- Editors' Suggestion
- Letter
- Open Access
Anharmonic collective oscillations and gap generation from thermal fluctuations in isotropic classical spin systems
Phys. Rev. B 113, L220411 – Published 23 June, 2026
DOI: https://doi.org/10.1103/h81q-rnry
Abstract
Spin waves are the fundamental excitations in magnetically ordered spin systems and are ubiquitously observed in magnetic materials. However, the standard understanding of spin waves as collective spin oscillations in an effective harmonic potential does not consider the possibility of soft modes, such as those due to an effective quartic potential. In this work, we show that such quartic potentials arise under very general conditions in a broad class of isotropic spin systems without a fine-tuning of the interaction parameters. Considering models with spin-spiral ground states in two and three spatial dimensions, we numerically demonstrate that quartic amplitude spin oscillations produce a fluctuation-induced spin-wave gap which grows with temperature according to a characteristic power-law. In conjunction with a phenomenological theory, the present work provides a general theoretical framework for describing soft spin modes. This framework generalizes earlier treatments of soft-spin dynamics and gap generation in order-by-disorder systems arising from accidental classical ground-state degeneracies, and highlights the important role of finite-size effects relevant to numerical studies. Our predictions of a temperature-dependent gap in spiral spin systems could be tested in inelastic neutron scattering experiments, providing direct spectroscopic evidence for thermal effects arising from soft spin modes in magnetic materials.
Physics Subject Headings (PhySH)
Article Text
Supplemental Material
References (40)
- P. Wölfle, Quasiparticles in condensed matter systems, Rep. Prog. Phys. 81, 032501 (2018).
- C. Kittel, Quantum Theory of Solids, 2nd ed. (Wiley, New York, NY, 1991).
- By “quartic potential”, we mean that the energy corresponding to a distortion of the state of the system with amplitude grows like with vanishing order (quadratic) contribution, such as in the problem of spiral order we consider in the present work. This should not be confused with order (quartic) quasiparticle (e.g., magnon-magnon) interactions arising beyond a linear spin-wave approximation.
- A. L. Fetter, Rotating vortex lattice in a Bose-Einstein condensate trapped in combined quadratic and quartic radial potentials, Phys. Rev. A 64, 063608 (2001).
- O. Gygi, H. G. Katzgraber, M. Troyer, S. Wessel, and G. G. Batrouni, Simulations of ultracold bosonic atoms in optical lattices with anharmonic traps, Phys. Rev. A 73, 063606 (2006).
- M. Lakshmanan and R. Sahadevan, Painlevé analysis, Lie symmetries, and integrability of coupled nonlinear oscillators of polynomial type, Phys. Rep. 224, 1 (1993).
- V. M. Bannur, P. K. Kaw, and J. C. Parikh, Statistical mechanics of quartic oscillators, Phys. Rev. E 55, 2525 (1997).
- T. Lan, C. W. Li, O. Hellman, D. S. Kim, J. A. Muñoz, H. Smith, D. L. Abernathy, and B. Fultz, Phonon quarticity induced by changes in phonon-tracked hybridization during lattice expansion and its stabilization of rutile , Phys. Rev. B 92, 054304 (2015).
- B. Wehinger, A. Bosak, and P. T. Jochym, Soft phonon modes in rutile , Phys. Rev. B 93, 014303 (2016).
- C. Csáki, C.-S. Guan, T. Ma, and J. Shu, Generating a Higgs potential quartic term, Phys. Rev. Lett. 124, 251801 (2020).
- N. Arkani-Hamed, A. G. Cohen, E. Katz, and A. E. Nelson, The littlest Higgs, J. High Energy Phys. 07 (2002) 034.
- N. Arkani-Hamed, A. G. Cohen, E. Katz, A. E. Nelson, T. Gregoire, and J. G. Wacker, The minimal moose for a little Higgs, J. High Energy Phys. 08 (2002) 021.
- J. G. Rau, P. A. McClarty, and R. Moessner, Pseudo-Goldstone gaps and order-by-quantum disorder in frustrated magnets, Phys. Rev. Lett. 121, 237201 (2018).
- M. Gohlke, L. E. Chern, H.-Y. Kee, and Y. B. Kim, Emergence of nematic paramagnet via quantum order-by-disorder and pseudo-Goldstone modes in Kitaev magnets, Phys. Rev. Res. 2, 043023 (2020).
- S. Khatua, M. J. P. Gingras, and J. G. Rau, Pseudo-Goldstone modes and dynamical gap generation from order by thermal disorder, Phys. Rev. Lett. 130, 266702 (2023).
- A. Hickey, J. G. Rau, S. Khatua, and M. J. P. Gingras, Universal temperature-dependent power law excitation gaps in frustrated quantum spin systems harboring order-by-disorder, arXiv:2505.18253.
- Y. V. Tymoshenko, Y. A. Onykiienko, T. Müller, R. Thomale, S. Rachel, A. S. Cameron, P. Y. Portnichenko, D. V. Efremov, V. Tsurkan, D. L. Abernathy, J. Ollivier, A. Schneidewind, A. Piovano, V. Felea, A. Loidl, and D. S. Inosov, Pseudo-Goldstone magnons in the frustrated Heisenberg helimagnet with a pyrochlore magnetic sublattice, Phys. Rev. X 7, 041049 (2017).
