on a chain coupled to metallic reservoirs (leads) and calculate the charge and current responses at the RPA level. We find a complex phase diagram where the nature of the breakdown depends on the strength of the interaction, leading to various current-carrying nonequilibrium phases. For weak to intermediate interaction strengths, we identify a conducting charge-density-wave (CDW) phase with a bias-dependent ordering wave vector. At large interaction strength, the breakdown leads to a charge-separated insulating phase. Additionally, we observe instances of hysteretic behavior, sharp current onset, and negative differential conductance. Our results can help shed light on recent experimental findings and unveil a clean reference mechanism for current-induced breakdown of electronic order.