Pressure-induced resurgence of the superconducting transition in spinel thin films
Phys. Rev. B 111, 224512 – Published 23 June, 2025
DOI: https://doi.org/10.1103/blwl-l16s
Abstract
is a spinel superconductor with an optimal K recently discovered by employing superlattice engineering. Here, we study the pressure effect on the superconducting properties of thin films deposited on the ()-oriented substrate via measurements of resistance under various pressures up to 12 GPa. We find that the superconducting () displays a nonmonotonic evolution, i.e., it first shows a gradual decrease and then exhibits an enhancement above GPa, resulting in a V-shaped double dome with two maxima. In addition, our results reveal an interesting correlation between and the normal-state resistance, which exhibits an opposite trend with respect to (). Moreover, the extracted (0) that exceeds the Pauli limit and the obtained large Maki parameter α suggest that the dominant pair-breaking effect is a spin-paramagnetic channel in the measured pressure range. In this work, we not only demonstrate the potential to further raise of the Ti-based spinel superconductors but also offer more insight into the rich physics related to the superconducting mechanism of this family.