- D. S. Inosov, Y. O. Onykiienko, Y. V. Tymoshenko, A. Akopyan, D. Shukla, N. Prasai, M. Doerr, D. Gorbunov, S. Zherlitsyn, D. J. Voneshen, M. Boehm, V. Tsurkan, V. Felea, A. Loidl, and J. L. Cohn, Magnetic field dependence of low-energy magnons, anisotropic heat conduction, and spontaneous relaxation of magnetic domains in the cubic helimagnet , Phys. Rev. B 102, 184431 (2020).
- A. S. Sukhanov, Y. A. Onykiienko, R. Bewley, C. Shekhar, C. Felser, and D. S. Inosov, Magnon spectrum of the Weyl semimetal half-Heusler compound GdPtBi, Phys. Rev. B 101, 014417 (2020).
- E. Rastelli, A. Tassi, and L. Reatto, Nonsimple magnetic order for simple Hamiltonians, Physica B+C 97, 1 (1979).
- The absence of a phase transition in 2D follows from the Mermin-Wagner-Hohenberg theorem [29, 30]. Below a certain temperature, finite systems appear magnetically ordered when the correlation length becomes comparable to the system size. However, true long-range order is absent in the thermodynamic limit.
- L. Seabra, P. Sindzingre, T. Momoi, and N. Shannon, Novel phases in a square-lattice frustrated ferromagnet : -magnetization plateau, helicoidal spin liquid, and vortex crystal, Phys. Rev. B 93, 085132 (2016).
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/h81q-rnry for the analytical expansion of the energy of the quartic perturbation, details on the sMD and MC simulations, fitting procedures, additional data for the cubic lattice, and the derivation of the quartic oscillator frequency in the presence of the entropic term, which includes Refs. [31, 32, 33, 34, 35, 36, 37, 38].
- Accidental continuous ground-state degeneracies are known to occur in systems with fine-tuned interactions that display simpler ground-state wave vectors, such as and [39]. By considering systems with spin-spiral ground states, we avoid such accidental zero modes.
- B. J. Alder and T. E. Wainwright, Phase transition for a hard sphere system, J. Chem. Phys. 27, 1208 (1957).
- L. Savary, K. A. Ross, B. D. Gaulin, J. P. C. Ruff, and L. Balents, Order by quantum disorder in , Phys. Rev. Lett. 109, 167201 (2012).
- S. M. Rezende, Fundamentals of Magnonics (Springer, Berlin, 2020), Vol. 969.
- R. Lifshitz and M. C. Cross, Nonlinear dynamics of nanomechanical and micromechanical resonators, in Reviews of Nonlinear Dynamics and Complexity (John Wiley & Sons, Ltd, 2008), Chap. 1, pp. 1–52.
- N. D. Mermin and H. Wagner, Absence of ferromagnetism or antiferromagnetism in one- or two-dimensional isotropic Heisenberg models, Phys. Rev. Lett. 17, 1133 (1966).
- P. C. Hohenberg, Existence of long-range order in one and two dimensions, Phys. Rev. 158, 383 (1967).
- J. D. Alzate-Cardona, D. Sabogal-Suárez, R. F. L. Evans, and E. Restrepo-Parra, Optimal phase space sampling for Monte Carlo simulations of Heisenberg spin systems, J. Phys.: Condens. Matter 31, 095802 (2019).
- L. D. Landau and E. Lifshitz, On the theory of the dispersion of magnetic permeability in ferromagnetic bodies, Phys. Z. Sowjet. 8, 153 (1935).
- K. Ahnert and M. Mulansky, Boost C++ library: Odeint (2012).
- S. Zhang, H. J. Changlani, K. W. Plumb, O. Tchernyshyov, and R. Moessner, Dynamical structure factor of the three-dimensional quantum spin liquid candidate , Phys. Rev. Lett. 122, 167203 (2019).
- H. Suhl, The theory of ferromagnetic resonance at high signal powers, J. Phys. Chem. Solids 1, 209 (1957).
- E. Schlömann, Fine structure in the decline of the ferromagnetic resonance absorption with increasing power level, Phys. Rev. 116, 828 (1959).
- P. Krivosik and C. E. Patton, Hamiltonian formulation of nonlinear spin-wave dynamics: Theory and applications, Phys. Rev. B 82, 184428 (2010).
- T. Holstein and H. Primakoff, Field dependence of the intrinsic domain magnetization of a ferromagnet, Phys. Rev. 58, 1098 (1940).
- C. L. Henley, Ordering due to disorder in a frustrated vector antiferromagnet, Phys. Rev. Lett. 62, 2056 (1989).
- A. Fancelli, M. G. Gonzalez, S. Khatua, B. Lake, M. J. P. Gingras, J. G. Rau, and J. Reuther, Data for Figures in “Anharmonic collective oscillations and gap generation from thermal fluctuations in isotropic classical spin systems” [Data set], In Physical Review B, Zenodo, 2026, https://doi.org/10.5281/zenodo.20287611.