Fermiology of the kagome compound probed by de Haas–van Alphen oscillations
Phys. Rev. B 114, 185132 – Published 28 September, 2026
DOI: https://doi.org/10.1103/cfgl-ggn6
Abstract
We report a detailed de Haas–van Alphen (dHvA) study of the recently discovered kagome metal using torque magnetometry, electrical transport, magnetization, and heat-capacity measurements. Temperature-dependent torque, resistivity, and heat capacity data reveal a charge density wave (CDW) transition at . The thermal hysteresis observed in both measurements establishes the first-order nature of the transition. Quantum oscillation measurements identify two major dHvA frequencies: and for a field applied within the ab plane, and their angular dependence is consistent with ellipsoidal Fermi surface (FS) pockets. Landau fan diagram analysis reveals evidence for a nontrivial Berry phase associated with the pocket, indicating possible nontrivial electronic topology in . Analysis of the temperature and magnetic field dependence of the oscillations using the Lifshitz-Kosevich formula yields electronic parameters that suggest anisotropic quantum transport properties. First-principles calculations provide further insight into the electronic structure, revealing Dirac-like band crossings, a flat band, and multiple van Hove singularities near the Fermi level. Our calculations based on the pristine phase cannot fully reproduce the experimentally observed quantum oscillation frequencies, suggesting that CDW-induced Fermi surface (FS) reconstruction plays a crucial role in the ground-state electronic structure of . These results provide new insight into the FS topology and electronic structure of , enriching our understanding of the electronic properties of kagome materials.