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    Evolution of pairing correlation with 3dz2 electron filling in a bilayer two-orbital model for La3Ni2O7

    Yufei Chen1, Yang Shen2, Xiangjian Qian1,3, Guang-Ming Zhang2,*, and Mingpu Qin1,4,†

    • *Contact author: zhanggm@shanghaitech.edu.cn
    • †Contact author: qinmingpu@sjtu.edu.cn

    Phys. Rev. B 114, 245132 – Published 26 October, 2026

    DOI: https://doi.org/10.1103/d5j5-tlh6

    Abstract

    The discovery of high-Tc superconductivity in pressurized bilayer nickelate La3Ni2O7 presents a new arena for exploring unconventional pairing mechanisms. A pivotal yet unresolved issue is the specific role of the 3dz2 orbital of Ni. While its interlayer superexchange antiferromagnetic coupling is widely considered crucial for superconductivity, the role of its itinerancy remains undetermined. Early studies showed that the superconductivity is accompanied by the emergence of a small Fermi pocket of 3dz2 orbitals. However, recent experiments show controversial results on the role of the 3dz2 Fermi pocket on superconductivity. Motivated by these experimental results, we investigate an effective bilayer two-orbital model for La3Ni2O7 using density-matrix renormalization group on a minimal one-dimensional geometry. By systematically varying the 3dz2 orbital filling from 1/12 doping to half filling, we observe a pronounced suppression of superconducting correlations near half filling. Our results demonstrate the itinerancy of the 3dz2 orbital is favorable for pairing in the bilayer two-orbital model for La3Ni2O7. Moreover, we observe that the pairing correlation is enhanced in regions where charge fluctuations are large, suggesting a competition between charge order and superconductivity in the model.

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