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    Pressure-induced resurgence of the superconducting transition in spinel MgTi2O4 thin films

    Lifen Shi1,2,*, Zhuang Ni1,2,*, Jun Hou1,2,*, Wei Hu1,2, Qian Li1,2, Pengtao Yang1,2, Bosen Wang1,2, Yoshiya Uwatoko3, Xiaoli Dong1,2 et al.

    Kui Jin1,2,†, Jianping Sun1,2,‡, and Jinguang Cheng1,2

    • *These authors contributed equally to this work.
    • †Contact author: kuijin@iphy.ac.cn
    • ‡Contact author: jpsun@iphy.ac.cn

    Phys. Rev. B 111, 224512 – Published 23 June, 2025

    DOI: https://doi.org/10.1103/blwl-l16s

    Abstract

    MgTi2O4 is a spinel superconductor with an optimal Tc≈5 K recently discovered by employing superlattice engineering. Here, we study the pressure effect on the superconducting properties of MgTi2O4 thin films deposited on the (00l)-oriented MgAl2O4 substrate via measurements of resistance under various pressures up to 12 GPa. We find that the superconducting Tc(P) displays a nonmonotonic evolution, i.e., it first shows a gradual decrease and then exhibits an enhancement above Pc∼3 GPa, resulting in a V-shaped double dome with two maxima. In addition, our results reveal an interesting correlation between Tc and the normal-state resistance, which exhibits an opposite trend with respect to Tc(P). Moreover, the extracted μ0Hc2(0) that exceeds the Pauli limit and the obtained large Maki parameter α suggest that the dominant pair-breaking effect is a spin-paramagnetic channel in the measured pressure range. In this work, we not only demonstrate the potential to further raise Tc of the Ti-based spinel superconductors but also offer more insight into the rich physics related to the superconducting mechanism of this family.

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