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    Electrical detection of the spin-flip transition in a metal/Na5Co15.5Te6O36 heterostructure

    Hirotsugu Tagami*, Takuya Kawada, and Yuki Shiomi

    • *Contact author: hirotsugu@g.ecc.u-tokyo.ac.jp

    Phys. Rev. B 114, 235123 – Published 19 October, 2026

    DOI: https://doi.org/10.1103/b1d1-ls28

    Abstract

    We report on the longitudinal magnetoresistance (MR) in thin metal films on an Ising-type antiferromagnetic insulator, Na5Co15.5Te6O36 (NCTO). Steep changes in the MR spectra with hysteresis were observed at spin-flip transitions driven by magnetic fields applied along the easy axis of the NCTO crystal. The MR jumps almost follow steplike changes in magnetization at the spin-flip transition. At very low temperatures where Co moments are partially frozen, the MR anomalies exhibit a tunnel-magnetoresistance-like shape. The observed MR anomalies at the spin-flip transition are attributed to strain effects via magnetostriction upon the magnetic-structure change of the Co nets in NCTO because similar MR jumps are observed in Pt/NCTO, Pt/SiOx/NCTO, and Cu/NCTO heterostructures. Interestingly, we find that the high-field slopes of the MR spectra show opposite signs between Pt/NCTO and Cu/NCTO at low temperatures. Because similar MR spectra are observed for Pt/SiOx/NCTO, in which the interface magnetic interaction is negligible, the weak antilocalization due to the strong spin-orbit interaction of the Pt films is likely to contribute to the low-temperature MR.

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