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Flat band in the multiband metal MnSb2

Carl Jonas Linnemann1, Davide Ceresoli2, Kim-Khuong Huynh1,*, and Martin Bremholm1,†

  • *Contact author: hkkhuong@chem.au.dk
  • †Contact author: bremholm@chem.au.dk

Phys. Rev. B 114, L231115 – Published 30 October, 2026

DOI: https://doi.org/10.1103/cp97-khvn

Abstract

We report the realization of a metallic flat band in the marcasite compound MnSb2. The material was synthesized under high pressure, and its crystal structure was established by x-ray diffraction. Electrical and thermoelectric transport measurements reveal signatures of a flat band near the Fermi level that persist across three structural, magnetic, and electronic transitions. These observations are supported by extensive density-functional-theory calculations. Related marcasite diantimonides, including FeSb2 and CrSb2, also host flat bands, but these lie far from the Fermi level and therefore do not produce a metallic flat-band state. MnSb2 therefore emerges as the only known metallic marcasite antimonide in which a flat band lies in the vicinity of the Fermi level.

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