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    Directional selection of field-induced phases by weak anisotropy in triangular-lattice K2Mn(SeO3)2

    Bin Wang1,2,3,*, Yantao Cao4,3,*, Andi Liu5,3, Guoliang Wu6, Jin Zhou5, Xiaobai Ma7, Wenyun Yang8, Takashi Ohhara9, Akiko Nakao10 et al.

    Koji Munakata10, Bing Shen1, Zhendong Fu3, Zhaoming Tian5, Qian Tao11, Zhu-an Xu11, Wei Li6, Jinkui Zhao2,†, and Hanjie Guo3,‡

    • *These authors contributed equally to this work.
    • †Contact author: jkzhao@gbu.edu.cn
    • ‡Contact author: hjguo@sslab.org.cn

    Phys. Rev. B 114, 204429 – Published 28 October, 2026

    DOI: https://doi.org/10.1103/npjh-dyyx

    Abstract

    Triangular-lattice systems host a variety of ground states, ranging from quantum spin liquids to magnetically ordered phases, the latter of which can exhibit a sequence of magnetic phase transitions under applied magnetic fields. Here, we report magnetic and thermodynamic measurements, combined with powder and single-crystal neutron diffraction, on a high-spin, nearly isotropic Mn2+ triangular-lattice system K2Mn(SeO3)2. The compound undergoes long-range magnetic ordering below TN∼4K in zero field. Contrary to expectations for an ideal Heisenberg system, an up-down-zero (UD0) magnetic structure is favored down to the lowest temperature (0.05 K), rather than the commonly expected Y-type structure. This UD0 state is, however, highly sensitive to external magnetic fields. For fields applied along the c axis, it is readily destabilized and replaced by the Y-type structure, followed by an up-up-down (UUD) phase corresponding to the 1/3 magnetization plateau. In contrast, when the field is applied within the triangular plane, the system evolves into a canted Y state at a higher critical field. These results reveal that weak anisotropy, though small in magnitude, exerts a strongly orientation-dependent influence, playing a key role in selecting the field-induced phases in this frustrated magnet.

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